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1. Hot and Heterogenous High‐ ³ He/ ⁴ He Components: New Constraints From Proto‐Iceland Plume Lavas From Baffin Island

   https://doi.org/10.1029/2019GC008654  

   Willhite, Lori N.; Jackson, Matthew G.; Blichert‐Toft, Janne; Bindeman, Ilya; Kurz, Mark D.; Halldórsson, Sæmundur A.; Harðardóttir, Sunna; Gazel, Esteban; Price, Allison A.; Byerly, Benjamin L. (December 2019, Geochemistry, Geophysics, Geosystems)

   Abstract The Icelandic hotspot has erupted basaltic magma with the highest mantle‐derived³He/⁴He over a period spanning much of the Cenozoic, from the early‐Cenozoic Baffin Island‐West Greenland flood basalt province (49.8R_A), to mid‐Miocene lavas in northwest Iceland (40.2 to 47.5R_A), to Pleistocene lavas in Iceland's neovolcanic zone (34.3R_A). The Baffin Island lavas transited through and potentially assimilated variable amounts of Precambrian continental basement. We use geochemical indicators sensitive to continental crust assimilation (Nb/Th, Ce/Pb, MgO) to identify the least crustally contaminated lavas. Four lavas, identified as “least crustally contaminated,” have high MgO (>15 wt.%), and Nb/Th and Ce/Pb that fall within the mantle range (Nb/Th = 15.6 ± 2.6, Ce/Pb = 24.3 ± 4.3). These lavas have⁸⁷Sr/⁸⁶Sr = 0.703008–0.703021,¹⁴³Nd/¹⁴⁴Nd = 0.513094–0.513128,¹⁷⁶Hf/¹⁷⁷Hf = 0.283265–0.283284,²⁰⁶Pb/²⁰⁴Pb = 17.7560–17.9375,³He/⁴He up to 39.9R_A, and mantle‐like δ¹⁸O of 5.03–5.21‰. The radiogenic isotopic compositions of the least crustally contaminated lavas are more geochemically depleted than Iceland high‐³He/⁴He lavas, a shift that cannot be explained by continental crust assimilation in the Baffin suite. Thus, we argue for the presence oftwogeochemically distinct high‐³He/⁴He components within the Iceland plume. Additionally, the least crustally contaminated primary melts from Baffin Island‐West Greenland have higher mantle potential temperatures (1510 to 1630 °C) than Siqueiros mid‐ocean ridge basalts (1300 to 1410 °C), which attests to a hot, buoyant plume origin for early Iceland plume lavas. These observations support the contention that the geochemically heterogeneous high‐³He/⁴He domain is dense, located in the deep mantle, and sampled by only the hottest plumes. 

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2. Petrogenesis and Geodynamic Evolution in the Northern Westfjords, Iceland, Elucidated by Iceland's Oldest Silicic Rocks

   https://doi.org/10.1029/2022JB026265  

   Banik, Tenley J.; Coble, Matthew A.; Miller, Calvin F.; Fisher, Christopher M.; Jordan, Brennan T.; Vervoort, Jeffrey D.; Carley, Tamara L. (June 2023, Journal of Geophysical Research: Solid Earth)

   Abstract Iceland's oldest silicic rocks provide unique insight into the island's early crustal evolution. We present new zircon U‐Pb ages bolstered with zircon trace element and isotopic compositions, and whole rock Nd, Hf, and Pb isotope compositions, from three silicic magmatic centers—Hrafnsfjörður, Árnes, and Kaldalón—to understand the petrogenesis of large silicic volcanic centers in the northern Westfjords, Iceland. Our data confirm Hrafnsfjörður as the oldest known central volcano in Iceland (∼14 Ma) and establish an older age for Árnes (∼13 Ma) than previously estimated. We also report the first U‐Pb zircon dates from Kaldalón (∼13.5 Ma). Zircon oxygen isotope compositions range from δ¹⁸O∼+2 to +4‰ and indicate involvement of a low‐¹⁸O component in their source magmas. Hrafnsfjörður zircon Hf (mean sampleε_Hf∼ +15.3–16.0) and whole rock Hf and Nd (ε_Hf = +14.5 to +15;ε_Nd = +7.9 to +8.1) isotopic compositions are more radiogenic than those from Árnes (zircon sampleε_Hf∼ +11.8–13; whole rockε_Hf = +12.8 to +15.1;ε_Nd = +7.3 to +7.7), but Hrafnsfjörður whole rock Pb isotope compositions (^208/204Pb = 37.95–37.96;^206/204Pb = 18.33–18.35) are less radiogenic than those from Árnes (^208/204Pb = 38.34–38.48;^206/204Pb = 18.64–18.78). Kaldalón has zircon Hf isotope compositions ofε_Hf∼+14.8 and 15.5 (sample means). These age and isotopic differences suggest that interaction of rift and plume, and thus the geodynamic evolution of the Westfjords, is complex. Isotopic compositions of Hrafnsfjörður and Árnes support involvement of an enriched mantle (EM)‐like mantle component associated with a pulsing plume that resulted in variable spreading rates and magma fluxes and highlight the heterogeneity of the Icelandic mantle. 

