More Like this

1. Magnetic properties of a staggered $S=1$ chain with an alternating single-ion anisotropy direction

   https://doi.org/10.1103/PhysRevB.111.014421  

   Vaidya, S; Curley, S_P M; Manuel, P; Stewart, J Ross; Le, M Duc; Balz, C; Shiroka, T; Blundell, S J; Wheeler, K A; Calderon-Lin, I; et al (January 2025, Physical Review B)

   Materials composed of spin-1 antiferromagnetic (AFM) chains are known to adopt complex ground states that are sensitive to the single-ion-anisotropy (SIA) energy ( $D$), and intrachain ( $J_0$) and interchain ( $J_{1,2}^{\prime }$) exchange energy scales. While theoretical and experimental studies have extended this model to include various other energy scales, the effect of the lack of a common SIA axis is not well explored. Here we investigate the magnetic properties of $\mathrm{Ni}\left(\mathrm{pyrimidine}\right){\left({\mathrm{H}}_2\mathrm{O}\right)}_2{\left({\mathrm{NO}}_3\right)}_2$, a chain compound where the tilting of Ni octahedra leads to a twofold alternation of the easy-axis directions along the chain. Muon-spin relaxation measurements indicate a transition to long-range order at $T_{\text{N}}=2.3\mathrm{K}$and the magnetic structure is initially determined to be antiferromagnetic and collinear using elastic neutron diffraction experiments. Inelastic neutron scattering measurements were used to find $J_0=5.107\left(7\right)\mathrm{K}, D=2.79\left(1\right)\mathrm{K},J_1^{\prime }=0.00\left(5\right)\mathrm{K}, J_2^{\prime }=0.18\left(3\right)\mathrm{K}$, and a rhombic anisotropy energy $E=0.19\left(9\right)\mathrm{K}$. Mean-field modeling reveals that the ground state structure hosts spin canting of $\varphi \approx 6.5^{\circ }$, which is not detectable above the noise floor of the elastic neutron diffraction data. Monte Carlo simulation of the powder-averaged magnetization, $M\left(H\right)$, is then used to confirm these Hamiltonian parameters, while single-crystal $M\left(H\right)$simulations provide insight into features observed in the data. Published by the American Physical Society2025 

   more » « less
2. Asymptotic normalization coefficients for $\alpha +{}^{12}\mathrm{C}$ synthesis and the $S$ factor for ${}^{12}\mathrm{C}(\alpha ,\gamma ){}^{16}\mathrm{O}$ radiative capture

   https://doi.org/10.1103/PhysRevC.110.055803  

   Mukhamedzhanov, A M; deBoer, R J; Irgaziev, B F; Blokhintsev, L D; Kadyrov, A S; Savin, D A (November 2024, Physical Review C)

   : The ${}^{12}\mathrm{C}(\alpha ,\gamma ){}^{16}\mathrm{O}$reaction, determining the survival of carbon in red giants, is of interest for nuclear reaction theory and nuclear astrophysics. A specific feature of the ${}^{16}\mathrm{O}$nuclear structure is the presence of two subthreshold bound states, (6.92 MeV, $2^{+}$) and (7.12 MeV, $1^{-}$), that dominate the behavior of the low-energy $S$factor. The strength of these subthreshold states is determined by their asymptotic normalization coefficients (ANCs), which need to be known with high accuracy. : The objective of this research is to examine how the subthreshold and ground-state ANCs impact the low-energy $S$factor, especially at the key astrophysical energy of $300\mathrm{keV}$. The $S$factors are calculated within the framework of the $R$-matrix method using the code. Our total $S$factor takes into account the $E1$and $E2$transitions to the ground state of ${}^{16}\mathrm{O}$including the interference of the subthreshold and higher resonances, which also interfere with the corresponding direct captures, and cascade radiative captures to the ground state of ${}^{16}\mathrm{O}$through four subthreshold states: $0_2^{+},3^{-},2^{+}$, and $1^{-}$. To evaluate the impact of subthreshold ANCs on the low-energy $S$factor, we employ two sets of the ANCs. The first selection, which offers higher ANC values, is attained through the extrapolation process [Blokhintsev , ]. The set with low ANC values was employed by deBoer []. A detailed comparison of the $S$factors at the most effective astrophysical energy of 300 keV is provided, along with an investigation into how the ground-state ANC affects this $S$factor. : The contribution to the total $E1$and $E2S$factors from the corresponding subthreshold resonances at $300\mathrm{keV}$are $(71–74)\%$and $(102–103)\%$, respectively. The correlation of the uncertainties of the subthreshold ANCs with the $E1$and $E2S\left(300\mathrm{keV}\right)$factors is found. The $E1$transition of the subthreshold resonance $1^{-}$does not depend on the ground-state ANC but interferes constructively with a broad $(9.585\mathrm{MeV};1^{-})$resonance giving (for the present subthreshold ANC) an additional $26\%$contribution to the total $E1S\left(300\mathrm{keV}\right)$factor. Interference of the $E2$transition through the subthreshold resonance $2^{+}$with direct capture is almost negligible for small ground-state ANC of $58{\mathrm{fm}}^{-1/2}$. However, its interference with direct capture for higher ground-state ANC of $337{\mathrm{fm}}^{-1/2}$is significant and destructive, contributing $-27\%$. The low-energy $S_{E2}\left(300\mathrm{keV}\right)$factor experiences a smaller increase when both subthfreshold and the ground-state ANCs rise together due to their anticorrelation, compared to when only the subthreshold ANCs increase. Published by the American Physical Society2024 

   more » « less
3. Strength measurements of the $E_{\mathrm{R}}^{\mathrm{lab}}=647$ and 1842 keV resonances in the ${}^{40}\mathrm{Ca}(p,\gamma ){}^{41}\mathrm{Sc}$ reaction and their relevance in novae nucleosynthesis

   https://doi.org/10.1103/PhysRevC.111.025804  

   Sidhu, R S; deBoer, R J; Görres, J; Wiescher, M; Koros, J; Manukyan, K; Matney, M; McDonaugh, J; Picciotto, V; Sanchez, A T; et al (February 2025, Physical Review C)

