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Abstract The properties of a two‐level quantum dipole emitter near an ultrathin transdimensional plasmonic film are studied theoretically. The model system studied mimics a solid‐state single‐photon source device. Using realistic experimental parameters, the spontaneous and stimulated emission intensity profiles are computed as functions of the excitation frequency and film thickness, followed by the analysis of the second‐order photon correlations to explore the photon antibunching effect. It is shown that ultrathin transdimensional plasmonic films can greatly improve photon antibunching with thickness reduction, which allows one to control the quantum properties of light and make them more pronounced. Knowledge of these features is advantageous for solid‐state single‐photon source device engineering and overall for the development of the new integrated quantum photonics material platform based on the transdimensional plasmonic films.more » « less
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Engheta, Nader; Noginov, Mikhail A.; Zheludev, Nikolay I. (Ed.)
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Subramania, Ganapathi S.; Foteinopoulou, Stavroula (Ed.)
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We present a semi-analytical expression for the dielectric response function of quasi-2D ultrathin films of periodically aligned single-walled carbon nanotubes. We derive the response function in terms of the individual nanotube conductivity, plasma frequency, and the volume fraction of carbon nanotubes in the film. The real part of the dielectric response function is negative for a sufficiently wide range of the incident photon energy, indicating that the film behaves as a hyperbolic metamaterial. Inhomogeneous broadening increases the effect.more » « less
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We use quantum electrodynamics and the confinement-induced nonlocal dielectric response model based on the Keldysh-Rytova electron interaction potential to study the epsilon-near-zero modes of metallic films in the transdimensional regime. Peculiar effects are revealed such as the plasmon mode degeneracy lifting and the dipole emitter coupling to the split epsilon-near-zero modes, leading to thickness-controlled spontaneous decay with rates increased by up to three orders of magnitude.more » « less
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We show that the optical response of ultrathin metallic films of finite lateral size and thickness can feature peculiar magneto-optical effects resulting from the spatial confinement of the electron motion. In particular, the frequency dependence of the magnetic permeability of the film exhibits a sharp resonance structure shifting to the red as the film aspect ratio increases. The films can also be negatively refractive in the IR frequency range under proper tuning. We show that these magneto-optical properties can be controlled by adjusting the film chemical composition, plasmonic material quality, the aspect ratio, and the surroundings of the film.more » « less
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