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Title: Surface-assisted self-assembly of 2D, DNA binary crystals
Surface-assisted, tile-based DNA self-assembly is a powerful method to construct large, two-dimensional (2D) nanoarrays. To further increase the structural complexity, one idea is to incorporate different types of tiles into one assembly system. However, different tiles have different adsorption strengths to the solid surface. The differential adsorptions make it difficult to control the effective molar ratio between different DNA tile concentrations on the solid surface, leading to assembly failure. Herein, we propose a solution to this problem by engineering the tiles with comparable molecular weights while maintaining their architectures. As a demonstration, we have applied this strategy to successfully assemble binary DNA 2D arrays out of very different tiles. We expect that this strategy would facilitate assembly of other complicated nanostructures as well.  more » « less
Award ID(s):
2025187 2107393
PAR ID:
10441731
Author(s) / Creator(s):
; ; ; ; ;
Publisher / Repository:
Royal Society of Chemistry
Date Published:
Journal Name:
Nanoscale
Volume:
15
Issue:
23
ISSN:
2040-3364
Page Range / eLocation ID:
9941 to 9945
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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