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1. Neutron Scattering Study of the kagome metal Sc3Mn3Al7Si5

   Li, X. Y. ; Reig-i-Plessis, D. ; Liu, P. F. ; Wu, S. ; Wanf, B. T. ; Hallas, A. M. ; Stone, M. B. ; Aronson, M. C. ( October 2021 , Physical review)

   null (Ed.)

   Sc 3 Mn 3 Al 7 Si 5 is a rare example of a correlated metal in which the Mn moments form a kagome lattice. The absence of magnetic ordering to the lowest temperatures suggests that geometrical frustration of magnetic interactions may lead to strong magnetic fluctuations. We have performed inelastic neutron scattering measurements on Sc 3 Mn 3 Al 7 Si 5 , finding that phonon scattering dominates for energies from ∼20–50 meV. These results are in good agreement with ab initio calculations of the phonon dispersions and densities of states, and as well reproduce the measured specific heat. A weak magnetic signal was detected at energies less than ∼10 meV, present only at the lowest temperatures. The magnetic signal is broad and quasielastic, as expected for metallic paramagnets. 

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2. Energetic Electron Precipitation Driven by Electromagnetic Ion Cyclotron Waves from ELFIN’s Low Altitude Perspective

   https://doi.org/10.1007/s11214-023-00984-w  

   Angelopoulos, V. ; Zhang, X. -J. ; Artemyev, A. V. ; Mourenas, D. ; Tsai, E. ; Wilkins, C. ; Runov, A. ; Liu, J. ; Turner, D. L. ; Li, W. ; et al ( July 2023 , Space Science Reviews)

   We review comprehensive observations of electromagnetic ion cyclotron (EMIC) wave-driven energetic electron precipitation using data collected by the energetic electron detector on the Electron Losses and Fields InvestigatioN (ELFIN) mission, two polar-orbiting low-altitude spinning CubeSats, measuring 50-5000 keV electrons with good pitch-angle and energy resolution. EMIC wave-driven precipitation exhibits a distinct signature in energy-spectrograms of the precipitating-to-trapped flux ratio: peaks at >0.5 MeV which are abrupt (bursty) (lasting ∼17 s, or$\Delta L\sim 0.56$$\Delta L\sim 0.56$) with significant substructure (occasionally down to sub-second timescale). We attribute the bursty nature of the precipitation to the spatial extent and structuredness of the wave field at the equator. Multiple ELFIN passes over the same MLT sector allow us to study the spatial and temporal evolution of the EMIC wave - electron interaction region. Case studies employing conjugate ground-based or equatorial observations of the EMIC waves reveal that the energy of moderate and strong precipitation at ELFIN approximately agrees with theoretical expectations for cyclotron resonant interactions in a cold plasma. Using multiple years of ELFIN data uniformly distributed in local time, we assemble a statistical database of ∼50 events of strong EMIC wave-driven precipitation. Most reside at$L\sim 5-7$$L\sim 5-7$at dusk, while a smaller subset exists at$L\sim 8-12$$L\sim 8-12$at post-midnight. The energies of the peak-precipitation ratio and of the half-peak precipitation ratio (our proxy for the minimum resonance energy) exhibit an$L$$L$-shell dependence in good agreement with theoretical estimates based on prior statistical observations of EMIC wave power spectra. The precipitation ratio’s spectral shape for the most intense events has an exponential falloff away from the peak (i.e., on either side of$\sim 1.45$$\sim 1.45$MeV). It too agrees well with quasi-linear diffusion theory based on prior statistics of wave spectra. It should be noted though that this diffusive treatment likely includes effects from nonlinear resonant interactions (especially at high energies) and nonresonant effects from sharp wave packet edges (at low energies). Sub-MeV electron precipitation observed concurrently with strong EMIC wave-driven >1 MeV precipitation has a spectral shape that is consistent with efficient pitch-angle scattering down to ∼ 200-300 keV by much less intense higher frequency EMIC waves at dusk (where such waves are most frequent). At ∼100 keV, whistler-mode chorus may be implicated in concurrent precipitation. These results confirm the critical role of EMIC waves in driving relativistic electron losses. Nonlinear effects may abound and require further investigation.

