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1. The Key Role of Coupled Chemistry–Climate Interactions in Tropical Stratospheric Temperature Variability

   https://doi.org/10.1175/JCLI-D-20-0071.1  

   Yook, Simchan; Thompson, David W.; Solomon, Susan; Kim, Seo-Yeon (September 2020, Journal of Climate)

   null (Ed.)

   Abstract The purpose of this study is to quantify the effects of coupled chemistry–climate interactions on the amplitude and structure of stratospheric temperature variability. To do so, the authors examine two simulations run on version 4 of the Whole Atmosphere Coupled Climate Model (WACCM): a “free-running” simulation that includes fully coupled chemistry–climate interactions and a “specified chemistry” version of the model forced with prescribed climatological-mean chemical composition. The results indicate that the inclusion of coupled chemistry–climate interactions increases the internal variability of temperature by a factor of ~2 in the lower tropical stratosphere and—to a lesser extent—in the Southern Hemisphere polar stratosphere. The increased temperature variability in the lower tropical stratosphere is associated with dynamically driven ozone–temperature feedbacks that are only included in the coupled chemistry simulation. The results highlight the fundamental role of two-way feedbacks between the atmospheric circulation and chemistry in driving climate variability in the lower stratosphere. 

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2. Sudden Stratospheric Warmings

   https://doi.org/10.1029/2020RG000708  

   Baldwin, Mark P.; Ayarzagüena, Blanca; Birner, Thomas; Butchart, Neal; Butler, Amy H.; Charlton‐Perez, Andrew J.; Domeisen, Daniela I. V.; Garfinkel, Chaim I.; Garny, Hella; Gerber, Edwin P.; et al (January 2021, Reviews of Geophysics)

   Abstract Sudden stratospheric warmings (SSWs) are impressive fluid dynamical events in which large and rapid temperature increases in the winter polar stratosphere (∼10–50 km) are associated with a complete reversal of the climatological wintertime westerly winds. SSWs are caused by the breaking of planetary‐scale waves that propagate upwards from the troposphere. During an SSW, the polar vortex breaks down, accompanied by rapid descent and warming of air in polar latitudes, mirrored by ascent and cooling above the warming. The rapid warming and descent of the polar air column affect tropospheric weather, shifting jet streams, storm tracks, and the Northern Annular Mode, making cold air outbreaks over North America and Eurasia more likely. SSWs affect the atmosphere above the stratosphere, producing widespread effects on atmospheric chemistry, temperatures, winds, neutral (nonionized) particles and electron densities, and electric fields. These effects span both hemispheres. Given their crucial role in the whole atmosphere, SSWs are also seen as a key process to analyze in climate change studies and subseasonal to seasonal prediction. This work reviews the current knowledge on the most important aspects of SSWs, from the historical background to dynamical processes, modeling, chemistry, and impact on other atmospheric layers. 

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3. Global seasonal distribution of CH ₂ Br ₂ and CHBr ₃ in the upper troposphere and lower stratosphere

   https://doi.org/10.5194/acp-22-15049-2022  

   Jesswein, Markus; Fernandez, Rafael P.; Berná, Lucas; Saiz-Lopez, Alfonso; Grooß, Jens-Uwe; Hossaini, Ryan; Apel, Eric C.; Hornbrook, Rebecca S.; Atlas, Elliot L.; Blake, Donald R.; et al (January 2022, Atmospheric Chemistry and Physics)

