We report spectroscopic and time-resolved experimental observations to characterize the state in ions. We access this state from the metastable manifold and observe an unexpectedly long lifetime of that allows visible Rabi oscillations and resolved-sideband spectroscopy. Using a combination of coherent population dynamics, high-fidelity detection and heralded state preparation, and optical pumping methods, we measure the branching ratios to the , and states to be , 0.639(2), and , respectively. The branching ratio to the is compatible with zero within our experimental resolution. We also report measurements of Landé -factor of the state. Further, the branching ratio of the to decay in was measured to be 0.188(3), improving its relative uncertainty by an order of magnitude. Our measurements provide experimental benchmarks for better understanding the atomic structure of ions, which still lacks accurate numerical descriptions, and the use of high-lying excited states for partial detection and qubit manipulation in the architecture.
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Measurement of the hyperfine coupling constants and absolute energies of the 12s 2S1/2, 13s 2S1/2 , and 11d 2DJ levels in atomic cesium
We report measurements of the absolute energies of the hyperfine components of the $$12s \ ^2S_{1/2}$$ and $$13s \ ^2S_{1/2}$$ levels of atomic cesium, $$^{133}$$Cs. Using the frequency difference between these components, we determine the hyperfine coupling constants for these states, and report these values with a relative uncertainty of $$\sim$$0.06\%. We also examine the hyperfine structure of the $$11d \ ^2D_{J}$$ ($J=3/2, 5/2$) states, and resolve the sign ambiguity of the hyperfine coupling constants from previous measurements of these states. We also derive new, high precision values for the state energies of the $$12s \ ^2S_{1/2}$$, $$13s \ ^2S_{1/2}$$ and $$11d \ ^2D_{J}$$ states of cesium.
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- Award ID(s):
- 1912519
- PAR ID:
- 10518327
- Publisher / Repository:
- American Physical Society
- Date Published:
- Journal Name:
- Physical Review A
- Volume:
- 105
- Issue:
- 2
- ISSN:
- 2469-9926
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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