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Laser frequency combs (LFCs) are an important component of Doppler radial velocity (RV) spectroscopy that pushes fractional precision to the 10−10level, as required to identify and characterize Earth-like exoplanets. However, large intensity variations across the LFC spectrum that arise in the nonlinear broadening limit the range of comb modes that can be used for optimal wavelength calibration with sufficient signal-to-noise ratio. Furthermore, temporal spectral-intensity fluctuations of the LFC, that are coupled to flux-dependent detector defects, alter the instrumental point spread function (PSF) and result in spurious RV shifts. To address these issues and improve calibration precision, spectral flattening is crucial for LFCs to maintain a constant photon flux per comb mode. In this work, we demonstrate a dynamic spectral shaping setup using a spatial light modulator (SLM) over the wavelength range of 800–1300 nm. The custom shaping compensates for amplitude fluctuations in real time and can also correct for wavelength-dependent spectrograph transmission, achieving a spectral profile that delivers the constant readout necessary for maximizing precision. Importantly, we characterize the out-of-loop properties of the spectral flattener to verify a twofold improvement in spectral stability. This technique, combined with our approach of pumping the waveguide spectral broadener out-of-band at 1550 nm, reduces the required dynamic range. While this spectral region is tailored for the LFC employed at the Habitable-zone Planet Finder (HPF) spectrograph, the method is broadly applicable to any LFC used for astronomical spectrograph calibration.more » « less
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The search for Earth-like exoplanets with the Doppler radial velocity (RV) technique is an extremely challenging and multifaceted precision spectroscopy problem. Currently, one of the limiting instrumental factors in reaching the required long-term 10−10level of radial velocity precision is the defect-driven subpixel quantum efficiency (QE) variations in the large-format detector arrays used by precision echelle spectrographs. Tunable frequency comb calibration sources that can fully map the point spread function (PSF) across a spectrograph’s entire bandwidth are necessary for quantifying and correcting these detector artifacts. In this work, we demonstrate a combination of laser frequency and mode spacing control that allows full and deterministic tunability of a 30 GHz electro-optic comb together with its filter cavity. After supercontinuum generation, this gives access to any optical frequency across 700–1300 nm. Our specific implementation is intended for the comb deployed at the Habitable-Zone Planet Finder (HPF) spectrograph and its near-infrared Hawaii-2RG array, but the techniques apply to all laser frequency combs (LFCs) used for precision astronomical spectrograph calibration and other applications that require broadband tuning.more » « less
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Molecular diagnostics are a primary tool of modern chemistry, enabling researchers to map chemical reaction pathways and rates to better design and control chemical systems. Many chemical reactions are complex, involving multiple species and reaction pathways occurring on µs or shorter timescales. Existing diagnostic approaches provide a subset of chemical and thermodynamic information. Here we optimize across many diagnostic objectives by introducing a high-speed and broadband, mid-infrared dual-frequency-comb absorption spectrometer. The optical bandwidth of >1000cm−1covers absorption fingerprints of many species with spectral resolution <0.03cm−1to accurately discern their absolute quantities. Key to this advance are 1 GHz pulse repetition rate mode-locked frequency combs covering the 3–5 µm region that enable a spectral acquisition rate of 290cm−1per 17.5 µs per detector forin situtracking of fast chemical process dynamics. We demonstrate this system to quantify the abundances and temperatures of each species in the complete reactants-to-products breakdown of 1,3,5-trioxane, which exhibits a formaldehyde decomposition pathway that is critical to modern low-temperature combustion systems. By maximizing the number of observed species and improving the accuracy of temperature and concentration measurements, this spectrometer provides a pathway for modern chemistry approaches such as combining chemical models with machine learning to constrain or predict complex reaction mechanisms and rates.more » « less
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Frequency combs with mode spacing of 10–20 GHz are critical for increasingly important applications such as astronomical spectrograph calibration, high-speed dual-comb spectroscopy, and low-noise microwave generation. While electro-optic modulators and microresonators can provide narrowband comb sources at this repetition rate, a significant remaining challenge is a means to produce pulses with sufficient peak power to initiate nonlinear supercontinuum generation spanning hundreds of terahertz (THz) as required for self-referencing. Here, we provide a simple, robust, and universal solution to this problem using off-the-shelf polarization-maintaining amplification and nonlinear fiber components. This fiber-integrated approach for nonlinear temporal compression and supercontinuum generation is demonstrated with a resonant electro-optic frequency comb at 1550 nm. We show how to readily achieve pulses shorter than 60 fs at a repetition rate of 20 GHz. The same technique can be applied to picosecond pulses at 10 GHz to demonstrate temporal compression by 9× and achieve 50 fs pulses with a peak power of 5.5 kW. These compressed pulses enable flat supercontinuum generation spanning more than 600 nm after propagation through multi-segment dispersion-tailored anomalous-dispersion highly nonlinear fibers or tantala waveguides. The same 10 GHz source can readily achieve an octave-spanning spectrum for self-referencing in dispersion-engineered silicon nitride waveguides. This simple all-fiber approach to nonlinear spectral broadening fills a critical gap for transforming any narrowband 10–20 GHz frequency comb into a broadband spectrum for a wide range of applications that benefit from the high pulse rate and require access to the individual comb modes.more » « less