    

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3. Phonon mixing in the charge density wave state of ScV6Sn6

   https://doi.org/10.1038/s41535-023-00590-7  

   Gu, Yanhong ; Ritz, Ethan T. ; Meier, William R. ; Blockmon, Avery ; Smith, Kevin ; Madhogaria, Richa Pokharel ; Mozaffari, Shirin ; Mandrus, David ; Birol, Turan ; Musfeldt, Janice L. ( December 2023 , npj Quantum Materials)

   Kagomé metals are widely recognized, versatile platforms for exploring topological properties, unconventional electronic correlations, magnetic frustration, and superconductivity. In theRV₆Sn₆family of materials (R= Sc, Y, Lu), ScV₆Sn₆hosts an unusual charge density wave ground state as well as structural similarities with theAV₃Sb₅system (A= K, Cs, Rb). In this work, we combine Raman scattering spectroscopy with first-principles lattice dynamics calculations to reveal phonon mixing processes in the charge density wave state of ScV₆Sn₆. In the low temperature phase, we find at least four new peaks in the vicinity of the V-containing totally symmetric mode near 240 cm⁻¹suggesting that the density wave acts to mix modes ofP6/mmmand$$R\bar{3}m$$$R\overline{3}m$symmetry - a result that we quantify by projecting phonons of the high symmetry state onto those of the lower symmetry structure. We also test the stability of the short-range ordered density wave state under compression and propose that both physical and chemical pressure quench the effect. We discuss these findings in terms of symmetry and the structure-property trends that can be unraveled in this system.

    

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4. Hot-carrier dynamics in InAs/AlAsSb multiple-quantum wells

   https://doi.org/10.1038/s41598-021-89815-y  

   Piyathilaka, Herath P. ; Sooriyagoda, Rishmali ; Esmaielpour, Hamidreza ; Whiteside, Vincent R. ; Mishima, Tetsuya D. ; Santos, Michael B. ; Sellers, Ian R. ; Bristow, Alan D. ( May 2021 , Scientific Reports)

   A type-II InAs/AlAs$$_{0.16}$$${}_{0.16}$Sb$$_{0.84}$$${}_{0.84}$multiple-quantum well sample is investigated for the photoexcited carrier dynamics as a function of excitation photon energy and lattice temperature. Time-resolved measurements are performed using a near-infrared pump pulse, with photon energies near to and above the band gap, probed with a terahertz probe pulse. The transient terahertz absorption is characterized by a multi-rise, multi-decay function that captures long-lived decay times and a metastable state for an excess-photon energy of$$>100$$$>100$meV. For sufficient excess-photon energy, excitation of the metastable state is followed by a transition to the long-lived states. Excitation dependence of the long-lived states map onto a nearly-direct band gap ($$E{_g}$$$E{}_g$) density of states with an Urbach tail below$$E{_g}$$$E{}_g$. As temperature increases, the long-lived decay times increase$$$<E{}_g$, due to the increased phonon interaction of the unintentional defect states, and by phonon stabilization of the hot carriers$$>E{_g}$$$>E{}_g$. Additionally, Auger (and/or trap-assisted Auger) scattering above the onset of the plateau may also contribute to longer hot-carrier lifetimes. Meanwhile, the initial decay component shows strong dependence on excitation energy and temperature, reflecting the complicated initial transfer of energy between valence-band and defect states, indicating methods to further prolong hot carriers for technological applications.

    

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5. Gapless Dirac magnons in CrCl3

   https://doi.org/10.1038/s41535-022-00473-3  

   Schneeloch, John A. ; Tao, Yu ; Cheng, Yongqiang ; Daemen, Luke ; Xu, Guangyong ; Zhang, Qiang ; Louca, Despina ( December 2022 , npj Quantum Materials)

   Abstract Bosonic Dirac materials are testbeds for dissipationless spin-based electronics. In the quasi two-dimensional honeycomb lattice of CrX 3 (X = Cl, Br, I), Dirac magnons have been predicted at the crossing of acoustical and optical spin waves, analogous to Dirac fermions in graphene. Here we show that, distinct from CrBr 3 and CrI 3 , gapless Dirac magnons are present in bulk CrCl 3 , with inelastic neutron scattering intensity at low temperatures approaching zero at the Dirac K point. Upon warming, magnon-magnon interactions induce strong renormalization and decreased lifetimes, with a ~25% softening of the upper magnon branch intensity from 5 to 50 K, though magnon features persist well above T N . Moreover, on cooling below ~50 K, an anomalous increase in the a -axis lattice constant and a hardening of a ~26 meV phonon feature are observed, indicating magnetoelastic and spin-phonon coupling arising from an increase in the in-plane spin correlations that begins tens of Kelvin above T N . 

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