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Abstract Dual-comb interferometry harnesses the interference of two laser frequency combs to provide unprecedented capability in spectroscopy applications. In the past decade, the state-of-the-art systems have reached a point where the signal-to-noise ratio per unit acquisition time is fundamentally limited by shot noise from vacuum fluctuations. To address the issue, we propose an entanglement-enhanced dual-comb spectroscopy protocol that leverages quantum resources to significantly improve the signal-to-noise ratio performance. To analyze the performance of real systems, we develop a quantum model of dual-comb spectroscopy that takes practical noises into consideration. Based on this model, we propose quantum combs with side-band entanglement around each comb lines to suppress the shot noise in heterodyne detection. Our results show significant quantum advantages in the uW to mW power range, making this technique particularly attractive for biological and chemical sensing applications. Furthermore, the quantum comb can be engineered using nonlinear optics and promises near-term experimentation.more » « less
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Liu, Shuai; Zhang, Yuheng; Hariri, Abdulkarim; Al-Hallak, Abdur-Raheem; Zhang, Zheshen (, ACS Photonics)Free, publicly-accessible full text available February 19, 2026
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Liu, Shuai; Wu, Bo-Han; Huang, Jeffrey; Zhang, Zheshen (, Photonics Research)Bound states in the continuum (BICs) hold significant promise in manipulating electromagnetic fields and reducing losses in optical structures, leading to advancements in fundamental research and practical applications. Despite their observation in various optical systems, the behavior of BIC in whispering-gallery-modes (WGMs) optical microcavities, essential components of photonic integrated chips, has yet to be thoroughly explored. In this study, we propose and experimentally identify a robust mechanism for generating quasi-BIC in a single deformed microcavity. By introducing boundary deformations, we construct stable unidirectional radiation channels as leaking continuum shared by different resonant modes and experimentally verify their external strong mode coupling. This results in drastically suppressed leaking loss of one originally long-lived resonance, manifested as more than a threefold enhancement of its quality (Q) factor, while the other short-lived resonance becomes more lossy, demonstrating the formation of Friedrich–Wintgen quasi-BICs as corroborated by the theoretical model and experimental data. This research will provide a practical approach to enhance theQ-factor of optical microcavities, opening up potential applications in the area of deformed microcavities, nonlinear optics, quantum optics, and integrated photonics.more » « less
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