Materials composed of spin-1 antiferromagnetic (AFM) chains are known to adopt complex ground states that are sensitive to the single-ion-anisotropy (SIA) energy ( ), and intrachain ( ) and interchain ( ) exchange energy scales. While theoretical and experimental studies have extended this model to include various other energy scales, the effect of the lack of a common SIA axis is not well explored. Here we investigate the magnetic properties of , a chain compound where the tilting of Ni octahedra leads to a twofold alternation of the easy-axis directions along the chain. Muon-spin relaxation measurements indicate a transition to long-range order at and the magnetic structure is initially determined to be antiferromagnetic and collinear using elastic neutron diffraction experiments. Inelastic neutron scattering measurements were used to find , and a rhombic anisotropy energy . Mean-field modeling reveals that the ground state structure hosts spin canting of , which is not detectable above the noise floor of the elastic neutron diffraction data. Monte Carlo simulation of the powder-averaged magnetization, , is then used to confirm these Hamiltonian parameters, while single-crystal simulations provide insight into features observed in the data. Published by the American Physical Society2025 
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                            High-angular-momentum Rydberg states in a room-temperature vapor cell for dc electric-field sensing
                        
                    
    
            We prepare and analyze Rydberg states with orbital quantum numbers using three-optical-photon electromagnetically induced transparency (EIT) and radio frequency (rf) dressing, and employ the high- states in electric-field sensing. Rubidium-85 atoms in a room-temperature vapor cell are first promoted into the state via Rydberg-EIT with three infrared laser beams. Two rf dressing fields then (near-)resonantly couple the , and Rydberg states. The dependence of the rf-dressed Rydberg-state level structure on rf powers, rf and laser frequencies is characterized using EIT. Furthermore, we discuss the principles of dc-electric-field sensing using high- Rydberg states and experimentally demonstrate the method using test electric fields of V/m induced via photo-illumination of the vapor-cell wall. We measure the highly nonlinear dependence of the dc-electric-field strength on the power of the photo-illumination laser. Numerical calculations, which reproduce our experimental observations well, elucidate the underlying physics. Our paper is relevant to high-precision spectroscopy of high- Rydberg states, Rydberg-atom-based electric-field sensing, and plasma electric-field diagnostics. Published by the American Physical Society2024 
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                            - Award ID(s):
- 2110049
- PAR ID:
- 10533993
- Publisher / Repository:
- APS
- Date Published:
- Journal Name:
- Physical Review Research
- Volume:
- 6
- Issue:
- 2
- ISSN:
- 2643-1564
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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