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1. Neutron Scattering Study of the kagome metal Sc3Mn3Al7Si5

   Li, X. Y.; Reig-i-Plessis, D.; Liu, P. F.; Wu, S.; Wanf, B. T.; Hallas, A. M.; Stone, M. B.; Aronson, M. C. (October 2021, Physical review)

   null (Ed.)

   Sc 3 Mn 3 Al 7 Si 5 is a rare example of a correlated metal in which the Mn moments form a kagome lattice. The absence of magnetic ordering to the lowest temperatures suggests that geometrical frustration of magnetic interactions may lead to strong magnetic fluctuations. We have performed inelastic neutron scattering measurements on Sc 3 Mn 3 Al 7 Si 5 , finding that phonon scattering dominates for energies from ∼20–50 meV. These results are in good agreement with ab initio calculations of the phonon dispersions and densities of states, and as well reproduce the measured specific heat. A weak magnetic signal was detected at energies less than ∼10 meV, present only at the lowest temperatures. The magnetic signal is broad and quasielastic, as expected for metallic paramagnets. 

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2. The anomalous temperature dependent low energy electron diffraction intensity at epitaxial Sr ₃ Ir ₂ O ₇ thin film surfaces

   https://doi.org/10.1088/1361-648X/adbaa8  

   Adegbite, Peace Ikeoluwa; Subedi, Arjun; Zhang, Yuanyuan; Hong, Xia; Komesu, Takashi; Dowben, P A (March 2025, Journal of Physics: Condensed Matter)

   Abstract We report on the temperature dependent low energy electron diffraction (LEED) studies of 12 nm epitaxial Sr₃Ir₂O₇(001) thin films. The Debye temperature has been extracted from the temperature-dependence of LEED intensity at elevated temperatures and different electron kinetic energies. For the most surface sensitive LEED, obtained at the lowest electron kinetic energies, the extracted surface Debye temperature is 270 ± 22 K, which is much lower than the 488 ± 40 K Debye temperature obtained using higher electron kinetic energies. Surprisingly, the LEED diffraction intensity, at the lowest electron kinetic energies, increases rather than decreases, with increasing sample temperatures up to about 440 K. This anomalous behavior has been attributed to the reduction of the lattice vibrational amplitudes along the surface normal. This damping of the normal mode vibrations with increasing temperature results from the enhanced electronic screening via thermally activated carriers. This scenario is corroborated by the transport measurement, showing that Sr₃Ir₂O₇is a narrow band Mott insulator with a band gap of about 32 meV. We have identified criteria for finding anomalous scattering behavior in other transition metal oxide systems. 

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3. Enhanced near-infrared absorption in lattice-matched Sc _0.14 Al _0.86 N/GaN multi-quantum wells: growth optimization and insights into polarization parameters

   https://doi.org/10.1364/OME.545820  

   Abdin, Zain_Ul; Gopakumar, Govardan; Kumar, Rajendra; Manfra, Michael_J; Malis, Oana (January 2025, Optical Materials Express)

   We report on the near-infrared intersubband (ISB) absorption properties of strain-free Sc_0.14Al_0.86N/GaN multiple quantum wells (MQWs) grown on c-plane GaN substrates by molecular beam epitaxy. These MQWs exhibit strong, sharp, and tunable absorption energies between 515 meV and 709 meV, for well widths ranging from 7 nm to 1.5 nm, respectively. Observation of ISB absorption in ultra-thin Sc_0.14Al_0.86N/GaN MQWs not only extends the near-infrared range accessible with Sc-containing nitrides but also highlights the challenges of growing nanometer-thick GaN quantum wells. We explore the effects of growth temperature on absorption characteristics and find that substrate temperatures above 600°C significantly enhance ISB absorption intensity but also introduce an energy redshift for the narrowest wells. The redshift is attributed to increased interface roughness due to ScAlN surface morphology degradation at higher temperatures. Additionally, a comparison of experimental results with simulated band-structures indicates that the magnitude of net polarization rises faster with Sc-composition than previously suggested by theoretical calculations. This study advances the prospects of ScAlN/GaN heterostructures for novel photonic devices in the technologically important near-infrared range. 

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4. The Qz5 Survey. I. How the H i Mass Density of the Universe Evolves with Cosmic Time

   https://doi.org/10.3847/1538-4357/adb430  

   Oyarzún, Grecco A; Rafelski, Marc; Christensen, Lise; Ozyurt, Fiona; Jorgenson, Regina A; Neeleman, M; Fumagalli, Michele; Prochaska, J Xavier; Worseck, G; Wisz, M E; et al (April 2025, The Astrophysical Journal)

   Abstract We report that the neutral hydrogen (Hi) mass density of the Universe (ρ_Hi) increases with cosmic time sincez ∼ 5, peaks atz ∼ 3, and then decreases towardz ∼ 0. This is the first result of Qz5, our spectroscopic survey of 63 quasars atz ≳ 5 with VLT/X-SHOOTER and Keck/ESI aimed at characterizing intervening Higas absorbers atz ∼ 5. The main feature of Qz5 is the high resolution (R ∼ 7000–9000) of the spectra, which allows us to (1) accurately detect high column density Higas absorbers in an increasingly neutral intergalactic medium atz ∼ 5 and (2) determine the reliability of previousρ_Himeasurements derived with lower resolution spectroscopy. We find five intervening damped Lyαabsorbers (DLAs) atz > 4.5, which corresponds to the lowest DLA incidence rate ( $0.034_{0.02}^{0.05}$) atz ≳ 2. We also measure the lowestρ_Hiatz ≳ 2 from our sample of DLAs and subDLAs, corresponding toρ_Hi $=0.56_{0.31}^{0.82}\times 10^8{M}_{\odot }$Mpc⁻³atz ∼ 5. Taking into account our measurements atz ∼ 5 and systematic biases in the DLA detection rate at lower spectral resolutions, we conclude thatρ_Hidoubles fromz ∼ 5 toz ∼ 3. From these results emerges a qualitative agreement between how the cosmic densities of Higas mass, molecular gas mass, and star formation rate build up with cosmic time. 

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5. Gapless Dirac magnons in CrCl3

   https://doi.org/10.1038/s41535-022-00473-3  

   Schneeloch, John A.; Tao, Yu; Cheng, Yongqiang; Daemen, Luke; Xu, Guangyong; Zhang, Qiang; Louca, Despina (December 2022, npj Quantum Materials)

   Abstract Bosonic Dirac materials are testbeds for dissipationless spin-based electronics. In the quasi two-dimensional honeycomb lattice of CrX 3 (X = Cl, Br, I), Dirac magnons have been predicted at the crossing of acoustical and optical spin waves, analogous to Dirac fermions in graphene. Here we show that, distinct from CrBr 3 and CrI 3 , gapless Dirac magnons are present in bulk CrCl 3 , with inelastic neutron scattering intensity at low temperatures approaching zero at the Dirac K point. Upon warming, magnon-magnon interactions induce strong renormalization and decreased lifetimes, with a ~25% softening of the upper magnon branch intensity from 5 to 50 K, though magnon features persist well above T N . Moreover, on cooling below ~50 K, an anomalous increase in the a -axis lattice constant and a hardening of a ~26 meV phonon feature are observed, indicating magnetoelastic and spin-phonon coupling arising from an increase in the in-plane spin correlations that begins tens of Kelvin above T N . 

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