skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.

Explore Research Products in the PAR
It may take a few hours for recently added research products to appear in PAR search results.


Title: Enabling Robust Self‐Folding Origami by Pre‐Biasing Vertex Buckling Direction
Abstract Self‐folding is a powerful approach to fabricate materials with complex 3D forms and advanced properties using planar patterning steps, but suffers from intrinsic limitations in robustness due to the highly bifurcated nature of configuration space around the flat state. Here, a simple mechanism is introduced to achieve robust self‐folding of microscale origami by separating actuation into two discrete steps using different thermally responsive hydrogels. First, the vertices are pre‐biased to move in the desired direction from the flat state by selectively swelling one of the two hydrogels at high temperature. Subsequently, the creases are folded toward their target angles by activating swelling of the second hydrogel upon cooling to room temperature. Since each vertex can be individually programmed to move upward or downward, it is possible to robustly select the desired branch even in multi‐vertex structures with reasonably high complexity. This strategy provides key new principles for designing shaping‐morphing materials that avoid undesired distractor states, expanding their potential applications in areas such as soft robotics, sensors, mechanical metamaterials, and deployable devices.  more » « less
Award ID(s):
1822638 1507377
PAR ID:
10460110
Author(s) / Creator(s):
 ;  ;  ;  
Publisher / Repository:
Wiley Blackwell (John Wiley & Sons)
Date Published:
Journal Name:
Advanced Materials
Volume:
31
Issue:
39
ISSN:
0935-9648
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. ; ; ; ; ; (, Journal of computational geometry)
    null (Ed.)
    In this paper, we show that the rigid-foldability of a given crease pattern using all creases is weakly NP-hard by a reduction from the partition problem, and that rigid-foldability with optional creases is NP-hard by a reduction from the 1-in-3 SAT problem. Unlike flat-foldabilty of origami or flexibility of other kinematic linkages, whose complexity originates in the complexity of the layer ordering and possible self-intersection of the material, rigid foldabilltiy from a planar state is hard even though there is no potential self-intersection. In fact, the complexity comes from the combinatorial behavior of the different possible rigid folding configurations at each vertex. The results underpin the fact that it is harder to fold from an unfolded sheet of paper than to unfold a folded state back to a plane, frequently encountered problem when realizing folding-based systems such as self-folding matters and reconfigurable robots. 
    more » « less
  2. ; ; ; ; (, Proceedings of the 2019 International Design Engineering Conference)
    Abstract Stopping origami in arbitrary fold states can present a challenge for origami-based design. In this paper two categories of kirigami-based models are presented for stopping the fold motion of individual creases using deployable hard stops. These models are transcrease (across a crease) and deploy from a flat sheet. The first category is planar and has behavior similar to a four-bar linkage. The second category is spherical and behaves like a degree-4 origami vertex. These models are based on the zero-thickness assumption of paper and can be applied to origami patterns made from thin materials, limiting the motion of the base origami pattern through self-interference within the original facets. Model parameters are based on a desired fold or dihedral angle, as well as facet dimensions. Examples show model benefits and limitations. 
    more » « less
  3. ; ; ; ; (, Nanoscale)
    Stimuli-responsive hydrogels with self-strengthening properties are promising for the use of autonomous growth and adaptation systems to the surrounding environments by mimicking biological materials. However, conventional stimuli-responsive hydrogels require structural destruction to initiate mechanochemical reactions to grow new polymeric networks and strengthen themselves. Here we report continuous self-strengthening of a nanocomposite hydrogel composed of poly( N -isopropylacrylamide) (PNIPAM) and nanoclay (NC) by using external stimuli such as heat and ionic strength. The internal structures of the NC-PNIPAM hydrogel are rearranged through the swelling–deswelling cycles or immersing in a salt solution, thus its mechanical properties are significantly improved. The effects of concentration of NC in hydrogels, number of swelling–deswelling cycles, and presence of salt in the surrounding environment on the mechanical properties of hydrogels are characterized by nanoindentation and tensile tests. The self-strengthening mechanical performance of the hydrogels is demonstrated by the loading ability. This work may offer promise for applications such as artificial muscles and soft robotics. 
    more » « less
  4. ; ; ; (, Advanced Materials Technologies)
    Abstract Hydrogels, which are hydrophilic soft porous networks, are an important class of materials of broad relevance to bioanalytical chemistry, soft‐robotics, drug delivery, and regenerative medicine. Transformer hydrogels are micro‐ and mesostructured hydrogels that display a dramatic transformation of shape, form, or dimension with associated changes in function, due to engineered local variations such as in swelling or stiffness, in response to external controls or environmental stimuli. This review describes principles that can be utilized to fabricate transformer hydrogels such as by layering, patterning, or generating anisotropy, and gradients. Transformer hydrogels are classified based on their responsivity to different stimuli such as temperature, electromagnetic fields, chemicals, and biomolecules. A survey of the current research progress suggests applications of transformer hydrogels in biomimetics, soft robotics, microfluidics, tissue engineering, drug delivery, surgery, and biomedical engineering. 
    more » « less
  5. ; ; (, Advanced Materials)
    Abstract New fluorochromic materials that reversibly change their emission properties in response to their environment are of interest for the development of sensors and light‐emitting materials. A new design of Eu‐containing polymer hydrogels showing fast self‐healing and tunable fluorochromic properties in response to five different stimuli, including pH, temperature, metal ions, sonication, and force, is reported. The polymer hydrogels are fabricated using Eu–iminodiacetate (IDA) coordination in a hydrophilic poly(N,N‐dimethylacrylamide) matrix. Dynamic metal–ligand coordination allows reversible formation and disruption of hydrogel networks under various stimuli which makes hydrogels self‐healable and injectable. Such hydrogels show interesting switchable ON/OFF luminescence along with the sol–gel transition through the reversible formation and dissociation of Eu–IDA complexes upon various stimuli. It is demonstrated that Eu‐containing hydrogels display fast and reversible mechanochromic response as well in hydrogels having interpenetrating polymer network. Those multistimuli responsive fluorochromic hydrogels illustrate a new pathway to make smart optical materials, particularly for biological sensors where multistimuli response is required. 
    more » « less
  • Citation Formats
  • MLA
  • APA
  • Chicago
  • BibTeX
  • Save / Share this Record
  • Send to Email