First-order phase transitions produce abrupt changes to the character of both ground and excited electronic states. Here we conduct electronic compressibility measurements to map the spin phase diagram and Landau level (LL) energies of monolayer in a magnetic field. We resolve a sequence of first-order phase transitions between completely spin-polarized LLs and states with LLs of both spins. Unexpectedly, the LL gaps are roughly constant over a wide range of magnetic fields below the transitions, which we show reflects spin-polarized ground states with opposite spin excitations. These transitions also extend into compressible regimes, with a sawtooth boundary between full and partial spin polarization. We link these observations to the important influence of LL filling on the exchange energy beyond a smooth density-dependent contribution. Our results show that realizes a unique hierarchy of energy scales where such effects induce reentrant magnetic phase transitions tuned by density and magnetic field. Published by the American Physical Society2024
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This content will become publicly available on May 1, 2026
Decoupling dipolar interactions in dense spin ensembles
Dense spin ensembles in solids present a natural platform for studying quantum many-body dynamics. Multiple-pulse coherent control can be used to manipulate the magnetic dipolar interaction between the spins to engineer their dynamics. Here, we investigate the performance of a series of well-known pulse sequences that aim to suppress interspin dipolar couplings. We use a combination of numerical simulations and solid-state nuclear magnetic resonance experiments on adamantane to evaluate and compare sequence performance. We study the role of sequence parameters like interpulse delays and resonance offsets. Disagreements between experiments and theory are typically explained by the presence of control errors and experimental nonidealities. The simulations allow us to explore the influence of factors such as finite pulse widths, rotation errors, and phase transient errors. We also investigate the role of local disorder and establish that it is, perhaps unsurprisingly, a distinguishing factor in the decoupling efficiency of spectroscopic sequences (that preserve Hamiltonian terms proportional to ) and time-suspension sequences (which refocus all terms in the internal Hamiltonian). We discuss our findings in the context of previously known analytical results from average Hamiltonian theory. Finally, we explore the ability of time-suspension sequences to protect multispin correlations in the system. Published by the American Physical Society2025
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- Award ID(s):
- 1921199
- PAR ID:
- 10609831
- Publisher / Repository:
- American Physical Society
- Date Published:
- Journal Name:
- Physical Review Research
- Volume:
- 7
- Issue:
- 2
- ISSN:
- 2643-1564
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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