Abstract Single crystals of disordered Mn4–xCrxAl11have been synthesized via the flux method. EDS on several crystals of various sizes and shapes revealed an average molar ratio of 17:9:74 for Mn:Cr:Al, while x-ray diffraction on three different crystals yield compositions Mn2.26Cr1.74Al11(Mn4–xCrxAl11,x= 1.74), Mn0.83Cr3.17Al11, and Mn1.07Cr2.93Al11. This compound crystallizes in space group , isostructural with both Mn4Al11and Cr4Al11. Magnetic measurements on several crystals show that this disordered compound is ferrimagnetic with a low effective moment of and a non-reachable transition temperature. Density functional theory calculations display opening of a bandgap in the spin-up channel near the Fermi level with increasing Cr content, an indication of half-metallicity.
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Magnetic order in nanogranular iron germanium (Fe 0.53 Ge 0.47 ) films
Abstract We study the effect of strain on the magnetic properties and magnetization configurations in nanogranular FexGe films ( ) with and without B20 FeGe nanocrystals surrounded by an amorphous structure. Relaxed films on amorphous silicon nitride membranes reveal a disordered skyrmion phase while films near and on top of a rigid substrate favor ferromagnetism and an anisotropic hybridization of Fedlevels and spin-polarized Gespband states. The weakly coupled topological states emerge at room temperature and become more abundant at cryogenic temperatures without showing indications of pinning at defects or confinement to individual grains. These results demonstrate the possibility to control magnetic exchange and topological magnetism by strain and inform magnetoelasticity-mediated voltage control of topological phases in amorphous quantum materials.
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- PAR ID:
- 10597074
- Publisher / Repository:
- Institute of Physics
- Date Published:
- Journal Name:
- Journal of Physics: Condensed Matter
- Volume:
- 37
- Issue:
- 4
- ISSN:
- 0953-8984
- Page Range / eLocation ID:
- 045802
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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