Resonant periodic nanostructures provide perfect reflection across small or large spectral bandwidths depending on the choice of materials and design parameters. This effect has been known for decades, observed theoretically and experimentally via one-dimensional and two-dimensional structures commonly known as resonant gratings, metamaterials, and metasurfaces. The physical cause of this extraordinary phenomenon is guided-mode resonance mediated by lateral Bloch modes excited by evanescent diffraction orders in the subwavelength regime. In recent years, hundreds of papers have declared Fabry-Perot or Mie resonance to be the basis of the perfect reflection possessed by periodic metasurfaces. Treating a simple one-dimensional cylindrical-rod lattice, here we show clearly and unambiguously that Mie resonance does not cause perfect reflection. In fact, the spectral placement of the Bloch-mode-mediated zero-order reflectance is primarily controlled by the lattice period by way of its direct effect on the homogenized effective-medium refractive index of the lattice. In general, perfect reflection appears away from Mie resonance. However, when the lateral leaky-mode field profiles approach the isolated-particle Mie field profiles, the resonance locus tends towards the Mie resonance wavelength. The fact that the lattice fields“remember” the isolated particle fields is referred here as“Mie modal memory.” On erasure of the Mie memory by an index-matched sublayer, we show that perfect reflection survives with the resonance locus approaching the homogenized effective-medium waveguide locus. The results presented here will aid in clarifying the physical basis of general resonant photonic lattices.
more »
« less
Mie‐Resonant Metasurfaces with Controlled Silicon Oxidation in Electron‐Beam Deposition
Abstract Electron‐beam deposition stands as a versatile technique utilized for the accurate and controlled thin‐film deposition of a wide range of materials that readily undergo evaporation. However, silicon, a commonly used material, is prone to oxidation during the deposition process because of the presence of water vapors and oxygen in the chamber. To overcome this challenge, a tailored approach is developed that involves controlling the deposition conditions, including the base pressure in the chamber and the deposition rate. Silicon oxidation is successfully overcome, and this results in achieving refractive index values comparable to those obtained with alternative deposition methods for amorphous silicon. The research shows that the deposition conditions can be utilized effectively to tune the refractive index, providing flexibility in achieving the desired optical properties. It is demonstrated that Mie‐resonant metasurfaces exhibit strong collective resonances, driven by the coherent coupling of Mie modes within the periodic nanoantenna lattice, as evidenced by distinct spectral features in the scattering response. These resonances are observed to be highly tunable, with spectral shifts corresponding to controlled variations in the electron‐beam deposition parameters and silicon oxidation. The approach enables silicon deposition for metasurfaces, which presents exciting possibilities for tailoring and designing advanced nanostructures with unique optical characteristics.
more »
« less
- Award ID(s):
- 2418519
- PAR ID:
- 10640995
- Publisher / Repository:
- Wiley Blackwell (John Wiley & Sons)
- Date Published:
- Journal Name:
- Advanced Materials Interfaces
- Volume:
- 12
- Issue:
- 14
- ISSN:
- 2196-7350
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
More Like this
-
-
Resonant periodic nanostructures provide perfect reflection across small or large spectral bandwidths depending on the choice of materials and design parameters. This effect has been known for decades, observed theoretically and experimentally via one-dimensional and two-dimensional structures commonly known as resonant gratings, metamaterials, and metasurfaces. The physical cause of this extraordinary phenomenon is guided-mode resonance mediated by lateral Bloch modes excited by evanescent diffraction orders in the subwavelength regime. In recent years, hundreds of papers have declared Fabry-Perot or Mie resonance to be basis of the perfect reflection possessed by periodic metasurfaces. Treating a simple one-dimensional cylindrical-rod lattice, here we show clearly and unambiguously that Mie resonance does not cause perfect reflection. In fact, the spectral placement of the Bloch-mode-mediated zero-order reflectance is primarily controlled by the lattice period by way of its direct effect on the homogenized effective-medium refractive index of the lattice. In general, perfect reflection appears away from Mie resonance. However, when the lateral leaky-mode field profiles approach the isolated-particle Mie field profiles, the resonance locus tends towards the Mie resonance wavelength. The fact that the lattice fields remember the isolated particle fields is referred here as Mie modal memory. On erasure of the Mie memory by an index-matched sublayer, we show that perfect reflection survives with the resonance locus approaching the homogenized effective-medium waveguide locus. The results presented here will aid in clarifying the physical basis of general resonant photonic lattices.more » « less
