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Title: Chirality dependent photon transport and helical superradiance

Chirality, or handedness, is a geometrical property denoting a lack of mirror symmetry. Chirality is ubiquitous in nature and is associated with the nonreciprocal interactions observed in complex systems ranging from biomolecules to topological materials. Here, we demonstrate that chiral arrangements of dipole-coupled atoms or molecules can facilitate the helicity-dependent superradiant emission of light. We show that the collective modes of these systems experience an emergent spin-orbit coupling that leads to chirality-dependent photon transport and nontrivial topological properties. These phenomena are fully described within the electric dipole approximation, resulting in very strong optical responses. Our results demonstrate an intimate connection between chirality, superradiance, and photon helicity and provide a comprehensive framework for studying electron transport dynamics in chiral molecules using cold atom quantum simulators.

<supplementary-material><permissions><copyright-statement>Published by the American Physical Society</copyright-statement><copyright-year>2024</copyright-year></permissions></supplementary-material></sec> </span> <a href='#' class='show open-abstract' style='margin-left:10px;'>more »</a> <a href='#' class='hide close-abstract' style='margin-left:10px;'>« less</a> <div style="clear:both;margin-bottom:20px;"></div> <dl class="dl-horizontal small semi-colon-delimited-data"> <dt>Award ID(s):</dt> <dd> <span> <a target="_blank" rel="noopener noreferrer" href="https://par.nsf.gov/search/award_ids:2207972"> 2207972</a> </span> </dd> </dl> <dl class="dl-horizontal small"> <dt>PAR ID:</dt> <dd>10538955</dd> </dl> <dl class="dl-horizontal small"> <dt>Author(s) / Creator(s):</dt> <dd> <a target="_blank" rel="noopener noreferrer" href="https://par.nsf.gov/search/author:"Peter, Jonah S""><span class="author" itemprop="author">Peter, Jonah S</span></a><span class="sep">; </span><a target="_blank" rel="noopener noreferrer" href="https://par.nsf.gov/search/author:"Ostermann, Stefan""><span class="author" itemprop="author">Ostermann, Stefan</span></a><span class="sep">; </span><a target="_blank" rel="noopener noreferrer" href="https://par.nsf.gov/search/author:"Yelin, Susanne F""><span class="author" itemprop="author">Yelin, Susanne F</span></a></dd> </dl> <dl class="dl-horizontal small"> <dt>Publisher / Repository:</dt> <dd itemprop="publisher">APS</dd> </dl> <dl class="dl-horizontal small"> <dt>Date Published:</dt> <dd> <time itemprop="datePublished" datetime="2024-05-01">2024-05-01</time> </dd> </dl> <dl class="dl-horizontal small"> <dt>Journal Name:</dt> <dd>Physical Review Research</dd> </dl> <dl class="dl-horizontal small"> <dt>Volume:</dt> <dd>6</dd> </dl> <dl class="dl-horizontal small"> <dt>Issue:</dt> <dd>2</dd> </dl> <dl class="dl-horizontal small"> <dt>ISSN:</dt> <dd>2643-1564</dd> </dl> <dl class="dl-horizontal small"> <dt>Format(s):</dt> <dd>Medium: X</dd> </dl> <dl class="dl-horizontal small semi-colon-delimited-data"> <dt>Sponsoring Org:</dt> <dd itemprop="sourceOrganization"> <span>National Science Foundation</span> </dd> </dl> <div class="clearfix"></div> </div> </div> <div id="citation-addl" class="hidden-print"> <h5 id='mlt-header'>More Like this</h5> <ol class="item-list documents" id="citation-mlt" style="min-height: 80px;"> <li> <div class="article item document" itemscope itemtype="http://schema.org/TechArticle"> <div class="item-info"> <div class="title"> <a href="https://par.nsf.gov/biblio/10558546-circularly-polarized-photon-emission-from-magnetized-chiral-plasmas" itemprop="url"> <span class='span-link' itemprop="name">Circularly polarized photon emission from magnetized chiral plasmas</span> </a> </div> <div> <strong> <a class="misc external-link" href="https://doi.org/10.1103/PhysRevD.110.116005" target="_blank" title="Link to document DOI">https://doi.org/10.1103/PhysRevD.110.116005  <span class="fas fa-external-link-alt"></span></a> </strong> </div> <div class="metadata"> <span class="authors"> <span class="author" itemprop="author">Wang, Xinyang</span> <span class="sep">; </span><span class="author" itemprop="author">Shovkovy, Igor A</span> </span> <span class="year">( <time itemprop="datePublished" datetime="2024-12-05">December 2024</time> , Physical Review D) </span> </div> <div style="cursor: pointer;-webkit-line-clamp: 5;" class="abstract" itemprop="description"> <p>We investigate the emission of circularly polarized photons from a magnetized quark-gluon plasma with nonzero quark-number and chiral charge chemical potentials. 