An official website of the United States government
Abstract Accurate characterization of an attosecond pulse from streaking trace is an indispensable step in studying the ultrafast electron dynamics on the attosecond scale. Conventional attosecond pulse retrieval methods face two major challenges: the ability to incorporate a complete physics model of the streaking process, and the ability to model the uncertainty of pulse reconstruction in the presence of noise. Here we propose a pulse retrieval method based on conditional variational generative network (CVGN) that can address both demands. Instead of learning the inverse mapping from a streaking trace to a pulse profile, the CVGN models the distribution of the pulse profile conditioned on a given streaking trace measurement, and is thus capable of assessing the uncertainty of the retrieved pulses. This capability is highly desirable for low-photon level measurement, which is typical in attosecond streaking experiments in the water window X-ray range. In addition, the proposed scheme incorporates a refined physics model that considers the Coulomb-laser coupling and photoelectron angular distribution in streaking trace generation. CVGN pulse retrievals under various simulated noise levels and experimental measurement have been demonstrated. The results showed high pulse reconstruction consistency for streaking traces when peak signal-to-noise ratio (SNR) exceeds 6, which could serve as a reference for future learning-based attosecond pulse retrieval.
more »
« less
Electron bunch dynamics and emission in particle-in-cell simulations of relativistic laser–solid interactions: On density artifacts, collisions, and numerical dispersion
Sub-optical-cycle dynamics of dense electron bunches in relativistic-intensity laser–solid interactions lead to the emission of high-order harmonics and attosecond light pulses. The capacity of particle-in-cell simulations to accurately model these dynamics is essential for the prediction of emission properties because the attosecond pulse intensity depends on the electron density distribution at the time of emission and on the temporal distribution of individual electron Lorentz-factors in an emitting electron bunch. Here, we show that in one-dimensional collisionless simulations, the peak density of the emitting electron bunch increases with the increase in the spatial resolution of the simulation grid. When collisions are added to the model, the peak electron density becomes independent of the spatial resolution. Collisions are shown to increase the spread of the peaks of Lorentz-factors of emitting electrons in time, especially in the regimes far from optimum generation conditions, thus leading to lower intensities of attosecond pulses as compared to those obtained in collisionless simulations.
more »
« less
- Award ID(s):
- 2206711
- PAR ID:
- 10425129
- Date Published:
- Journal Name:
- Physics of Plasmas
- Volume:
- 30
- Issue:
- 6
- ISSN:
- 1070-664X
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Context. There has been significant technological and scientific progress in our ability to detect, monitor, and model the physics of γ -ray bursts (GRBs) over the 50 years since their first discovery. However, the dissipation process thought to be responsible for their defining prompt emission is still unknown. Recent efforts have focused on investigating how the ultrarelativistic jet of the GRB propagates through the progenitor’s stellar envelope for different initial composition shapes, jet structures, magnetisation, and, consequently, possible energy dissipation processes. Study of the temporal variability – in particular the shortest duration of an independent emission episode within a GRB – may provide a unique way to distinguish the imprint of the inner engine activity from geometry and propagation related effects. The advent of new high-energy detectors with exquisite time resolution now makes this possible. Aims. We aim to characterise the minimum variability timescale (MVT) defined as the shortest duration of individual pulses that shape a light curve for a sample of GRBs in the keV–MeV energy range and test correlations with other key observables such as the peak luminosity, the Lorentz factor, and the jet opening angle. We compare these correlations with predictions from recent numerical simulations for a relativistic structured – possibly wobbling – jet and assess the value of temporal variability studies as probes of prompt-emission dissipation physics. Methods. We used the peak detection algorithm MEPSA to identify the shortest pulse within a GRB time history and preliminarily calibrated MEPSA to estimate the full width at half maximum duration. We then applied this framework to two sets of GRBs: Swift GRBs (from 2005 to July 2022) and Insight Hard Modulation X-ray Telescope (Insight-HXMT) GRBs (from June 2017 to July 2021, including the exceptional 221009A). We then selected 401 GRBs with measured redshift to test for correlations. Results. We confirm that, on average, short GRBs