skip to main content


This content will become publicly available on May 1, 2024

Title: Measurement of isotopic separation of argon with the prototype of the cryogenic distillation plant Aria for dark matter searches
Abstract The Aria cryogenic distillation plant, located in Sardinia, Italy, is a key component of the DarkSide-20k experimental program for WIMP dark matter searches at the INFN Laboratori Nazionali del Gran Sasso, Italy. Aria is designed to purify the argon, extracted from underground wells in Colorado, USA, and used as the DarkSide-20k target material, to detector-grade quality. In this paper, we report the first measurement of argon isotopic separation by distillation with the 26 m tall Aria prototype. We discuss the measurement of the operating parameters of the column and the observation of the simultaneous separation of the three stable argon isotopes: $${}^{36}\hbox {Ar}$$ 36 Ar , $${}^{38}\textrm{Ar}$$ 38 Ar , and $${}^{40}\textrm{Ar}$$ 40 Ar . We also provide a detailed comparison of the experimental results with commercial process simulation software. This measurement of isotopic separation of argon is a significant achievement for the project, building on the success of the initial demonstration of isotopic separation of nitrogen using the same equipment in 2019.  more » « less
Award ID(s):
1935947 2131857 1812540 1812453 1812482
NSF-PAR ID:
10429061
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; more » ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; « less
Date Published:
Journal Name:
The European Physical Journal C
Volume:
83
Issue:
5
ISSN:
1434-6052
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. Abstract

    Aria is a plant hosting a$${350}\,\hbox {m}$$350mcryogenic isotopic distillation column, the tallest ever built, which is being installed in a mine shaft at Carbosulcis S.p.A., Nuraxi-Figus (SU), Italy. Aria is one of the pillars of the argon dark-matter search experimental program, lead by the Global Argon Dark Matter Collaboration. It was designed to reduce the isotopic abundance of$${^{39}\hbox {Ar}}$$39Arin argon extracted from underground sources, called Underground Argon (UAr), which is used for dark-matter searches. Indeed,$${^{39}\hbox {Ar}}$$39Aris a$$\beta $$β-emitter of cosmogenic origin, whose activity poses background and pile-up concerns in the detectors. In this paper, we discuss the requirements, design, construction, tests, and projected performance of the plant for the isotopic cryogenic distillation of argon. We also present the successful results of the isotopic cryogenic distillation of nitrogen with a prototype plant.

     
    more » « less
  2. null (Ed.)
    Finding unambiguous evidence of dark matter interactions in a particle detector is a main objective of physics research. The liquid argon time projection chamber technique for the detection of Weakly Interacting Massive Particles (WIMP) allows sensitivities down to the so-called neutrino floor for high and low WIMP masses. Based on the successful operation of the DarkSide-50 detector, a new and more sensitive experiment, DarkSide-20k, was designed and is now under construction. A thorough understanding of the DarkSide-50 detector response to events classified as dark matter as well as all other interactions is essential for an optimal design of the new experiment. In this paper, we report on a particular set of events, for which scintillation-ionization signals are observed in association with signals from single or few isolated electrons. We identified and provided an interpretation for two event types in which electrons are produced via photoelectric effect on the cathode electrode and in the bulk liquid. Events with photoelectric emissions are observed in association with most interactions with large energy depositions in the detector. From the measured rate of these events, we determine the photo-ionization probability, or photoelectric quantum efficiency, of tetraphenyl butadiene (TPB) at wavelengths around 128 nm. 
    more » « less
  3. Abstract

    The Hamburg meteorite fell on January 16, 2018, near Hamburg, Michigan, after a fireball event widely observed in the U.S. Midwest and in Ontario, Canada. Several fragments fell onto frozen surfaces of lakes and, thanks to weather radar data, were recovered days after the fall. The studied rock fragments show no or little signs of terrestrial weathering. Here, we present the initial results from an international consortium study to describe the fall, characterize the meteorite, and probe the collision history of Hamburg. About 1 kg of recovered meteorites was initially reported. Petrology, mineral chemistry, trace element and organic chemistry, and O and Cr isotopic compositions are characteristic of H4 chondrites. Cosmic ray exposure ages based on cosmogenic3He,21Ne, and38Ar are ~12 Ma, and roughly agree with each other. Noble gas data as well as the cosmogenic10Be concentration point to a small 40–60 cm diameter meteoroid. An40Ar‐39Ar age of 4532 ± 24 Ma indicates no major impact event occurring later in its evolutionary history, consistent with data of other H4 chondrites. Microanalyses of phosphates with LA‐ICPMS give an average Pb‐Pb age of 4549 ± 36 Ma. This is in good agreement with the average SIMS Pb‐Pb phosphate age of 4535.3 ± 9.5 Ma and U‐Pb Concordia age of 4535 ± 10 Ma. The weighted average age of 4541.6 ± 9.5 Ma reflects the metamorphic phosphate crystallization age after parent body formation in the early solar system.

     
    more » « less
  4. Abstract

    White micas are major rock forming minerals in igneous and metamorphic rocks, and their chemical and isotopic variations can be used to determine pressure, temperature and time (P‐T‐t) histories. We apply40Ar/39Ar multi‐diffusion domain modelling to white micas from blueschists blocks in serpentinite matrix mélange from the exhumed Baja California subduction complex. Thermal history models yielded T‐t paths suggesting that40Ar* resides within multiple diffusion domains with varying40Ar* retentivity. Modelled white mica thermal histories and thermobarometric data were used to forward model continuous P‐T‐t paths. P‐T‐t paths are consistent with previous studies and are interpreted to constrain blueschist block exhumation paths within the Baja accretionary wedge. Our P‐T‐t models use temperature controlled40Ar/39Ar step heat data in which argon loss by volume diffusion can be demonstrated, and for which the white mica petrogenesis is known.

     
    more » « less
  5. null (Ed.)
    The continental crust is a major geochemical reservoir, the evolution of which has shaped the surface environment of Earth. In this study, we present a new model of coupled crust-mantle-atmosphere evolution to constrain the growth of continental crust with atmospheric 40 Ar/ 36 Ar. Our model is the first to combine argon degassing with the thermal evolution of Earth in a self-consistent manner and to incorporate the effect of crustal recycling and reworking using the distributions of crustal formation and surface ages. Our results suggest that the history of argon degassing favors rapid crustal growth during the early Earth. The mass of continental crust, highly enriched in potassium, is estimated to have already reached >80% of the present-day level during the early Archean. The presence of such potassium-rich, likely felsic, crust has important implications for tectonics, surface environment, and the regime of mantle convection in the early Earth. 
    more » « less