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We present results of a search for spin-independent dark matter-nucleus interactions in a $1{\mathrm{cm}}^2$by 1 mm thick (0.233 g) high-resolution silicon athermal phonon detector operated above ground. For interactions in the substrate, this detector achieves an rms baseline energy resolution of $361.5\left(4\right)\mathrm{m}\mathrm{eV}$(statistical error), the best for any athermal phonon detector to date. With an exposure of $0.233\mathrm{g}\times 12$hours, we place the most stringent constraints on dark matter masses between 44 and $87\mathrm{M}\mathrm{eV}/{\mathrm{c}}^2$, with the lowest unexplored cross section of $4\times {10}^{-32}{\mathrm{c}\mathrm{m}}^2$at $87\mathrm{M}\mathrm{eV}/{\mathrm{c}}^2$. We employ a conservative salting technique to reach the lowest dark matter mass ever probed via direct detection experiment. This constraint is enabled by two-channel rejection of low energy backgrounds that are coupled to individual sensors. 

Oxygen isotopes (δ18O) are the most commonly utilized speleothem proxy and have provided many foundational records of paleoclimate. Thus, understanding processes affecting speleothem δ18O is crucial. Yet, prior calcite precipitation (PCP), a process driven by local hydrology, is a widely ignored control of speleothem δ18O. Here we investigate the effects of PCP on a stalagmite δ18O record from central Vietnam, spanning 45 – 4 ka. We employ a geochemical model that utilizes speleothem Mg/Ca and cave monitoring data to correct the δ18O record for PCP effects. The resulting record exhibits improved agreement with regional speleothem δ18O records and climate model simulations, suggesting that the corrected record more accurately reflects precipitation δ18O (δ18Op). Without considering PCP, our interpretations of the δ18O record would have been misleading. To avoid misinterpretations of speleothem δ18O, our results emphasize the necessity of considering PCP as a significant driver of speleothem δ18O. 

Most paleoclimate studies of Mainland Southeast Asia hydroclimate focus on the summer monsoon, with few studies investigating rainfall in other seasons. Here we present a multiproxy stalagmite record (45,000 – 4,000 years) from central Vietnam, a region that receives most of its annual rainfall in autumn (September-November). We find evidence of a prolonged dry period spanning the last glacial maximum that is punctuated by an abrupt shift to wetter conditions during the deglaciation at ~14ka. Paired with climate model simulations, we show that sea level change drives autumn monsoon rainfall variability on glacial-orbital timescales. Consistent with the dry signal in the stalagmite record, climate model simulations reveal that lower glacial sea level exposes land in the Gulf of Tonkin and along the South China Shelf, reducing convection and moisture delivery to central Vietnam. When sea level rises and these landmasses flood at ~14ka, moisture delivery to central Vietnam increases causing an abrupt shift from dry to wet conditions. On millennial timescales, we find signatures of well-known Heinrich Stadials (dry conditions) and Dansgaard-Oeschger Events (wet conditions). Model simulations show that during the dry Heinrich Stadials, changes in sea surface temperature related to meltwater forcing cause the formation of an anomalous anticyclone in the Western Pacific, which advects dry air across central Vietnam decreasing autumn rainfall. Notably, sea level modulates the magnitude of millennial-scale dry and wet phases by muting dry events and enhancing wet events during periods of low sea level, highlighting the importance of this mechanism to autumn monsoon variability. 

Abstract. The evolution of organic aerosol (OA) and aerosol sizedistributions within smoke plumes is uncertain due to the variability inrates of coagulation and OA condensation/evaporation between different smokeplumes and at different locations within a single plume. We use aircraftdata from the FIREX-AQ campaign to evaluate differences in evolving aerosolsize distributions, OA, and oxygen to carbon ratios (O:C) between and withinsmoke plumes during the first several hours of aging as a function of smokeconcentration. The observations show that the median particle diameterincreases faster in smoke of a higher initial OA concentration (>1000 µg m−3), with diameter growth of over 100 nm in 8 h – despite generally having a net decrease in OA enhancementratios – than smoke of a lower initial OA concentration (<100 µg m−3), which had net increases in OA. Observations of OA and O:Csuggest that evaporation and/or secondary OA formation was greater in lessconcentrated smoke prior to the first measurement (5–57 min afteremission). We simulate the size changes due to coagulation and dilution andadjust for OA condensation/evaporation based on the observed changes in OA.We found that coagulation explains the majority of the diameter growth, withOA evaporation/condensation having a relatively minor impact. We found thatmixing between the core and edges of the plume generally occurred ontimescales of hours, slow enough to maintain differences in aging betweencore and edge but too fast to ignore the role of mixing for most of our cases. 

