Abstract. Anthropogenic aerosols (AAs) induce global and regionaltropospheric circulation adjustments due to the radiative energyperturbations. The overall cooling effects of AA, which mask a portion ofglobal warming, have been the subject of many studies but still have largeuncertainty. The interhemispheric contrast in AA forcing has also beendemonstrated to induce a major shift in atmospheric circulation. However,the zonal redistribution of AA emissions since start of the 20th century, with anotable decline in the Western Hemisphere (North America and Europe) and acontinuous increase in the Eastern Hemisphere (South Asia and East Asia),has received less attention. Here we utilize four sets of single-model initial-condition large-ensemblesimulations with various combinations of external forcings to quantify theradiative and circulation responses due to the spatial redistribution of AAforcing during 1980–2020. In particular, we focus on the distinct climateresponses due to fossil-fuel-related (FF) aerosols emitted from the Western Hemisphere (WH) versus the Eastern Hemisphere (EH). The zonal (west to east) redistribution of FF aerosol emission since the1980s leads to a weakening negative radiative forcing over the WHmid-to-high latitudes and an enhancing negative radiative forcing over theEH at lower latitudes. Overall, the FF aerosol leads to a northward shift of the Hadley cell and an equatorward shift of the Northernmore »
Two Distinct Modes of Climate Responses to the Anthropogenic Aerosol Forcing Changes
Unlike greenhouse gases (GHGs), anthropogenic aerosol (AA) concentrations have increased and then decreased over the past century or so, with the timing of the peak concentration varying in different regions. To date, it has been challenging to separate the climate impact of AAs from that due to GHGs and background internal variability. We use a pattern recognition method, taking advantage of spatiotemporal covariance information, to isolate the forced patterns for the surface ocean and associated atmospheric variables from the all-but-one forcing Community Earth System Model ensembles. We find that the aerosol-forced responses are dominated by two leading modes, with one associated with the historical increase and future decrease of global mean aerosol concentrations (dominated by the Northern Hemisphere sources) and the other due to the transition of the primary sources of AA from the west to the east and also from Northern Hemisphere extratropical regions to tropical regions. In particular, the aerosol transition effect, to some extent compensating the global mean effect, exhibits a zonal asymmetry in the surface temperature and salinity responses. We also show that this transition effect dominates the total AA effect during recent decades, e.g., 1967–2007.
- Award ID(s):
- 2048336
- Publication Date:
- NSF-PAR ID:
- 10367339
- Journal Name:
- Journal of Climate
- Volume:
- 35
- Issue:
- 11
- Page Range or eLocation-ID:
- p. 3445-3457
- ISSN:
- 0894-8755
- Publisher:
- American Meteorological Society
- Sponsoring Org:
- National Science Foundation
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