More Like this

1. Application of quantum-limited optical time transfer to space-based optical clock comparisons and coherent networks

   https://doi.org/10.1063/5.0170107  

   Caldwell, Emily_D; Sinclair, Laura_C; Deschenes, Jean-Daniel; Giorgetta, Fabrizio; Newbury, Nathan_R (January 2024, APL Photonics)

   With the demonstration of quantum-limited optical time transfer capable of tolerating the losses associated with long ground-to-space links, two future applications of free-space time transfer have emerged: intercontinental clock comparisons for time dissemination and coherence transfer for future distributed sensing in the mm-wave region. In this paper, we estimated the projected performance of these two applications using quantum-limited optical time transfer and assuming existing low-size, low-weight, and low-power hardware. In both cases, we limit the discussion to the simplest case of a single geosynchronous satellite linked to either one or two ground stations. One important consideration for such future space-based operations is the choice of reference oscillator onboard the satellite. We find that with a modestly performing optical reference oscillator and low-power fiber-based frequency combs, quantum-limited time transfer could support intercontinental clock comparisons through a common-view node in geostationary orbit with a modified Allan deviation at the 10−16 level at 10-s averaging time, limited primarily by residual turbulence piston noise. In the second application of coherence transfer from ground-to-geosynchronous orbit, we find the system should support high short-term coherence with ∼10 millirad phase noise on a 300 GHz carrier at essentially unlimited integration times. 

   more » « less
2. An optical atomic clock using $4D_J$ states of rubidium

   https://doi.org/10.1088/2058-9565/ad77ef  

   Duspayev, A.; Owens, C.; Dash, B.; Raithel, G. (September 2024, Quantum Science and Technology)

   Abstract We analyze an optical atomic clock using two-photon $5S_{1/2}\to 4D_J$transitions in rubidium. Four one- and two-color excitation schemes to probe the $4D_{3/2}$and $4D_{5/2}$fine-structure states are considered in detail. We compare key characteristics of Rb $4D_J$and $5D_{5/2}$two-photon clocks. The $4D_J$clock features a high signal-to-noise ratio due to two-photon decay at favorable wavelengths, low dc electric and magnetic susceptibilities, and minimal black-body shifts. Ac Stark shifts from the clock interrogation lasers are compensated by two-color Rabi-frequency matching. We identify a ‘magic’ wavelength near 1060 nm, which allows for in-trap, Doppler-free clock-transition interrogation with lattice-trapped cold atoms. From our analysis of clock statistics and systematics, we project a quantum-noise-limited relative clock stability at the ${10}^{-13}/\sqrt{\tau \left(s\right)}$-level, with integration timeτin seconds, and a relative accuracy of $\sim {10}^{-13}$. We describe a potential architecture for implementing the proposed clock using a single telecom clock laser at 1550 nm, which is conducive to optical communication and long-distance clock comparisons. Our work could be of interest in efforts to realize small and portable Rb clocks and in high-precision measurements of atomic properties of Rb $4D_J$-states. 

   more » « less
3. Two-photon excited deep-red and near-infrared emissive organic co-crystals

   https://doi.org/10.1038/s41467-020-18431-7  

   Wang, Yu; Wu, Huang; Li, Penghao; Chen, Su; Jones, Leighton O.; Mosquera, Martín A.; Zhang, Long; Cai, Kang; Chen, Hongliang; Chen, Xiao-Yang; et al (September 2020, Nature Communications)

   Abstract Two-photon excited near-infrared fluorescence materials have garnered considerable attention because of their superior optical penetration, higher spatial resolution, and lower optical scattering compared with other optical materials. Herein, a convenient and efficient supramolecular approach is used to synthesize a two-photon excited near-infrared emissive co-crystalline material. A naphthalenediimide-based triangular macrocycle and coronene form selectively two co-crystals. The triangle-shaped co-crystal emits deep-red fluorescence, while the quadrangle-shaped co-crystal displays deep-red and near-infrared emission centered on 668 nm, which represents a 162 nm red-shift compared with its precursors. Benefiting from intermolecular charge transfer interactions, the two co-crystals possess higher calculated two-photon absorption cross-sections than those of their individual constituents. Their two-photon absorption bands reach into the NIR-II region of the electromagnetic spectrum. The quadrangle-shaped co-crystal constitutes a unique material that exhibits two-photon absorption and near-infrared emission simultaneously. This co-crystallization strategy holds considerable promise for the future design and synthesis of more advanced optical materials. 

   more » « less
4. Nonvolatile Rewritable Photomemory Arrays Based on Reversible Phase‐Change Perovskite for Optical Information Storage

   https://doi.org/10.1002/adom.201900558  

   Zou, Chen; Zheng, Jiajiu; Chang, Cheng; Majumdar, Arka; Lin, Lih_Y (May 2019, Advanced Optical Materials)

   Abstract The high transmission speed of optical signals and their application in optical computation have created a growing demand for photon‐programmed memory devices. Rather than using electrical pulses to store data in one of two states, the photomemory (PM) devices exploit the optical stimulation to store the light information. In this work, the application of a nonvolatile rewritable PM array using the photochromic inorganic perovskite CsPbIBr₂grown by a vapor‐deposition process is demonstrated. Reversible phase transitions between orthorhombic (δ) and cubic (α) phases are achieved in CsPbIBr₂films through laser‐induced heat and moisture exposure. The PM pixels in an optically absorbing perovskite phase exhibit ≈50‐fold photoresponsivity as large as those in a transparent‐colored non‐perovskite phase. Storing optical data are achieved by heating pixels through a near‐infrared laser, while moisture exposure is used to erase the stored information. The nonvolatile PM array exhibits great write‐read‐erase cycle endurance and data retention capability without obvious performance degradation after storage in air for one week. This work demonstrates the promising application of vapor‐deposited inorganic perovskite for optical information storage and the unique potential of them for use in optical switches, tunable metasurfaces, and many other applications. 

   more » « less
5. Cavity-enhanced photon indistinguishability at room temperature and telecom wavelengths

   https://doi.org/10.1038/s41467-024-48119-1  

   Husel, Lukas; Trapp, Julian; Scherzer, Johannes; Wu, Xiaojian; Wang, Peng; Fortner, Jacob; Nutz, Manuel; Hümmer, Thomas; Polovnikov, Borislav; Förg, Michael; et al (December 2024, Nature Communications)

   Abstract Indistinguishable single photons in the telecom-bandwidth of optical fibers are indispensable for long-distance quantum communication. Solid-state single photon emitters have achieved excellent performance in key benchmarks, however, the demonstration of indistinguishability at room-temperature remains a major challenge. Here, we report room-temperature photon indistinguishability at telecom wavelengths from individual nanotube defects in a fiber-based microcavity operated in the regime of incoherent good cavity-coupling. The efficiency of the coupled system outperforms spectral or temporal filtering, and the photon indistinguishability is increased by more than two orders of magnitude compared to the free-space limit. Our results highlight a promising strategy to attain optimized non-classical light sources. 

   more » « less