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Abstract X-ray analysis is one of the most robust approaches to extract quantitative information from various materials and is widely used in various fields ever since Raimond Castaing established procedures to analyze electron-induced X-ray signals for materials characterization ‘70 years ago’. The recent development of aberration-correction technology in a (scanning) transmission electron microscopes (S/TEMs) offers refined electron probes below the Å level, making atomic-resolution X-ray analysis possible. In addition, the latest silicon drift detectors allow complex detector arrangements and new configurational designs to maximize the collection efficiency of X-ray signals, which make it feasible to acquire X-ray signals from single atoms. In this review paper, recent progress and advantages related to S/TEM-based X-ray analysis will be discussed: (i) progress in quantification for materials characterization including the recent applications to light element analysis, (ii) progress in analytical spatial resolution for atomic-resolution analysis and (iii) progress in analytical sensitivity toward single-atom detection and analysis in materials. Both atomic-resolution analysis and single-atom analysis are evaluated theoretically through multislice-based calculation for electron propagation in oriented crystalline specimen in combination with X-ray spectrum simulation.more » « less
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We report the first observation of the radiative decay with a statistical significance exceeding 10 standard deviations. The signal is observed in the continuum process, using combined data samples of from Belle and from Belle II, collected at the KEKB and SuperKEKB asymmetric-energy colliders, respectively. The branching fraction ratio is measured to be . This result provides crucial discrimination between theoretical models of the structure.more » « lessFree, publicly-accessible full text available June 1, 2027
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Using a data sample of collected by the Belle II detector at or near the and resonances, the cross sections for at center-of-mass energies ranging from 3.8 GeV or the production threshold to have been measured via initial-state radiation. The cross sections for the processes and are consistent with previously published results. The cross sections for these channels obtained by combining with previous Belle results are also given. The process is investigated for the first time. The yields are small and no significant structure is observed in the cross section versus energy. Searches for vector charmoniumlike states in the systems, and for associated intermediate states in the systems, are also presented.more » « lessFree, publicly-accessible full text available June 1, 2027
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We report a measurement of the branching fraction for the leptonic decay . This work presents the first result using Belle II data, an updated Belle measurement that supersedes the previous result, and their combination, which yields the most precise search to date. The analysis is based on of collision data collected at a center-of-mass energy of 10.58 GeV with the Belle and Belle II detectors at the KEKB and SuperKEKB colliders, respectively. We measure , where the first uncertainty is statistical and the second systematic. The observed significance relative to the background-only hypothesis is 2.4 standard deviations. We set a 90% confidence level upper limit of using a frequentist approach and a 90% credibility level upper limit of using a Bayesian approach. These are the most stringent limits to date. The result is interpreted as an exclusion region in the parameter space of type II and type III two-Higgs-doublet models. We search for stable sterile neutrinos with masses . No signal is observed, and the resulting exclusion on the squared mixing parameter provides improvement over previous limits. We report a measurement of the partial branching fraction of semileptonic decays with , obtaining . We present a model-dependent study of weak annihilation decays using the muon momentum spectrum. We observe a signal of 2.4 standard deviations above the background-only hypothesis in regions where the distribution resembles that of decays.more » « lessFree, publicly-accessible full text available June 1, 2027
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A<sc>bstract</sc> Using data samples collected by the Belle and Belle II experiments at the Υ(4S) resonance with integrated luminosities of 571 fb−1and 365 fb−1, respectively, we measure the pseudoscalarB-meson mass difference to bem(B0) −m(B+) = (0.495 ± 0.024 ± 0.005) MeV/c2. The results are based on a simultaneous fit to the variable$${\overline{M} }_{bc}$$, which is related to theBmomentum, forB0andB+candidates; and to the energy dependence of$$\mathcal{R}=\sigma ({e}^{+}{e}^{-}\to {B}^{0}{\overline{B} }^{0}) / \sigma ({e}^{+}{e}^{-}\to {B}^{+}{B}^{-})$$, which is measured using changes in the average center-of-mass energy over the data taking periods. The phase-space hypothesis$$\mathcal{R}={({p}_{{B}^{0}} /{p}_{{B}^{+}})}^{3}$$, upon which previous measurements rely, is strongly disfavored by our fit; the measured mass-difference value for the phase-space hypothesis also differs significantly from our measurement. We constrain$$\mathcal{R}$$in a broader energy range than covered by the direct measurement and extract the energy dependence of$$\mathcal{R}$$in the range from the$$B\overline{B }$$threshold up to 10.59 GeV. We interpret the results using a phenomenological model and constrain the parameters of the$$B\overline{B }$$potential in the isovector channel.more » « lessFree, publicly-accessible full text available May 1, 2027
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A<sc>bstract</sc> We study the processesχbJωandχbJ(π+π−π0)non−ω(J= 0, 1, 2) at center-of-mass energies$$\sqrt{s}$$from 10.73 to 11.02 GeV using a 142.5 fb−1data sample collected with the Belle detector at the KEKB asymmetric-energye+e−collider; and at$$\sqrt{s}\sim 10.75$$GeV using a 19.8 fb−1sample collected with Belle II at SuperKEKB. We find that the Υ(10753) state decays intoχbJωbut not intoχbJ(π+π−π0)non−ω, while the Υ(10860) state, in contrast, decays intoχbJ(π+π−π0)non−ωbut not intoχbJω. The mass and width of the Υ(10753) state are measured to be (10756.1 ± 3.4(stat.) ± 2.7(syst.)) MeV/c2and (32.2 ± 11.3(stat.) ± 14.9(syst.)) MeV. The products of the partial width toe+e−and branching fractions for Υ(10753)→ χb1ωand Υ(10753)→ χb2ωare (1.57±0.27(stat.)±0.22(syst.)) eV and (1.39±0.41(stat.)±0.33(syst.)) eV.more » « lessFree, publicly-accessible full text available April 1, 2027
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