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1. Stochastic ultralight dark matter fluctuations in pulsar timing arrays

   https://doi.org/10.1103/PhysRevD.109.055017  

   Kim, Hyungjin; Mitridate, Andrea (March 2024, Physical Review D)

   Metric perturbations induced by ultralight dark matter (ULDM) fields have long been identified as a potential target for pulsar timing array (PTA) observations. Previous works have focused on the coherent oscillation of metric perturbations at the characteristic frequency set by the ULDM mass. In this work, we show that ULDM fields source low-frequency stochastic metric fluctuations and that these low-frequency fluctuations can produce distinctive detectable signals in PTA data. Using the NANOGrav 12.5-yr dataset and synthetic datasets mimicking present and future PTA capabilities, we show that the current and future PTA observations provide the strongest probe of ULDM density within the Solar System for masses in the range of ${10}^{-18}\mathrm{eV}-{10}^{-16}\mathrm{eV}$. Published by the American Physical Society2024 

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2. High-field/high-frequency electron spin resonances of Fe-doped $\beta \text{−}{\mathrm{Ga}}_2{\mathrm{O}}_3$ by terahertz generalized ellipsometry: Monoclinic symmetry effects

   https://doi.org/10.1103/PhysRevB.109.214106  

   Richter, Steffen; Knight, Sean; Bulancea-Lindvall, Oscar; Mu, Sai; Kühne, Philipp; Stokey, Megan; Ruder, Alexander; Rindert, Viktor; Ivády, Viktor; Abrikosov, Igor A; et al (June 2024, Physical Review B)

   We demonstrate detection and measurement of electron paramagnetic spin resonances (EPR) of iron defects in $\beta \text{−}{\mathrm{Ga}}_2{\mathrm{O}}_3$utilizing generalized ellipsometry at frequencies between 110 and 170 GHz. The experiments are performed on an Fe-doped single crystal in a free-beam configuration in reflection at ${45}^{\circ }$and magnetic fields between 3 and 7 T. In contrast with low-field, low-frequency EPR measurements, we observe all five transitions of the $s=5/2$high-spin state ${\mathrm{Fe}}^{3+}$simultaneously. We confirm that ferric ${\mathrm{Fe}}^{3+}$is predominantly found at octahedrally coordinated Ga sites. We obtain the full set of fourth-order monoclinic zero-field splitting parameters for both octahedrally and tetrahedrally coordinated sites by employing measurements at multiple sample azimuth rotations. The capability of high-field EPR allows us to demonstrate that simplified second-order orthorhombic spin Hamiltonians are insufficient, and fourth-order terms as well as consideration of the monoclinic symmetry are needed. These findings are supported by computational approaches based on density-functional theory for second-order and on ligand-field theory for fourth-order parameters of the spin Hamiltonian. Terahertz ellipsometry is a way to measure spin resonances in a cavity-free setup. Its possibility of varying the probe frequency arbitrarily without otherwise changing the experimental setup offers unique means of truly disentangling different components of highly anisotropic spin Hamiltonians. Published by the American Physical Society2024 

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3. Single-Shot Readout and Weak Measurement of a Tin-Vacancy Qubit in Diamond

   https://doi.org/10.1103/PhysRevX.14.041008  

   Rosenthal, Eric I; Biswas, Souvik; Scuri, Giovanni; Lee, Hope; Stein, Abigail J; Kleidermacher, Hannah C; Grzesik, Jakob; Rugar, Alison E; Aghaeimeibodi, Shahriar; Riedel, Daniel; et al (October 2024, Physical Review X)

   The negatively charged tin-vacancy center in diamond ( ${\mathrm{SnV}}^{-}$) is an emerging platform for building the next generation of long-distance quantum networks. This is due to the ${\mathrm{SnV}}^{-}$’s favorable optical and spin properties including bright emission, insensitivity to electronic noise, and long spin coherence times at temperatures above 1 K. Here, we demonstrate measurement of a single ${\mathrm{SnV}}^{-}$electronic spin with a single-shot readout fidelity of 87.4%, which can be further improved to 98.5% by conditioning on multiple readouts. In the process, we develop understanding of the relationship between strain, magnetic field, spin readout, and microwave spin control. We show that high-fidelity readout is compatible with rapid microwave spin control, demonstrating a favorable parameter regime for use of the ${\mathrm{SnV}}^{-}$center as a high-quality spin-photon interface. Finally, we use weak quantum measurement to study measurement-induced dephasing; this illuminates the fundamental interplay between measurement and decoherence in quantum mechanics, and provides a universal method to characterize the efficiency of color-center spin readout. Taken together, these results overcome an important hurdle in the development of the ${\mathrm{SnV}}^{-}$-based quantum technologies and, in the process, develop techniques and understanding broadly applicable to the study of solid-state quantum emitters. Published by the American Physical Society2024 

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4. First Search for Light Dark Matter in the Neutrino Fog with XENONnT

   https://doi.org/10.1103/PhysRevLett.134.111802  

   Aprile, E; Aalbers, J; Abe, K; Ahmed_Maouloud, S; Althueser, L; Andrieu, B; Angelino, E; Antón_Martin, D; Arneodo, F; Baudis, L; et al (March 2025, Physical Review Letters)

   We search for dark matter (DM) with a mass $[3,12]\mathrm{GeV}/c^2$using an exposure of $3.51\mathrm{tonne}\hspace{0.17em}\mathrm{year}$with the XENONnT experiment. We consider spin-independent DM-nucleon interactions mediated by a heavy or light mediator, spin-dependent DM-neutron interactions, momentum-dependent DM scattering, and mirror DM. Using a lowered energy threshold compared to the previous weakly interacting massive particle search, a blind analysis of [0.5, 5.0] keV nuclear recoil events reveals no significant signal excess over the background. XENONnT excludes spin-independent DM-nucleon cross sections $>2.5\times {10}^{-45}{\mathrm{cm}}^2$at 90% confidence level for $6\mathrm{GeV}/c^2$DM. In the considered mass range, the DM sensitivity approaches the “neutrino fog,” the limitation where neutrinos produce a signal that is indistinguishable from that of light DM-xenon nucleus scattering. Published by the American Physical Society2025 

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5. Valence, charge transfer, and orbital-dependent correlation in bilayer nickelates ${\mathrm{Nd}}_3{\mathrm{Ni}}_2{\mathrm{O}}_7$

   https://doi.org/10.1103/PhysRevB.111.165101  

   Takegami, Daisuke; Okauchi, Takaki; Morales, Edgar Abarca; Fujinuma, Koto; Furo, Mizuki; Yoshimura, Masato; Tsuei, Ku-Ding; Pan, Grace A; Segedin, Dan Ferenc; Song, Qi; et al (April 2025, Physical Review B)

   We examine the bulk electronic structure of ${\mathrm{Nd}}_3{\mathrm{Ni}}_2{\mathrm{O}}_7$using Ni $2p$core-level hard x-ray photoemission spectroscopy combined with density functional theory $+$dynamical mean-field theory. Our results reveal a large deviation of the Ni $3d$occupation from the formal ${\mathrm{Ni}}^{2.5+}$valency, highlighting the importance of the charge transfer from oxygen ligands. We find that the dominant $d^8$configuration is accompanied by nearly equal contributions from $d^7$and $d^9$states, exhibiting an unusual valence state among Ni-based oxides. Finally, we discuss the Ni $d_{x^2-y^2}$and $d_{z^2}$orbital-dependent hybridization, correlation and local spin dynamics. Published by the American Physical Society2025 

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