The infrared response of a system of two vibrational modes in a cavity is calculated by an effective non-Hermitian Hamiltonian derived by employing the nonequilibrium Green's function (NEGF) formalism. Degeneracies of the Hamiltonian (exceptional points, EPs) widely employed in theoretical analysis of optical cavity spectroscopies are used in an approximate treatment and compared with the full NEGF. Qualitative limitations of the EP treatment are explained by examining the approximations employed in the calculation.
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This content will become publicly available on January 28, 2025
Liouvillian exceptional points of an open driven two-level system
We study the applicability of the Liouvillian exceptional points (LEPs) approach to nanoscale open quantum systems. A generic model of the driven two-level system in a thermal environment is analyzed within the nonequilibrium Green’s function (NEGF) and Bloch quantum master equation formulations. We derive the latter starting from the exact NEGF Dyson equations and highlight the qualitative limitations of the LEP treatment by examining the approximations employed in its derivation. We find that the non-Markov character of evolution in open quantum systems does not allow for the introduction of the concept of exceptional points for a description of their dynamics. Theoretical analysis is illustrated with numerical simulations.
more » « less- Award ID(s):
- 2154323
- NSF-PAR ID:
- 10504850
- Publisher / Repository:
- AIP Publishing
- Date Published:
- Journal Name:
- The Journal of Chemical Physics
- Volume:
- 160
- Issue:
- 4
- ISSN:
- 0021-9606
- Page Range / eLocation ID:
- 044116
- Subject(s) / Keyword(s):
- Liouville space exceptional points non equilibrium Green's functions Bloch quantum master equation
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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