   Abstract. Bromine released from the decomposition of short-lived brominated source gases contributes as a sink of ozone in the lower stratosphere.The two major contributors are CH2Br2 and CHBr3.In this study, we investigate the global seasonal distribution of these two substances, based on four High Altitude and Long Range Research Aircraft (HALO) missions, the HIAPER Pole-to-Pole Observations (HIPPO) mission, and the Atmospheric Tomography (ATom) mission.Observations of CH2Br2 in the free and upper troposphere indicate a pronounced seasonality in both hemispheres, with slightly larger mixing ratios in the Northern Hemisphere (NH).Compared to CH2Br2, CHBr3 in these regions shows larger variability and less clear seasonality, presenting larger mixing ratios in winter and autumn in NH midlatitudes to high latitudes.The lowermost stratosphere of SH and NH shows a very similar distribution of CH2Br2 in hemispheric spring with differences well below 0.1 ppt, while the differences in hemispheric autumn are much larger with substantially smaller values in the SH than in the NH.This suggests that transport processes may be different in both hemispheric autumn seasons, which implies that the influx of tropospheric air (“flushing”) into the NH lowermost stratosphere is more efficient than in the SH.The observations of CHBr3 support the suggestion, with a steeper vertical gradient in the upper troposphere and lower stratosphere in SH autumn than in NH autumn.However, the SH database is insufficient to quantify this difference.We further compare the observations to model estimates of TOMCAT (Toulouse Off-line Model of Chemistry And Transport) and CAM-Chem (Community Atmosphere Model with Chemistry, version 4), both using the same emission inventory of Ordóñez et al. (2012).The pronounced tropospheric seasonality of CH2Br2 in the SH is not reproduced by the models,presumably due to erroneous seasonal emissions or atmospheric photochemical decomposition efficiencies.In contrast, model simulations of CHBr3 show a pronounced seasonality in both hemispheres, which is not confirmed by observations.The distributions of both species in the lowermost stratosphere of the Northern and Southern hemispheres are overall well captured by the models with the exception of southern hemispheric autumn,where both models present a bias that maximizes in the lowest 40 K above the tropopause, with considerably lower mixing ratios in the observations.Thus, both models reproduce equivalent flushing in both hemispheres, which is not confirmed by the limited available observations.Our study emphasizes the need for more extensive observations in the SH to fully understand the impact of CH2Br2 and CHBr3 on lowermost-stratospheric ozone loss and to help constrain emissions. 

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4. A New MEPED‐Based Precipitating Electron Data Set

   https://doi.org/10.1029/2021JA029667  

   Pettit, Joshua_M; Randall, Cora_E; Peck, Ethan_D; Harvey, V_Lynn (December 2021, Journal of Geophysical Research: Space Physics)

   Abstract The work presented here introduces a new data set for inclusion of energetic electron precipitation (EEP) in climate model simulations. Measurements made by the medium energy proton and electron detector (MEPED) instruments onboard both the Polar Orbiting Environmental Satellites and the European Space Agency Meteorological Operational satellites are used to create global maps of precipitating electron fluxes. Unlike most previous data sets, the electron fluxes are computed using both the 0° and 90° MEPED detectors. Conversion of observed, broadband electron count rates to differential spectral fluxes uses a linear combination of analytical functions instead of a single function. Two dimensional maps of electron spectral flux are created using Delaunay triangulation to account for the relatively sparse nature of the MEPED sampling. This improves on previous studies that use a 1D interpolation over magnetic local time or L‐shell zonal averaging of the MEPED data. A Whole Atmosphere Community Climate Model (WACCM) simulation of the southern hemisphere 2003 winter using the new precipitating electron data set is shown to agree more closely with observations of odd nitrogen than WACCM simulations using other MEPED‐based electron data sets. Simulated EEP‐induced odd nitrogen increases led to ozone losses of more than 15% in the polar stratosphere near 10 hPa in September of 2003. 

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5. Atmospheric Chemistry Signatures of an Equatorially Symmetric Matsuno–Gill Circulation Pattern

   https://doi.org/10.1175/JAS-D-20-0025.1  

   Wilka, Catherine; Solomon, Susan; Cronin, Timothy W.; Kinnison, Doug; Garcia, Rolando (January 2021, Journal of the Atmospheric Sciences)

   null (Ed.)

   Abstract Matsuno–Gill circulations have been widely studied in tropical meteorology, but their impact on stratospheric chemistry has seldom been explicitly evaluated. This study demonstrates that, in a model nudged to reanalysis, anticyclonic Rossby wave gyres that form near the tropopause as a result of equatorially symmetric heating in the troposphere provide a dynamical mechanism to influence tropical and subtropical atmospheric chemistry during near-equinox months. The anticyclonic flow entrains extratropical air from higher latitudes into the deep tropics of both hemispheres and induces cooling in the already cold upper-troposphere/lower-stratosphere (UTLS) region. Both of these aspects of the circulation allow heterogeneous chlorine activation on sulfuric acid aerosols to proceed rapidly, primarily via the HCl + ClONO 2 reaction. Precipitation rates and heating rates from reanalysis are shown to be consistent with these heating and circulation response patterns in the months of interest. This study analyzes specified dynamics simulations from the Whole Atmosphere Community Climate Model (SD-WACCM) with and without tropical heterogeneous chemistry to demonstrate that these circulations influence substantially the distributions of, for example, NO 2 and ClO in the UTLS tropics and subtropics of both hemispheres. This provides a previously unrecognized dynamical influence on the spatial structures of atmospheric composition changes in the UTLS during near-equinox months. 

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