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3. Eruption Rates, Tempo, and Stratigraphy of Paleocene Flood Basalts on Baffin Island, Canada

   https://doi.org/10.1029/2021GC010172  

   Biasi, Joseph; Asimow, Paul; Horton, Forrest; Boyes, Xenia (September 2022, Geochemistry, Geophysics, Geosystems)

   Abstract High‐temperature melting in mantle plumes produces voluminous eruptions that are often temporally coincident with mass extinctions. Paleocene Baffin Island lavas—products of early Iceland mantle plume activity—are exceptionally well characterized geochemically but have poorly constrained stratigraphy, geochronology, and eruptive tempos. To provide better geologic context, we measured seven stratigraphic sections of the volcanic deposits and collected paleomagnetic data from 38 sites in the lavas and underlying Cretaceous sediments (Quqaluit Fm.). The average paleomagnetic pole from this study does not overlap with the expected pole for a stable North American locality at 60 Ma, yet the data have sufficient dispersion to average out secular variation. After ruling out other possibilities, we find that the picrites were probably erupted during a polarity transition, over less than 5 kyr. If so, the average eruption interval was ∼67 years per flow for the thickest sequence of exposed lavas. We also calculate that the flood basalts had a minimum total volume of ∼176 km³(excluding submerged lavas in Baffin Bay). This implies a minimum eruption rate of ∼0.035 km³ yr⁻¹, which is similar to rates found in West Greenland lavas but less than rates found in larger flood basalts. Despite this, the Baffin and West Greenland lavas temporally correlate with the “End C27n event” (a period of ∼2°C global warming) and may be its underlying cause. 

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4. Insights into the Early Volcanic History of the Walvis Ridge recorded by Chemostratigraphy: Preliminary Data IODP Expedition 391 Site U1575

   Nelson, Wendy R; Greenwald, Z; Bowers, R; Shervais, J S; Potter, K E; White, D; Scholpp, J; Widdowson, M; Tshiningayamwe, M; Hoernle, K; et al (December 2023, American Geophysical Union)

   The Walvis Ridge system consists of a series of seamounts, ridges, and plateaus formed during the opening of the southern Atlantic Ocean since ~135 Ma. International Ocean Discovery Program Expeditions (IODP) 391 and 397T drilled six sites along the length of the hotspot track to understand the magmatic processes associated with evolving plume-ridge systems. The oldest drilled segment of the ridge system – Frio Ridge – extends from the Etendeka flood basalts in Namibia westward into the Atlantic Ocean. Site U1575 is on the Frio Ridge and is the closest site to the African continent. The site drilled 118.9 m of igneous basement with 70.7 m (59.5%) of recovery. The recovered core consisted of alternating sequences of submarine pillow lavas and sheet flows, some of which were massive (up to 21 m thick). Preliminary major and trace element data demonstrate the basaltic lavas are fractionated (MgO = 4.8-6.4 wt. %) with modest TiO2 contents (1.5-2.7 wt. %). The upper 52 m of igneous section (214-267 mbsf) are geochemically consistent throughout the various eruptive styles. However, an abrupt compositional shift to lavas with lower incompatible element abundances (TiO2, Zr, Sr, Nb, La, etc.) from 274-311 mbsf demonstrates a clear shift in magmatic source contributions. Below this, the lavas return to compositions similar to the upper portion of the hole. Shipboard natural gamma radiation (NGR) and magnetic susceptibility (MS) measurements correlate with mineralogical and compositional changes. Specifically, decreases in NGR correlate well with decreases in K2O, Sr, Y, and Zr. MS is positively correlated with zones containing olivine. Trace element discrimination plots demonstrate a dual character: Ti-V relationships are strongly MORB-like while Th/Nb suggests the lavas have both MORB and plume characteristics, consistent with the formation of the Frio Ridge through plume-ridge interaction. Elevated Zr/Nb and Y/Nb values are also consistent with a hybrid source. The composition of this core contrasts sharply with cores recovered from the younger Guyot Province to the southwest. Sites U1578 and U1585 have episodes of higher TiO2 contents (>3.5 wt. %) with trace element signatures (e.g. low Zr/Nb & Y/Nb) indicative of a pronounced plume component, consistent with an intraplate setting for the formation of the Guyot Province. 

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5. Oxygen isotope (δ18O, Δ′17O) insights into continental mantle evolution since the Archean

   https://doi.org/10.1038/s41467-022-31586-9  

   Bindeman, Ilya N.; Ionov, Dmitri A.; Tollan, Peter M. E.; Golovin, Alexander V. (July 2022, Nature Communications)

   Abstract Oxygen isotopic ratios are largely homogenous in the bulk of Earth’s mantle but are strongly fractionated near the Earth’s surface, thus these are robust indicators of recycling of surface materials to the mantle. Here we document a subtle but significant ~0.2‰ temporal decrease in δ¹⁸O in the shallowest continental lithospheric mantle since the Archean, no change in Δ′¹⁷O is observed. Younger samples document a decrease and greater heterogeneity of δ¹⁸O due to the development and progression of plate tectonics and subduction. We posit that δ¹⁸O in the oldest Archean samples provides the best δ¹⁸O estimate for the Earth of 5.37‰ for olivine and 5.57‰ for bulk peridotite, values that are comparable to lunar rocks as the moon did not have plate tectonics. Given the large volume of the continental lithospheric mantle, even small decreases in its δ¹⁸O may explain the increasing δ¹⁸O of the continental crust since oxygen is progressively redistributed by fluids between these reservoirs via high-δ¹⁸O sediment accretion and low-δ¹⁸O mantle in subduction zones. 

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