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Abstract All cloud and climate models assume ice crystals grow as if they were formed from pure water, even though cloud and haze droplets are solutions. The freezing process of a solution droplet is different than that of a pure water droplet, as shown in prior work. This difference can potentially affect the particle’s subsequent growth as an ice crystal. We present measurements of ice crystal growth from frozen sodium chloride (NaCl) solution droplets in the button electrode levitation diffusion chamber at temperatures between −61° and −40°C. Measured scattering patterns show that concentrated solution droplets remain unfrozen with classical scattering fringes until the droplets freeze. Upon freezing, the scattering patterns become complex within 0.1 s, which is in contrast with frozen pure water particles that retain liquid-like scattering patterns for about a minute. We show that after freezing, solution particles initially grow as spherical-like crystals and then transition to faster growth indicative of a morphological transformation. The measurements indicate that ice formed from solution droplets grows differently and has higher growth rates than ice formed from pure water droplets. We use these results to develop a power-law-based parameterization that captures the supersaturation and mass dependencies.
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Iridescent Water Droplets Beyond Mie Scattering
Abstract Looking at a cup of hot tea, an observer can see color patterns and granular textures both on the water surface and in the steam. Motivated by this example, we model the appearance of iridescent water droplets. Mie scattering describes the scattering of light waves by individual spherical particles and is the building block for both effects, but we show that other mechanisms must also be considered in order to faithfully reproduce the appearance. Iridescence on the water surface is caused by droplets levitating above the surface, and interference between light scattered by drops and reflected by the water surface, known as Quetelet scattering, is essential to producing the color. We propose a model, new to computer graphics, for rendering this phenomenon, which we validate against photographs. For iridescent steam, we show that variation in droplet size is essential to the characteristic color patterns. We build a droplet growth model and apply it as a post‐processing step to an existing computer graphics fluid simulation to compute collections of particles for rendering. We significantly accelerate the rendering of sparse particles with motion blur by intersecting rays with particle trajectories, blending contributions along viewing rays. Our model reproduces the distinctive color patterns correlated with the steam flow. For both effects, we instantiate individual droplets and render them explicitly, since the granularity of droplets is readily observed in reality, and demonstrate that Mie scattering alone cannot reproduce the visual appearance.
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- Award ID(s):
- 1909467
- PAR ID:
- 10479814
- Publisher / Repository:
- Eurographics Association
- Date Published:
- Journal Name:
- Computer Graphics Forum
- Volume:
- 42
- Issue:
- 4
- ISSN:
- 0167-7055
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.1111/cgf.14893
