skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.

Attention:

The DOI auto-population feature in the Public Access Repository (PAR) will be unavailable from 4:00 PM ET on Tuesday, July 8 until 4:00 PM ET on Wednesday, July 9 due to scheduled maintenance. We apologize for the inconvenience caused.


This content will become publicly available on April 1, 2026

Title: Valence, charge transfer, and orbital-dependent correlation in bilayer nickelates Nd3Ni2O7
We examine the bulk electronic structure of Nd 3 Ni 2 O 7 using Ni 2 p core-level hard x-ray photoemission spectroscopy combined with density functional theory + dynamical mean-field theory. Our results reveal a large deviation of the Ni 3 d occupation from the formal Ni 2.5 + valency, highlighting the importance of the charge transfer from oxygen ligands. We find that the dominant d 8 configuration is accompanied by nearly equal contributions from d 7 and d 9 states, exhibiting an unusual valence state among Ni-based oxides. Finally, we discuss the Ni d x 2 y 2 and d z 2 orbital-dependent hybridization, correlation and local spin dynamics. Published by the American Physical Society2025  more » « less
Award ID(s):
2039380
PAR ID:
10597690
Author(s) / Creator(s):
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;
Publisher / Repository:
APS
Date Published:
Journal Name:
Physical Review B
Volume:
111
Issue:
16
ISSN:
2469-9950
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. We used the monochromatic soft-x-ray beamline P04 at the synchrotron-radiation facility PETRA III to resonantly excite the strongest 2 p 3 d transitions in neonlike Ni ions, [ 2 p 6 ] J = 0 [ ( 2 p 5 ) 1 / 2 3 d 3 / 2 ] J = 1 and [ 2 p 6 ] J = 0 [ ( 2 p 5 ) 3 / 2 3 d 5 / 2 ] J = 1 , respectively dubbed 3 C and 3 D , achieving a resolving power of 15 000 and signal-to-background ratio of 30. We obtain their natural linewidths, with an accuracy of better than 10%, as well as the oscillator-strength ratio f ( 3 C ) / f ( 3 D ) = 2.51 ( 11 ) from analysis of the resonant fluorescence spectra. These results agree with those of previous experiments, earlier predictions, and our own advanced calculations. Published by the American Physical Society2024 
    more » « less
  2. Nuclear medium effects on B + meson production are studied using the binary-collision scaled cross section ratio between events of different charged-particle multiplicities from proton-lead collisions. Data, collected by the CMS experiment in 2016 at a nucleon-nucleon center-of-mass energy of s NN = 8.16 TeV , corresponding to an integrated luminosity of 175 nb 1 , were used. The scaling factors in the ratio are determined using a novel approach based on the Z μ μ + cross sections measured in the same events. The scaled ratio for B + is consistent with unity for all event multiplicities, putting stringent constraints on nuclear modification for heavy flavor. © 2025 CERN, for the CMS Collaboration2025CERN 
    more » « less
  3. Ever since the discovery of the charge density wave (CDW) transition in the kagome metal CsV 3 Sb 5 , the nature of its symmetry breaking has been under intense debate. While evidence suggests that the rotational symmetry is already broken at the CDW transition temperature ( T CDW ), an additional electronic nematic instability well below T CDW has been reported based on the diverging elastoresistivity coefficient in the anisotropic channel ( m E 2 g ). Verifying the existence of a nematic transition below T CDW is not only critical for establishing the correct description of the CDW order parameter, but also important for understanding low-temperature superconductivity. Here, we report elastoresistivity measurements of CsV 3 Sb 5 using three different techniques probing both isotropic and anisotropic symmetry channels. Contrary to previous reports, we find the anisotropic elastoresistivity coefficient m E 2 g is temperature independent, except for a step jump at T CDW . The absence of nematic fluctuations is further substantiated by measurements of the elastocaloric effect, which show no enhancement associated with nematic susceptibility. On the other hand, the symmetric elastoresistivity coefficient m A 1 g increases below T CDW , reaching a peak value of 90 at T * = 20 K . Our results strongly indicate that the phase transition at T * is not nematic in nature and the previously reported diverging elastoresistivity is due to the contamination from the A 1 g channel. Published by the American Physical Society2024 
    more » « less
  4. Double- and single-differential cross sections for inclusive charged-current ν μ -nucleus scattering are reported for the kinematic domain 0 to 2 GeV / c in three-momentum transfer and 0 to 2 GeV in available energy, at a mean ν μ energy of 1.86 GeV. The measurements are based on an estimated 995,760 ν μ charged-current (CC) interactions in the scintillator medium of the NOvA Near Detector. The subdomain populated by 2-particle-2-hole (2p2h) reactions is identified by the cross section excess relative to predictions for ν μ -nucleus scattering that are constrained by a data control sample. Models for 2-particle-2-hole processes are rated by χ 2 comparisons of the predicted-versus-measured ν μ CC inclusive cross section over the full phase space and in the restricted subdomain. Shortfalls are observed in neutrino generator predictions obtained using the theory-based València and SuSAv2 2p2h models. Published by the American Physical Society2025 
    more » « less
  5. We measure the complete set of angular coefficients J i for exclusive B ¯ D * ν ¯ decays ( = e , μ ). Our analysis uses the full 711 fb 1 Belle dataset with hadronic tag-side reconstruction. The results allow us to extract the form factors describing the B ¯ D * transition and the Cabibbo-Kobayashi-Maskawa matrix element | V cb | . Using recent lattice QCD calculations for the hadronic form factors, we find | V cb | = ( 40.7 ± 0.7 ) × 10 3 using the Boyd-Grinstein-Lebed parametrization, compatible with determinations from inclusive semileptonic decays. We search for lepton flavor universality violation as a function of the hadronic recoil parameter w and investigate the differences of the electron and muon angular distributions. We find no deviation from standard model expectations. Published by the American Physical Society2024 
    more » « less