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Title: Precision measurement of lifetime and branching ratios of the 4f135d6s1[5/2]5/2 state in Yb+ ions
We report spectroscopic and time-resolved experimental observations to characterize the [ Xe ] 4 f 13 ( F 5 / 2 o 2 ) 5 d 6 s ( D 1 ) 1 [ 5 / 2 ] 5 / 2 o state in Yb + 172  ions. We access this state from the metastable 4 f 14 5 d ( D 3 / 2 , 5 / 2 2 ) manifold and observe an unexpectedly long lifetime of τ = 37.9 ( 9 ) µ s  that allows visible Rabi oscillations and resolved-sideband spectroscopy. Using a combination of coherent population dynamics, high-fidelity detection and heralded state preparation, and optical pumping methods, we measure the branching ratios to the D 3 / 2 2 ,   D 5 / 2 2 , and S 1 / 2 2 states to be 0.359 ( 2 ) , 0.639(2), and 0.0023 ( 16 ) , respectively. The branching ratio to the 4 f 13 6 s 2 ( F 2 7 / 2 ) is compatible with zero within our experimental resolution. We also report measurements of Landé g -factor of the 1 [ 5 / 2 ] 5 / 2 o state. Further, the branching ratio of the D 5 / 2 2 to S 1 / 2 2 decay in Yb + 172  was measured to be 0.188(3), improving its relative uncertainty by an order of magnitude. Our measurements provide experimental benchmarks for better understanding the atomic structure of Yb +  ions, which still lacks accurate numerical descriptions, and the use of high-lying excited states for partial detection and qubit manipulation in the architecture.  more » « less
Award ID(s):
2144910
PAR ID:
10653300
Author(s) / Creator(s):
; ; ; ; ;
Publisher / Repository:
APS
Date Published:
Journal Name:
Physical Review Research
Volume:
7
Issue:
4
ISSN:
2643-1564
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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