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Retrieved from https://par.nsf.gov/biblio/10538955. <em>Physical Review Research</em> 6.2 Web. doi:10.1103/PhysRevResearch.6.023200. </div> <div class="modal-footer"> <button class="btn btn-sm btn-default" data-dismiss="modal" aria-hidden="true">Close</button> </div> </div> </div> </div></li> <li class="links-format"><a href="#cite-apa" data-toggle="modal">APA</a> <div id="cite-apa" class="modal" tabindex="-1" role="dialog" aria-labelledby="cite-apa_label" aria-hidden="true"> <div class="modal-dialog"> <div class="modal-content"> <div class="modal-header"> <button type="button" class="close" data-dismiss="modal" aria-hidden="true">×</button> <strong id="cite-apa_label">Cite: APA Format</strong> </div> <div class="modal-body">Peter, Jonah S, Ostermann, Stefan, & Yelin, Susanne F. <em>Chirality dependent photon transport and helical superradiance</em>. <em>Physical Review Research</em>, <em>6</em> (2). Retrieved from https://par.nsf.gov/biblio/10538955. <a href="https://doi.org/10.1103/PhysRevResearch.6.023200">https://doi.org/10.1103/PhysRevResearch.6.023200</a> </div> <div class="modal-footer"> <button class="btn btn-sm btn-default" data-dismiss="modal" aria-hidden="true">Close</button> </div> </div> </div> </div></li> <li class="links-format"><a href="#cite-chi" data-toggle="modal">Chicago</a> <div id="cite-chi" class="modal" tabindex="-1" role="dialog" aria-labelledby="cite-chi_label" aria-hidden="true"> <div class="modal-dialog"> <div class="modal-content"> <div class="modal-header"> <button type="button" class="close" data-dismiss="modal" aria-hidden="true">×</button> <strong id="cite-chi_label">Cite: Chicago Format</strong> </div> <div class="modal-body">Peter, Jonah S, Ostermann, Stefan, and Yelin, Susanne F. "Chirality dependent photon transport and helical superradiance". <em>Physical Review Research</em> 6 (2). Country unknown/Code not available: APS. <a href="https://doi.org/10.1103/PhysRevResearch.6.023200">https://doi.org/10.1103/PhysRevResearch.6.023200.</a> <a href="https://par.nsf.gov/biblio/10538955">https://par.nsf.gov/biblio/10538955</a>. </div> <div class="modal-footer"> <button class="btn btn-sm btn-default" data-dismiss="modal" aria-hidden="true">Close</button> </div> </div> </div> </div></li> <li class="links-format"><a href="#cite-bib" data-toggle="modal">BibTeX</a> <div id="cite-bib" class="modal" tabindex="-1" role="dialog" aria-labelledby="cite-bib_label" aria-hidden="true"> <div class="modal-dialog"> <div class="modal-content"> <div class="modal-header"> <button type="button" class="close" data-dismiss="modal" aria-hidden="true">×</button> <strong id="cite-bib_label">Cite: BibTeX Format</strong> </div> <div class="modal-body"> @article{osti_10538955,<br/> place = {Country unknown/Code not available}, title = {Chirality dependent photon transport and helical superradiance}, url = {https://par.nsf.gov/biblio/10538955}, DOI = {10.1103/PhysRevResearch.6.023200}, abstractNote = {Chirality, or handedness, is a geometrical property denoting a lack of mirror symmetry. Chirality is ubiquitous in nature and is associated with the nonreciprocal interactions observed in complex systems ranging from biomolecules to topological materials. Here, we demonstrate that chiral arrangements of dipole-coupled atoms or molecules can facilitate the helicity-dependent superradiant emission of light. We show that the collective modes of these systems experience an emergent spin-orbit coupling that leads to chirality-dependent photon transport and nontrivial topological properties. These phenomena are fully described within the electric dipole approximation, resulting in very strong optical responses. Our results demonstrate an intimate connection between chirality, superradiance, and photon helicity and provide a comprehensive framework for studying electron transport dynamics in chiral molecules using cold atom quantum simulators. Published by the American Physical Society2024}, journal = {Physical Review Research}, volume = {6}, number = {2}, publisher = {APS}, author = {Peter, Jonah S and Ostermann, Stefan and Yelin, Susanne F}, }</div> <div class="modal-footer"> <button class="btn btn-sm btn-default" data-dismiss="modal" aria-hidden="true">Close</button> </div> </div> </div> </div></li> <li class="divider"></li> </ul> <ul class="nav nav-list" style="font-size: 14px; font-family: Arial Regular;"> <li class="nav-header header-format">Export Metadata</li> <li class="links-format"><a href="https://par.nsf.gov/endnote?osti_id=10538955">EndNote</a></li> <li class="links-format"><a href="https://par.nsf.gov/export/format:excel/osti-id:10538955">Excel</a></li> <li class="links-format"><a href="https://par.nsf.gov/export/format:csv/osti-id:10538955">CSV</a></li> <li class="links-format"><a href="https://par.nsf.gov/export/format:xml/osti-id:10538955">XML</a></li> <li class="divider"></li> </ul> <ul class="nav nav-list" style="font-size: 14px; 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