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Title: High-angular-momentum Rydberg states in a room-temperature vapor cell for dc electric-field sensing
We prepare and analyze Rydberg states with orbital quantum numbers 6 using three-optical-photon electromagnetically induced transparency (EIT) and radio frequency (rf) dressing, and employ the high- states in electric-field sensing. Rubidium-85 atoms in a room-temperature vapor cell are first promoted into the 25 F 5 / 2 state via Rydberg-EIT with three infrared laser beams. Two rf dressing fields then (near-)resonantly couple the 25 F ,   25 H ( = 5 ) , and 25 I ( = 6 ) Rydberg states. The dependence of the rf-dressed Rydberg-state level structure on rf powers, rf and laser frequencies is characterized using EIT. Furthermore, we discuss the principles of dc-electric-field sensing using high- Rydberg states and experimentally demonstrate the method using test electric fields of 50 V/m induced via photo-illumination of the vapor-cell wall. We measure the highly nonlinear dependence of the dc-electric-field strength on the power of the photo-illumination laser. Numerical calculations, which reproduce our experimental observations well, elucidate the underlying physics. Our paper is relevant to high-precision spectroscopy of high- Rydberg states, Rydberg-atom-based electric-field sensing, and plasma electric-field diagnostics. Published by the American Physical Society2024  more » « less
Award ID(s):
2110049
PAR ID:
10533993
Author(s) / Creator(s):
; ; ;
Publisher / Repository:
APS
Date Published:
Journal Name:
Physical Review Research
Volume:
6
Issue:
2
ISSN:
2643-1564
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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