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Although electro-optic (EO) nonlinearities are essential for many quantum and classical photonics applications, a major challenge is inefficient modulation in cryogenic environments. Guided by the connection between phase transitions and nonlinearity, we identify the quantum paraelectric perovskite SrTiO3as a strong cryogenic EO [>500 picometers per volt (pm/V)] and piezo-electric material (>90 picocoulombs per newton) atT= 5 K, at frequencies to at least 1 megahertz. Furthermore, by tuning SrTiO3toward quantum criticality, we more than double the EO and piezo-electric effects, demonstrating a linear Pockels coefficient above 1000 pm/V. Our results probe the link between quantum phase transitions, dielectric susceptibility, and nonlinearity, unlocking opportunities in cryogenic optical and mechanical systems and providing a framework for discovering new nonlinear materials.
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Investigation of the electro-optic effect in high-Q 4H-SiC microresonators
Silicon carbide (SiC) recently emerged as a promising photonic and quantum material owing to its unique material properties. In this work, we carried out an exploratory investigation of the Pockels effect in high-quality-factor (high- Q ) 4H-SiC microresonators and demonstrated gigahertz-level electro-optic modulation for the first time. The extracted Pockels coefficients show certain variations among 4H-SiC wafers from different manufacturers, with the magnitudes of r 13 and r 33 estimated to be in the range of (0.3–0.7) pm/V and (0–0.03) pm/V, respectively.
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- Award ID(s):
- 2127499
- PAR ID:
- 10457178
- Date Published:
- Journal Name:
- Optics Letters
- Volume:
- 48
- Issue:
- 6
- ISSN:
- 0146-9592
- Page Range / eLocation ID:
- 1482
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
-
Accepted Manuscript
- Journal Article:
- https://doi.org/10.1364/OL.482844