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The unique benefits of Fabry–Pérot resonators as frequency-stable reference cavities and as an efficient interface between atoms and photons make them an indispensable resource for emerging photonic technologies. To bring these performance benefits to next-generation communications, computation, and time-keeping systems, it will be necessary to develop strategies to integrate compact Fabry–Pérot resonators with photonic integrated circuits. In this paper, we demonstrate a novel reflection cancellation circuit that utilizes a numerically optimized multi-port polarization-splitting grating coupler to efficiently interface high-finesse Fabry–Pérot resonators with a silicon photonic circuit. This circuit interface produces a spatial separation of the incident and reflected waves, as required for on-chip Pound–Drever–Hall frequency locking, while also suppressing unwanted back reflections from the Fabry–Pérot resonator. Using inverse design principles, we design and fabricate a polarization-splitting grating coupler that achieves 55% coupling efficiency. This design realizes an insertion loss of 5.8 dB for the circuit interface and more than 9 dB of back reflection suppression, and we demonstrate the versatility of this system by using it to interface several reflective off-chip devices.more » « less
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Precision laser spectroscopy is key to many developments in atomic and molecular physics and the advancement of related technologies such as atomic clocks and sensors. However, in important spectroscopic scenarios, such as astronomy and remote sensing, the light is of thermal origin, and interferometric or diffractive spectrometers typically replace laser spectroscopy. In this work, we employ laser-based heterodyne radiometry to measure incoherent light sources in the near-infrared and introduce techniques for absolute frequency calibration with a laser frequency comb. Measuring the solar continuum, we obtain a signal-to-noise ratio that matches the fundamental quantum-limited prediction given by the thermal photon distribution and our system’s efficiency, bandwidth, and averaging time. With resolving power , we determine the center frequency of an iron line in the solar spectrum to sub-MHz absolute frequency uncertainty in under 10 min, a fractional precision 1/4000 the linewidth. Additionally, we propose concepts that take advantage of refractive beam shaping to decrease the effects of pointing instabilities by , and of frequency comb multiplexing to increase data acquisition rates and spectral bandwidths by comparable factors. Taken together, our work brings the power of telecommunications photonics and the precision of frequency comb metrology to laser heterodyne radiometry, with implications for solar and astronomical spectroscopy, remote sensing, and precise Doppler velocimetry.more » « less
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Abstract We report the discovery of a close-in (Porb= 3.349 days) warm Neptune with clear transit timing variations (TTVs) orbiting the nearby (d= 47.3 pc) active M4 star, TOI-2015. We characterize the planet's properties using Transiting Exoplanet Survey Satellite (TESS) photometry, precise near-infrared radial velocities (RVs) with the Habitable-zone Planet Finder Spectrograph, ground-based photometry, and high-contrast imaging. A joint photometry and RV fit yields a radius , mass , and density for TOI-2015 b, suggesting a likely volatile-rich planet. The young, active host star has a rotation period ofProt= 8.7 ± 0.9 days and associated rotation-based age estimate of 1.1 ± 0.1 Gyr. Though no other transiting planets are seen in the TESS data, the system shows clear TTVs of super-period and amplitude ∼100 minutes. After considering multiple likely period-ratio models, we show an outer planet candidate near a 2:1 resonance can explain the observed TTVs while offering a dynamically stable solution. However, other possible two-planet solutions—including 3:2 and 4:3 resonances—cannot be conclusively excluded without further observations. Assuming a 2:1 resonance in the joint TTV-RV modeling suggests a mass of for TOI-2015 b and for the outer candidate. Additional transit and RV observations will be beneficial to explicitly identify the resonance and further characterize the properties of the system.more » « less
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High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to the ninth order (333 nm) in chirped periodically poled lithium niobate waveguides driven by phase-stable , 100 fs pulses at 3 µm with 100 MHz repetition rate. A mid-infrared to ultraviolet-visible conversion efficiency as high as 10% is observed, among an overall 23% conversion of the fundamental to all harmonics. We verify the coherence of the harmonic frequency combs despite the complex highly nonlinear process. Accommodating the extreme spectral bandwidth, numerical simulations based on a single broadband envelope equation with only quadratic nonlinearity give estimates for the conversion efficiency within approximately 1 order of magnitude over a wide range of experimental parameters. From this comparison between theory and experiment, we identify a dimensionless parameter capturing the competition between three-wave mixing and group-velocity walk-off of the harmonics that governs the cascaded HHG physics. We also gain insights into spectral optimization via tuning the waveguide poling profile and pump pulse parameters. These results can inform cascaded HHG in a range of different platforms.more » « less
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Abstract We perform an in-depth analysis of the recently validated TOI-3884 system, an M4-dwarf star with a transiting super-Neptune. Using high-precision light curves obtained with the 3.5 m Apache Point Observatory and radial velocity observations with the Habitable-zone Planet Finder, we derive a planetary mass of and radius of 6.4 ± 0.2R⊕. We detect a distinct starspot crossing event occurring just after ingress and spanning half the transit for every transit. We determine this spot feature to be wavelength dependent with the amplitude and duration evolving slightly over time. Best-fit starspot models show that TOI-3884b possesses a misaligned (λ= 75° ± 10°) orbit that crosses a giant pole spot. This system presents a rare opportunity for studies into the nature of both a misaligned super-Neptune and spot evolution on an active mid-M dwarf.more » « less