Multiphoton electromagnetically induced transparency (EIT) of atomic vapors involves several intermediate atomic levels. The substructure of these levels and their collisional interactions can drastically alter experimental EIT signals. Here we report on hyperfine structure and collision effects in three-photon Rydberg EIT on the cascade 5S1/2 → 5P1/2 → 5D3/2 → 25F5/2 in a room-temperature 85Rb vapor cell. In our measurements of EIT spectra, we identify two types of EIT signatures that correspond with distinct excitation pathways and atomic velocity classes in the atomic vapor. The 5D3/2 hyperfine structure and Autler-Townes splittings lead to complex patterns in the EIT spectra, which we analyze with the aid of 10-level EIT simulations. Adding 50 mTorr of Ar gas alters the EIT spectra and induces an additional, third EIT mode. Based on our simulation results, we attribute these changes to hyperfine collisions in the Rb 5D3/2 level. Our study may become useful in quantum technologies involving Rydberg EIT and hyperfine collisions in vapor cells, including noninvasive spatiotemporally resolved electric-field sensing of electric fields in low-pressure plasmas.
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Two-photon Rydberg EIT resonances in non-collinear beam configurations
We study the modifications of Rydberg EIT resonances in non-collinear geometry in which the two required optical fields cross at a small non-zero angle. We observe a strong broadening and amplitude reduction even for small angles when compared to exact counter-propagating and co-propagating collinear geometries. We confirm that such EIT peak deterioration results from the additional Doppler broadening due to the transverse velocity distribution of atoms. The numerical simulation closely matches the experimental measurements. While a non-collinear geometry provides improved spatial resolution for Rydberg EIT electrometry, we conclude that the crossing angle must be small to maintain field sensitivity.
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- Award ID(s):
- 2326736
- PAR ID:
- 10624962
- Publisher / Repository:
- OPG
- Date Published:
- Journal Name:
- Journal of the Optical Society of America B
- Volume:
- 42
- Issue:
- 4
- ISSN:
- 0740-3224
- Page Range / eLocation ID:
- 757
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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