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1. High resolution diagnostic tools for superconducting radio frequency cavities

   https://doi.org/10.1063/5.0117868  

   Parajuli, I.; Ciovati, G.; Delayen, J. R. (November 2022, Review of Scientific Instruments)

   Superconducting radio-frequency (SRF) cavities are one of the fundamental building blocks of modern particle accelerators. To achieve the highest quality factors (1010–1011), SRF cavities are operated at liquid helium temperatures. Magnetic flux trapped on the surface of SRF cavities during cool-down below the critical temperature is one of the leading sources of residual RF losses. Instruments capable of detecting the distribution of trapped flux on the cavity surface are in high demand in order to better understand its relation to the cavity material, surface treatments and environmental conditions. We have designed, developed, and commissioned two high-resolution diagnostic tools to measure the distribution of trapped flux at the surface of SRF cavities. One is a magnetic field scanning system, which uses cryogenic Hall probes and anisotropic magnetoresistance sensors that fit the contour of a 1.3 GHz cavity. This setup has a spatial resolution of ∼13μm in the azimuthal direction and ∼1 cm along the cavity contour. The second setup is a stationary, combined magnetic and temperature mapping system, which uses anisotropic magnetoresistance sensors and carbon resistor temperature sensors, covering the surface of a 3 GHz SRF cavity. This system has a spatial resolution of 5 mm close to the iris and 11 mm at the equator. Initial results show a non-uniform distribution of trapped flux on the cavities’ surfaces, dependent on the magnitude of the applied magnetic field during field-cooling below the critical temperature. 

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2. Direct current magnetic Hall probe technique for measurement of field penetration in thin film superconductors for superconducting radio frequency resonators

   https://doi.org/10.1063/5.0083309  

   Senevirathne, I. H.; Gurevich, A.; Delayen, J. R. (May 2022, Review of Scientific Instruments)

   Superconducting Radio Frequency (SRF) cavities used in particle accelerators are typically formed from or coated with superconducting materials. Currently, high purity niobium is the material of choice for SRF cavities that have been optimized to operate near their theoretical field limits. This brings about the need for significant R & D efforts to develop next generation superconducting materials that could outperform Nb and keep up with the demands of new accelerator facilities. To achieve high quality factors and accelerating gradients, the cavity material should be able to remain in the superconducting Meissner state under a high RF magnetic field without penetration of quantized magnetic vortices through the cavity wall. Therefore, the magnetic field at which vortices penetrate a superconductor is one of the key parameters of merit of SRF cavities. Techniques to measure the onset of magnetic field penetration on thin film samples need to be developed to mitigate the issues with the conventional magnetometry measurements that are strongly influenced by the film orientation and shape and edge effects. In this work, we report the development of an experimental setup to measure the field of full flux penetration through films and multi-layered superconductors. Our system combines a small superconducting solenoid that can generate a magnetic field of up to 500 mT at the sample surface and three Hall probes to detect the full flux penetration through the superconductor. This setup can be used to study alternative materials that could potentially outperform niobium, as well as superconductor–insulator–superconductor (SIS) multilayer coatings on niobium. 

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3. Characterization of dissipative regions of a N-doped superconducting radio-frequency cavity

   https://doi.org/10.3389/femat.2023.1235918  

   Lechner, Eric M.; Oli, Basu Dev; Makita, Junki; Ciovati, Gianluigi; Gurevich, Alex; Iavarone, Maria (August 2023, Frontiers in Electronic Materials)

   We report radio-frequency measurements of quality factors and temperature mapping of a nitrogen doped Nb superconducting RF cavity. Cavity cutouts of hot and cold spots were studied with low temperature scanning tunneling microscopy and spectroscopy, X-ray photoelectron spectroscopy and secondary electron microscopy. Temperature mapping revealed a substantial reduction of the residual resistance upon cooling the cavity with a greater temperature gradient and hysteretic losses at the quench location, pointing to trapped vortices as the dominant source of residual surface resistance. Analysis of the tunneling spectra in the framework of a proximity effect theory shows that hot spots have a reduced pair potential and a wider distribution of the contact resistance between the Nb and the top Nb oxide. Alone, these degraded superconducting properties account for a much weaker excess dissipation as compared with the vortex contribution. Based on the correlation between the quasiparticle density of states and temperature mapping, we suggest that degraded superconducting properties may facilitate vortex nucleation or settling of trapped flux during cooling the cavity through the critical temperature. 