have significantly shorter MVTs than long GRBs. The MVT distribution of short GRBs with extended emission such as 060614 and 211211A is compatible only with that of short GRBs. This is important because it provides a new clue concerning the progenitor’s nature. The MVT for long GRBs with measured redshift anti-correlates with peak luminosity; our analysis includes careful evaluation of selection effects. We confirm the anti-correlation with the Lorentz factor and find a correlation with the jet opening angle as estimated from the afterglow light curve, along with an inverse correlation with the number of pulses. Conclusions. The MVT can identify the emerging putative new class of long GRBs that are suggested to be produced by compact binary mergers. For otherwise typical long GRBs, the different correlations between MVT and peak luminosity, Lorentz factor, jet opening angle, and number of pulses can be explained within the context of structured, possibly wobbling, weakly magnetised relativistic jets.more » « less
-
Accelerator-based x-ray free-electron lasers (XFELs) are the latest addition to the revolutionary tools of discovery for the 21st century. The two major components of an XFEL are an accelerator-produced electron beam and a magnetic undulator, which tend to be kilometer-scale long and expensive. A proof-of-principle demonstration of free-electron lasing at 27 nm using beams from compact laser wakefield accelerators was shown recently by using a magnetic undulator. However, scaling these concepts to x-ray wavelengths is far from straightforward as the requirements on the beam quality and jitters become much more stringent. Here, we present an ultracompact scheme to produce tens of attosecond x-ray pulses with several GW peak power utilizing a novel aspect of the FEL instability using a highly chirped, prebunched, and ultrabright tens of MeVelectron beam from a plasma-based accelerator interacting with an optical undulator. The FEL resonant relation between the prebunched period and the energy selects resonant electrons automatically from the highly chirped beam which leads to a stable generation of attosecond x-ray pulses. Furthermore, two-color attosecond pulses with subfemtosecond separation can be produced by adjusting the energy distribution of the electron beam so that multiple FEL resonances occur at different locations within the beam. Such a tunable coherent attosecond x-ray sources may open up a new area of attosecond science enabled by x-ray attosecond pump/probe techniquesmore » « less
-
Efforts to push the spatiotemporal imaging-resolution limits of femtosecond laser-driven ultrafast electron microscopes (UEMs) to the combined angstrom–fs range will benefit from stable sources capable of generating high bunch charges. Recent demonstrations of unconventional off-axis photoemitting geometries are promising, but connections to the observed onset of structural dynamics are yet to be established. Here we use the in-situ photoexcitation of coherent phonons to quantify the relative time-of-flight (r-TOF) of photoelectron packets generated from the Ni Wehnelt aperture and from a Ta cathode set-back from the aperture plane. We further support the UEM experiments with particle-tracing simulations of the precise electron-gun architecture and photoemitting geometries. In this way, we measure discernible shifts in electron-packet TOF of tens of picoseconds for the two photoemitting surfaces. These shifts arise from the impact that the Wehnelt-aperture off-axis orientation has on the electron-momentum distribution, which modifies both the collection efficiency and the temporal-packet distribution relative to on-axis emission. Future needs are identified; we expect this and other developments in UEM electron-gun configuration to expand the range of material phenomena that can be directly imaged on scales commensurate with fundamental structural dynamics.more » « less
-
null (Ed.)Measuring the attosecond movement of electrons in molecules is challenging due to the high temporal and spatial resolutions required. X-ray scattering-based methods are promising, but many questions remain concerning the sensitivity of the scattering signals to changes in density, as well as the means of reconstructing the dynamics from these signals. In this paper, we present simulations of stationary core-holes and electron dynamics following inner-shell ionization of the oxazole molecule. Using a combination of time-dependent density functional theory simulations along with X-ray scattering theory, we demonstrate that the sudden core-hole ionization produces a significant change in the X-ray scattering response and how the electron currents across the molecule should manifest as measurable modulations to the time dependent X-ray scattering signal. This suggests that X-ray scattering is a viable probe for measuring electronic processes at time scales faster than nuclear motion.more » « less
- Free Publicly Accessible Full Text
-
Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1063/5.0140028
