Flexible thermoelectric generators (TEGs) have shown immense potential for serving as a power source for wearable electronics and the Internet of Things. A key challenge preventing large-scale application of TEGs lies in the lack of a high-throughput processing method, which can sinter thermoelectric (TE) materials rapidly while maintaining their high thermoelectric properties. Herein, we integrate high-throughput experimentation and Bayesian optimization (BO) to accelerate the discovery of the optimum sintering conditions of silver–selenide TE films using an ultrafast intense pulsed light (flash) sintering technique. Due to the nature of the high-dimensional optimization problem of flash sintering processes, a Gaussian process regression (GPR) machine learning model is established to rapidly recommend the optimum flash sintering variables based on Bayesian expected improvement. For the first time, an ultrahigh-power factor flexible TE film (a power factor of 2205 μW m −1 K −2 with a zT of 1.1 at 300 K) is demonstrated with a sintering time less than 1.0 second, which is several orders of magnitude shorter than that of conventional thermal sintering techniques. The films also show excellent flexibility with 92% retention of the power factor (PF) after 10 3 bending cycles with a 5 mm bending radius. In addition, a wearable thermoelectric generator based on the flash-sintered films generates a very competitive power density of 0.5 mW cm −2 at a temperature difference of 10 K. This work not only shows the tremendous potential of high-performance and flexible silver–selenide TEGs but also demonstrates a machine learning-assisted flash sintering strategy that could be used for ultrafast, high-throughput and scalable processing of functional materials for a broad range of energy and electronic applications.
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Topology Optimization of Permanent Magnets for Generators Using Level Set Methods
Generators are considered as the core application of electromagnetic machines, which require high-cost rare-earth-based permanent magnets. The development of generators is moving toward high efficiency and increased environmental friendliness. Minimizing the use of rare earth materials such as magnetic materials under the premise of machine performance emerges as a challenging task. Topology optimization has been promisingly applied to many application areas as a powerful generative design tool. It can identify the optimal distribution of magnetic material in the defined design space. This paper employs the level-set-based topology optimization method to design the permanent magnet for generators. The machine under study is a simplified 2D outer rotor direct-drive wind power generator. The dynamic and static models of this generator are studied, and the magnetostatic system is adopted to conduct the topology optimization. The optimization goals in this study mainly focused on two aspects, namely the maximization of the system magnetic energy and the generation of a target magnetic field in the region of the air gap. The continuum shape sensitivity analysis is derived by using the material time derivative, the Lagrange multiplier method, and the adjoint variable method. Two numerical examples are investigated, and the effectiveness of the proposed design framework is validated by comparing the performance of the original design against the optimized design.
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- Award ID(s):
- 1762287
- NSF-PAR ID:
- 10351916
- Date Published:
- Journal Name:
- ASME Design Engineering Technical Conferences
- ISSN:
- 1523-6501
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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