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Over the last few decades, nonlinear optics has become significantly more nonlinear, traversing nearly a billionfold improvement in energy efficiency, with ultrafast nonlinear nanophotonics in particular emerging as a frontier for combining both spatial and temporal engineering. At present, cutting-edge experiments in nonlinear nanophotonics place us just above themesoscopicregime, where a few hundred photons suffice to trigger highly nonlinear dynamics. In contrast to classical or deep-quantum optics, the mesoscale is characterized by dynamical interactions between mean-field, Gaussian, and non-Gaussian quantum features, all within a close hierarchy of scales. When combined with the inherent multimode complexity of optical fields, such hybrid quantum-classical dynamics present theoretical, experimental, and engineering challenges to the contemporary framework of quantum optics. In this review, we highlight the unique physics that emerges in multimode nonlinear optics at the mesoscale and outline key principles for exploiting both classical and quantum features to engineer novel functionalities. We briefly survey the experimental landscape and draw attention to outstanding technical challenges in materials, dispersion engineering, and device design for accessing mesoscopic operation. Finally, we speculate on how these capabilities might usher in some new paradigms in quantum photonics, from quantum-augmented information processing to nonclassical-light-driven dynamics and phenomena to all-optical non-Gaussian measurement and sensing. The physics unlocked at the mesoscale present significant challenges and opportunities in theory and experiment alike, and this review is intended to serve as a guide to navigating this new frontier in ultrafast quantum nonlinear optics.
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Onset of non-Gaussian quantum physics in pulsed squeezing with mesoscopic fields
We study the emergence of non-Gaussian quantum features in pulsed squeezed light generation with a mesoscopic number (i.e., dozens to hundreds) of pump photons. Due to the strong optical nonlinearities necessarily involved in this regime, squeezing occurs alongside significant pump depletion, compromising the predictions made by conventional semiclassical models for squeezing. Furthermore, nonlinear interactions among multiple frequency modes render the system dynamics exponentially intractable in naïve quantum models, requiring a more sophisticated modeling framework. To this end, we construct a nonlinear Gaussian approximation to the squeezing dynamics, defining a “Gaussian interaction frame” in which non-Gaussian quantum dynamics can be isolated and concisely described using a few dominant (i.e., principal) supermodes. Numerical simulations of our model reveal non-Gaussian distortions of squeezing in the mesoscopic regime, largely associated with signal-pump entanglement. We argue that state of the art in nonlinear nanophotonics is quickly approaching this regime, providing an all-optical platform for experimental studies of the semiclassical-to-quantum transition in a rich paradigm of coherent, multimode nonlinear dynamics. Mesoscopic pulsed squeezing, thus, provides an intriguing case study of the rapid rise in dynamic complexity associated with semiclassical-to-quantum crossover, which we view as a correlate of the emergence of new information processing capacities in the quantum regime.
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- PAR ID:
- 10369359
- Publisher / Repository:
- Optical Society of America
- Date Published:
- Journal Name:
- Optica
- Volume:
- 9
- Issue:
- 4
- ISSN:
- 2334-2536
- Format(s):
- Medium: X Size: Article No. 379
- Size(s):
- Article No. 379
- Sponsoring Org:
- National Science Foundation
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