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Abstract Charge modulations have been widely observed in cuprates, suggesting their centrality for understanding the high- T c superconductivity in these materials. However, the dimensionality of these modulations remains controversial, including whether their wavevector is unidirectional or bidirectional, and also whether they extend seamlessly from the surface of the material into the bulk. Material disorder presents severe challenges to understanding the charge modulations through bulk scattering techniques. We use a local technique, scanning tunneling microscopy, to image the static charge modulations on Bi 2− z Pb z Sr 2− y La y CuO 6+ x . The ratio of the phase correlation length ξ CDW to the orientation correlation length ξ orient points to unidirectional charge modulations. By computing new critical exponents at free surfaces including that of the pair connectivity correlation function, we show that these locally 1D charge modulations are actually a bulk effect resulting from classical 3D criticality of the random field Ising model throughout the entire superconducting doping range.
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Connecting Complex Electronic Pattern Formation to Critical Exponents
Scanning probes reveal complex, inhomogeneous patterns on the surface of many condensed matter systems. In some cases, the patterns form self-similar, fractal geometric clusters. In this paper, we advance the theory of criticality as it pertains to those geometric clusters (defined as connected sets of nearest-neighbor aligned spins) in the context of Ising models. We show how data from surface probes can be used to distinguish whether electronic patterns observed at the surface of a material are confined to the surface, or whether the patterns originate in the bulk. Whereas thermodynamic critical exponents are derived from the behavior of Fortuin–Kasteleyn (FK) clusters, critical exponents can be similarly defined for geometric clusters. We find that these geometric critical exponents are not only distinct numerically from the thermodynamic and uncorrelated percolation exponents, but that they separately satisfy scaling relations at the critical fixed points discussed in the text. We furthermore find that the two-dimensional (2D) cross-sections of geometric clusters in the three-dimensional (3D) Ising model display critical scaling behavior at the bulk phase transition temperature. In particular, we show that when considered on a 2D slice of a 3D system, the pair connectivity function familiar from percolation theory displays more robust critical behavior than the spin-spin correlation function, and we calculate the corresponding critical exponent. We discuss the implications of these two distinct length scales in Ising models. We also calculate the pair connectivity exponent in the clean 2D case. These results extend the theory of geometric criticality in the clean Ising universality classes, and facilitate the broad application of geometric cluster analysis techniques to maximize the information that can be extracted from scanning image probe data in condensed matter systems.
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- PAR ID:
- 10325882
- Date Published:
- Journal Name:
- Condensed Matter
- Volume:
- 6
- Issue:
- 4
- ISSN:
- 2410-3896
- Page Range / eLocation ID:
- 39
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.3390/condmat6040039