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4. MEASUREMENT OF THE MAGNETIC FIELD PENETRATION INTO SUPERCONDUCTING THIN FILMS

   https://doi.org/10.18429/JACoW-SRF2019-THP050  

   I. H. Senevirathne, G. Ciovati (November 2019, 19th Int. Conf. on RF Superconductivity, SRF2019, Dresden, Germany)

   The magnetic field at which first flux penetrates is a fundamental parameter characterizing superconducting materials for SRF cavities. Therefore, an accurate technique is needed to measure the penetration of the magnetic field directly. The conventional magnetometers are inconvenient for thin superconducting film measurements because these measurements are strongly influenced by orientation, edge and shape effects. In order to measure the onset of field penetration in bulk, thin films and multi-layered superconductors, we have designed, built and calibrated a system combining a small superconducting solenoid capable of generating surface magnetic field higher than 500 mT and Hall probe to detect the first entry of vortices. This setup can be used to study various promising alternative materials to Nb, especially SIS multilayer coatings on Nb that have been recently proposed to delay the vortex penetration in Nb surface. In this paper, the system will be described, and calibration will be presented. 

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5. Impact of submicron ${\mathrm{Nb}}_3\mathrm{Sn}$ stoichiometric surface defects on high-field superconducting radiofrequency cavity performance

   https://doi.org/10.1103/PhysRevResearch.6.043133  

   Willson, Sarah A; Harbick, Aiden V; Shpani, Liana; Do, Van; Lew-Kiedrowska, Helena; Liepe, Matthias U; Transtrum, Mark K; Sibener, S J (November 2024, Physical Review Research)

   ${\mathrm{Nb}}_3\mathrm{Sn}$film coatings have the potential to drastically improve the accelerating performance of Nb superconducting radiofrequency (SRF) cavities in next-generation linear particle accelerators. Unfortunately, persistent ${\mathrm{Nb}}_3\mathrm{Sn}$stoichiometric material defects formed during fabrication limit the cryogenic operating temperature and accelerating gradient by nucleating magnetic vortices that lead to premature cavity quenching. The SRF community currently lacks a predictive model that can explain the impact of chemical and morphological properties of ${\mathrm{Nb}}_3\mathrm{Sn}$defects on vortex nucleation and maximum accelerating gradients. Both experimental and theoretical studies of the material and superconducting properties of the first 100 nm of ${\mathrm{Nb}}_3\mathrm{Sn}$surfaces are complicated by significant variations in the volume distribution and topography of stoichiometric defects. This work contains a coordinated experimental study with supporting simulations to identify how the observed chemical composition and morphology of certain Sn-rich and Sn-deficient surface defects can impact the SRF performance. ${\mathrm{Nb}}_3\mathrm{Sn}$films were prepared with varying degrees of stoichiometric defects, and the film surface morphologies were characterized. Both Sn-rich and Sn-deficient regions were identified in these samples. For Sn-rich defects, we focus on elemental Sn islands that are partially embedded into the ${\mathrm{Nb}}_3\mathrm{Sn}$film. Using finite element simulations of the time-dependent Ginzburg-Landau equations, we estimate vortex nucleation field thresholds at Sn islands of varying size, geometry, and embedment. We find that these islands can lead to significant SRF performance degradation that could not have been predicted from the ensemble stoichiometry alone. For Sn-deficient ${\mathrm{Nb}}_3\mathrm{Sn}$surfaces, we experimentally identify a periodic nanoscale surface corrugation that likely forms because of extensive Sn loss from the surface. Simulation results show that the surface corrugations contribute to the already substantial drop in the vortex nucleation field of Sn-deficient ${\mathrm{Nb}}_3\mathrm{Sn}$surfaces. This work provides a systematic approach for future studies to further detail the relationship between experimental ${\mathrm{Nb}}_3\mathrm{Sn}$growth conditions, stoichiometric defects, geometry, and vortex nucleation. These findings have technical implications that will help guide improvements to ${\mathrm{Nb}}_3\mathrm{Sn}$fabrication procedures. Our outlined experiment-informed theoretical methods can assist future studies in making additional key insights about ${\mathrm{Nb}}_3\mathrm{Sn}$stoichiometric defects that will help build the next generation of SRF cavities and support related superconducting materials development efforts. Published by the American Physical Society2024 

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