-
null (Ed.)Abstract Actively tunable and reconfigurable wavefront shaping by optical metasurfaces poses a significant technical challenge often requiring unconventional materials engineering and nanofabrication. Most wavefront-shaping metasurfaces can be considered “local” in that their operation depends on the responses of individual meta-units. In contrast, “nonlocal” metasurfaces function based on the modes supported by many adjacent meta-units, resulting in sharp spectral features but typically no spatial control of the outgoing wavefront. Recently, nonlocal metasurfaces based on quasi-bound states in the continuum have been shown to produce designer wavefronts only across the narrow bandwidth of the supported Fano resonance. Here, we leverage the enhanced light-matter interactions associated with sharp Fano resonances to explore the active modulation of optical spectra and wavefronts by refractive-index tuning and mechanical stretching. We experimentally demonstrate proof-of-principle thermo-optically tuned nonlocal metasurfaces made of silicon and numerically demonstrate nonlocal metasurfaces that thermo-optically switch between distinct wavefront shapes. This meta-optics platform for thermally reconfigurable wavefront shaping requires neither unusual materials and fabrication nor active control of individual meta-units.more » « less
-
Abstract A sensing platform is presented that uses dielectric Huygens source metasurfaces to measure refractive index changes in a microfluidic channel with experimentally measured sensitivity of 323 nm RIU−1, a figure of merit (FOM) of 5.4, and a response of 8.2 (820%) change in transmittance per refractive index unit (T/RIU). Changes in the refractive index of liquids flown through the channel are measured by single‐wavelength transmittance measurement, requiring only a simple light source and photodetector, significantly reducing device expense in comparison to state‐of‐the‐art refractive index sensing technologies. A technoeconomic analysis predicts a device costing ≈$2400 that is capable of detecting refractive index changes of the order of 2*10−8. The metasurfaces utilized are low profile, scalable, and use materials and fabrication processes compatible with CMOS and other technologies making them suitable for device integration. The Huygens metasurface system, characterized by spectrally overlapping electric and magnetic dipole modes, offers a high degree of customizability. Interplay between the two resonances may be controlled via metasurface geometry, leading to tunability of device sensitivity and measurement range. Ultrahigh sensitivity of 350 nm RIU−1with FOM of 219, corresponding to single‐wavelength sensitivity of 360 RIU−1, is demonstrated computationally through use of antisymmetric resonances of a Huygens metasurface illuminated at small incidence angles.more » « less
-
Abstract All‐optical control and detection of magnetic states for high‐density recording necessitate nanophotonic approaches to amplify local light intensity below the diffraction limit. Sculpting the near‐field phase and polarization can additionally strengthen magneto‐optical effects that rely on circularly polarized pulses, such as all‐optical helicity‐dependent switching, imaging, and spin‐wave excitation. Here, high‐refractive‐index dielectric nanoantennas illuminated with circularly polarized light resonantly enhance local electric field rotation by more than sixfold within [Pt/Co]Nthin films. Sub‐wavelength arrays of amorphous Si nanodisks, or metasurfaces, patterned on perpendicularly magnetized films support Mie‐type resonances that modulate reflection and transmission dissymmetry by >±2% in experiments. Spatial and spectral interference between dipolar modes, proximity effects, and gain are evaluated by varying disk aspect ratio, metasurface–metal separation, and magnetic film thickness, respectively. Simulated enhancements in magnetic circular birefringence and differential absorption are correlated with amplified local field rotation at electric dipolar modes. Greater achievable amplifications are shown via simulations with single‐crystalline Si metasurfaces exhibiting lower losses, including a 12‐fold strengthened electric field rotation within ferromagnetic layers. The metasurface design rules established here could enable nanoscale localization of all‐optical magnetic switching with lowered laser fluence thresholds, as well as enhanced magneto‐optical responses for light‐assisted reading in spintronic devices.more » « less
An official website of the United States government