   Here we report on the direct measurement of the resonance strengths of the $E_{\mathrm{R}}^{\mathrm{lab}}=647\mathrm{keV}$and 1842 keV resonances in the ${}^{40}\mathrm{Ca}(p,\gamma ){}^{41}\mathrm{Sc}$reaction. At novae temperatures, $0.2<T_9<0.7$, the ${}^{40}\mathrm{Ca}(p,\gamma ){}^{41}\mathrm{Sc}$reaction is governed by the low energy resonance at $E_{\mathrm{R}}^{\mathrm{lab}}=647\mathrm{keV}$, whereas the $E_{\mathrm{R}}^{\mathrm{lab}}=1842\mathrm{keV}$resonance serves as a normalization standard for nuclear reaction experiments within the astrophysically relevant energy range. For the $E_{\mathrm{R}}^{\mathrm{lab}}=647\mathrm{keV}$resonance, we obtain a resonance strength $\omega \gamma =(2.51\pm 0.{09}_{\mathrm{stat}}\pm 0.{22}_{\mathrm{syst}})\mathrm{meV}$, with an uncertainty a factor of 2.5 smaller than the previous direct measurement value. For the $E_{\mathrm{R}}^{\mathrm{lab}}=1842\mathrm{keV}$resonance, we obtain a resonance strength $\omega \gamma =(0.148\pm 0.{006}_{\mathrm{stat}}\pm 0.{013}_{\mathrm{syst}})\mathrm{eV}$, which is consistent with previous studies but deviates by $2\sigma$from the most recent measurement. Our results suggest ${}^{40}\mathrm{Ca}$to be a strong waiting point in the nucleosynthesis path of oxygen-neon (ONe) novae. Published by the American Physical Society2025 

   more » « less
4. Systematic study of flow vector fluctuations in $\sqrt{s_{NN}}=5.02$ TeV Pb-Pb collisions

   https://doi.org/10.1103/PhysRevC.109.065202  

   Acharya, S; Adamová, D; Agarwal, A; Aglieri_Rinella, G; Aglietta, L; Agnello, M; Agrawal, N; Ahammed, Z; Ahmad, S; Ahn, S U; et al (June 2024, Physical Review C)

   Measurements of the $p_{\mathrm{T}}$-dependent flow vector fluctuations in Pb–Pb collisions at $\sqrt{s_{\mathrm{NN}}}=5.02\mathrm{TeV}$using azimuthal correlations with the ALICE experiment at the Large Hadron Collider are presented. A four-particle correlation approach [ALICE Collaboration, ] is used to quantify the effects of flow angle and magnitude fluctuations separately. This paper extends previous studies to additional centrality intervals and provides measurements of the $p_{\mathrm{T}}$-dependent flow vector fluctuations at $\sqrt{s_{\mathrm{NN}}}=5.02\mathrm{TeV}$with two-particle correlations. Significant $p_{\mathrm{T}}$-dependent fluctuations of the ${\vec{V}}_2$flow vector in Pb–Pb collisions are found across different centrality ranges, with the largest fluctuations of up to $\sim 15\%$being present in the 5% most central collisions. In parallel, no evidence of significant $p_{\mathrm{T}}$-dependent fluctuations of ${\vec{V}}_3$or ${\vec{V}}_4$is found. Additionally, evidence of flow angle and magnitude fluctuations is observed with more than $5\sigma$significance in central collisions. These observations in $\text{Pb–Pb}$collisions indicate where the classical picture of hydrodynamic modeling with a common symmetry plane breaks down. This has implications for hard probes at high $p_{\mathrm{T}}$, which might be biased by $p_{\mathrm{T}}$-dependent flow angle fluctuations of at least 23% in central collisions. Given the presented results, existing theoretical models should be reexamined to improve our understanding of initial conditions, quark–gluon plasma properties, and the dynamic evolution of the created system. ©2024 CERN, for the ALICE Collaboration2024CERN 

   more » « less
5. Valence, charge transfer, and orbital-dependent correlation in bilayer nickelates ${\mathrm{Nd}}_3{\mathrm{Ni}}_2{\mathrm{O}}_7$

   https://doi.org/10.1103/PhysRevB.111.165101  

   Takegami, Daisuke; Okauchi, Takaki; Morales, Edgar Abarca; Fujinuma, Koto; Furo, Mizuki; Yoshimura, Masato; Tsuei, Ku-Ding; Pan, Grace A; Segedin, Dan Ferenc; Song, Qi; et al (April 2025, Physical Review B)

   We examine the bulk electronic structure of ${\mathrm{Nd}}_3{\mathrm{Ni}}_2{\mathrm{O}}_7$using Ni $2p$core-level hard x-ray photoemission spectroscopy combined with density functional theory $+$dynamical mean-field theory. Our results reveal a large deviation of the Ni $3d$occupation from the formal ${\mathrm{Ni}}^{2.5+}$valency, highlighting the importance of the charge transfer from oxygen ligands. We find that the dominant $d^8$configuration is accompanied by nearly equal contributions from $d^7$and $d^9$states, exhibiting an unusual valence state among Ni-based oxides. Finally, we discuss the Ni $d_{x^2-y^2}$and $d_{z^2}$orbital-dependent hybridization, correlation and local spin dynamics. Published by the American Physical Society2025 

   more » « less