This paper details the first application of a software tagging algorithm to reduce radon-induced backgrounds in liquid noble element time projection chambers, such as XENON1T and XENONnT. The convection velocity field in XENON1T was mapped out using ${}^{222}\mathrm{Rn}$and ${}^{218}\mathrm{Po}$events, and the rms convection speed was measured to be $0.30\pm 0.01\mathrm{cm}/\mathrm{s}$. Given this velocity field, ${}^{214}\mathrm{Pb}$background events can be tagged when they are followed by ${}^{214}\mathrm{Bi}$and ${}^{214}\mathrm{Po}$decays, or preceded by ${}^{218}\mathrm{Po}$decays. This was achieved by evolving a point cloud in the direction of a measured convection velocity field, and searching for ${}^{214}\mathrm{Bi}$and ${}^{214}\mathrm{Po}$decays or ${}^{218}\mathrm{Po}$decays within a volume defined by the point cloud. In XENON1T, this tagging system achieved a ${}^{214}\mathrm{Pb}$background reduction of ${6.2}_{-0.9}^{+0.4}\%$with an exposure loss of $1.8\pm 0.2\%$, despite the timescales of convection being smaller than the relevant decay times. We show that the performance can be improved in XENONnT, and that the performance of such a software-tagging approach can be expected to be further improved in a diffusion-limited scenario. Finally, a similar method might be useful to tag the cosmogenic ${}^{137}\mathrm{Xe}$background, which is relevant to the search for neutrinoless double-beta decay. Published by the American Physical Society2024 

Oceans emit large quantities of dimethyl sulfide (DMS) to the marine atmosphere. The oxidation of DMS leads to the formation and growth of cloud condensation nuclei (CCN) with consequent effects on Earth’s radiation balance and climate. The quantitative assessment of the impact of DMS emissions on CCN concentrations necessitates a detailed description of the oxidation of DMS in the presence of existing aerosol particles and clouds. In the unpolluted marine atmosphere, DMS is efficiently oxidized to hydroperoxymethyl thioformate (HPMTF), a stable intermediate in the chemical trajectory toward sulfur dioxide (SO 2 ) and ultimately sulfate aerosol. Using direct airborne flux measurements, we demonstrate that the irreversible loss of HPMTF to clouds in the marine boundary layer determines the HPMTF lifetime ( τ HPMTF < 2 h) and terminates DMS oxidation to SO 2 . When accounting for HPMTF cloud loss in a global chemical transport model, we show that SO 2 production from DMS is reduced by 35% globally and near-surface (0 to 3 km) SO 2 concentrations over the ocean are lowered by 24%. This large, previously unconsidered loss process for volatile sulfur accelerates the timescale for the conversion of DMS to sulfate while limiting new particle formation in the marine atmosphere and changing the dynamics of aerosol growth. This loss process potentially reduces the spatial scale over which DMS emissions contribute to aerosol production and growth and weakens the link between DMS emission and marine CCN production with subsequent implications for cloud formation, radiative forcing, and climate. 

Abstract The precision in reconstructing events detected in a dual-phase time projection chamber depends on an homogeneous and well understood electric field within the liquid target. In the XENONnT TPC the field homogeneity is achieved through a double-array field cage, consisting of two nested arrays of field shaping rings connected by an easily accessible resistor chain. Rather than being connected to the gate electrode, the topmost field shaping ring is independently biased, adding a degree of freedom to tune the electric field during operation. Two-dimensional finite element simulations were used to optimize the field cage, as well as its operation. Simulation results were compared to$${}^{83\textrm{m}}\hbox {Kr }$$ ${}^{83\text{m}}\text{Kr}$calibration data. This comparison indicates an accumulation of charge on the panels of the TPC which is constant over time, as no evolution of the reconstructed position distribution of events is observed. The simulated electric field was then used to correct the charge signal for the field dependence of the charge yield. This correction resolves the inconsistent measurement of the drift electron lifetime when using different calibrations sources and different field cage tuning voltages.