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We report on an all-optical investigation of coupled spin excitation modes in a series of magnetic trilayer structures. Using time-resolved magneto-optic Kerr effect (tr-MOKE) magnetometry, we observe multi-mode coherent spin excitations in [Formula: see text]/Ru/[Formula: see text] multilayers even though the tr-MOKE optical detection is sensitive only to the [Formula: see text] magnetization dynamics. Frequency shifts of the different modes indicate that the coupling between the [Formula: see text] and [Formula: see text] layers varies from anti-ferromagnetic to ferromagnetic to uncoupled as the Ru spacer layer thickness is increased from 8 Å to 200 Å. The lifetime of the high frequency coherent oscillations in the [Formula: see text] layer increases by over 200%–300% even in the case of uncoupled [Formula: see text] and [Formula: see text] layers with a 200 Å thick Ru spacer. The results suggest an additional method to decrease the damping of high-moment alloys in layered magnetic nanostructures.
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Tunable coupling in magnetic thin film heterostructures with a magnetic phase transition
Abstract The magnetic properties of permalloy-based trilayers of the form Py 0.8 Cu 0.2 /Py 0.4 Cu 0.6 /Py/IrMn were studied as the spacer layer undergoes a paramagnetic to ferromagnetic phase transition. We find the coupling between the free Py 0.8 Cu 0.2 layer and the exchange bias pinned Py to be strongly temperature-dependent: there is negligible coupling above the Curie temperature of the Py 0.4 Cu 0.6 spacer layer, strong ferromagnetic coupling below that temperature, and a tunable coupling between these extremes. Polarized neutron reflectometry was used to measure the depth profile of the magnetic order in the system, allowing us to correlate the order parameter with the coupling strength. The thickness dependence shows that these are interface effects with an inverse relationship to thickness, and that there is a magnetic proximity effect that enhances the Curie temperature of the spacer layer with characteristic length scale of about 7 nm. As a demonstration of potential functionality of such a system, the structure is shown to spontaneously flip from the antiparallel to parallel magnetic configuration once the spacer layer has developed long-range magnetic order.
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- Award ID(s):
- 1609066
- PAR ID:
- 10425048
- Date Published:
- Journal Name:
- Scientific Reports
- Volume:
- 13
- Issue:
- 1
- ISSN:
- 2045-2322
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1038/s41598-023-34322-5
