- Award ID(s):
- 1904497
- NSF-PAR ID:
- 10469537
- Publisher / Repository:
- Nature
- Date Published:
- Journal Name:
- Nature Physics
- Volume:
- 19
- Issue:
- 5
- ISSN:
- 1745-2473
- Page Range / eLocation ID:
- 689 to 693
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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null (Ed.)The interplay between topology and correlations can generate a variety of unusual quantum phases, many of which remain to be explored. Recent advances have identified monolayer WTe2 as a promising material for exploring such interplay in a highly tunable fashion. The ground state of this two-dimensional (2D) crystal can be electrostatically tuned from a quantum spin Hall insulator (QSHI) to a superconductor. However, much remains unknown about the nature of these ground states, including the gap-opening mechanism of the insulating state. Here we report systematic studies of the insulating phase in WTe2 monolayer and uncover evidence supporting that the QSHI is also an excitonic insulator (EI). An EI, arising from the spontaneous formation of electron-hole bound states (excitons), is a largely unexplored quantum phase to date, especially when it is topological. Our experiments on high-quality transport devices reveal the presence of an intrinsic insulating state at the charge neutrality point (CNP) in clean samples. The state exhibits both a strong sensitivity to the electric displacement field and a Hall anomaly that are consistent with the excitonic pairing. We further confirm the correlated nature of this charge-neutral insulator by tunneling spectroscopy. Our results support the existence of an EI phase in the clean limit and rule out alternative scenarios of a band insulator or a localized insulator. These observations lay the foundation for understanding a new class of correlated insulators with nontrivial topology and identify monolayer WTe2 as a promising candidate for exploring quantum phases of ground-state excitons.more » « less
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articles obeying non-Abelian braid statistics have been predicted to emerge in the fractional quantum Hall effect. In particular, a model Hamiltonian with short-range three-body interaction (V^3 Pf) between electrons confined to the lowest Landau level provides exact solutions for quasiholes, and thereby allows a proof of principle for the existence of quasiholes obeying non-Abelian braid statistics. We construct, in terms of two-and three-body Haldane pseudopotentials, a model Hamiltonian that can be solved exactly for both quasiholes and quasiparticles, and provide evidence of non-Abelian statistics for the latter as well. The structure of the quasiparticle states of this model is in agreement with that predicted by the bipartite composite-fermion model of quasiparticles. We further demonstrate, for systems for which exact diagonalization is possible, adiabatic continuity for the ground state, the ordinary neutral excitation, and the topological exciton as we deform our model Hamiltonian continuously into the lowest Landau-level VˆPf Hamiltonian.more » « less
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Published by the American Physical Society 2024 -
The convergence of topology and correlations represents a highly coveted realm in the pursuit of novel quantum states of matter [1, 2]. Introducing electron correlations to a quantum spin Hall (QSH) insulator can lead to the emergence of a fractional topological insulator and other exotic time-reversal-symmetric topological order [3– 10], not possible in quantum Hall and Chern insulator systems. However, the QSH insulator with quantized edge conductance remains rare, let alone that with significant correlations. In this work, we report a novel dual QSH insulator within the intrinsic monolayer crystal of TaIrTe4, arising from the interplay of its single-particle topology and density-tuned electron correlations. At charge neutrality, monolayer TaIrTe4 demonstrates the QSH insulator that aligns with single-particle band structure calculations, manifesting enhanced nonlocal transport and quantized helical edge conductance. Interestingly, upon introducing electrons from charge neutrality, TaIrTe4 only shows metallic behavior in a small range of charge densities but quickly goes into a new insulating state, entirely unexpected based on TaIrTe4’s single-particle band structure. This insulating state could arise from a strong electronic instability near the van Hove singularities (VHS), likely leading to a charge density wave (CDW). Remarkably, within this correlated insulating gap, we observe a resurgence of the QSH state, marked by the revival of nonlocal transport and quantized helical edge conduction. Our observation of helical edge conduction in a CDW gap could bridge spin physics and charge orders. The discovery of a dual QSH insulator introduces a new method for creating topological flat minibands via CDW superlattices, which offer a promising platform for exploring time-reversal-symmetric fractional phases and electromagnetism [3–5, 11, 12].more » « less