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  • Spatiotemporal quantification of organic matter accumulation in the Eocene Green River Formation, Bridger Basin, Wyoming
Title: Spatiotemporal quantification of organic matter accumulation in the Eocene Green River Formation, Bridger Basin, Wyoming
It has long been recognized that lakes can bury large amounts of organic carbon (CORG) in their sediment, with important consequences for conventional and unconventional petroleum resources and potentially for the global carbon cycle. The detailed distribution of lacustrine organic carbon through space and time is important to understanding its commercial and climatic implications, but has seldom been documented in detail. The Green River Formation offers a unique opportunity to improve this understanding, due to extensive Fischer assay analyses of its oil generative potential and to recently published radioisotopic age analyses of intercalat ed volcanic tuffs. Fischer assay analyses reveal distinctly different patterns of organic matter enrichment that correlate with different lacustrine facies associations. Histograms of oil generative potential for evaporative facies of the Wilkins Peak Member exhibit an approximately exponential distribution. This pattern is interpret ed to result from episodic expansion and contraction of Eocene Lake Gosiute across a low-gradient basin floor that experienced frequent desiccation. In contrast, histograms for fluctuating profundal facies of the upper Rife Bed of the Tipton Member and the lower LaClede Bed of the Laney Member exhibit an approximately normal or log normal distribution, with modes as high as 16–18 gallons per ton. This pattern is interpreted to reflect generally deeper conditions when the lake often intersected basin-bounding uplifts. Within the Bridger basin, burial of CORG was greatest in the south during initial Wilkins Peak Member deposition, reflecting greater rates of accommodation near the Uinta uplift. The locus of CORG burial shifted north during upper Wilkins Peak Member deposition, coincident with a decrease in differential accommodation. CORG burial during deposition of the upper Rife and lower LaClede Beds was greatest in the southeast, due either to greater accommodation or localized influx of river-borne nutrients. Average CORG burial fluxes are consistently ~4-5 g/m2 yr for each interval, which is an order of magnitude less than fluxes reported for small Holocene lakes in the northern hemisphere. Maximum rates of CORG burial during deposition of organic-rich mudstone beds (oil shale) were likely similar to Holocene lakes however. Deposition of carbonate minerals in the Bridger basin resulted in additional, inorganic carbon burial. Overall it appears that carbon burial by Eocene lakes could have influenced the global carbon cycle, but only if synchronized across multiple lake systems.  more » « less
Award ID(s):
1813278
PAR ID:
10438619
Author(s) / Creator(s):
;
Date Published:
Journal Name:
Geosites
Volume:
50
ISSN:
0375-8176
Page Range / eLocation ID:
1 to 20
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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  1. ; ; ; ; (, Geological Society of America)
    Lacustrine chemical sediments of the Wilkins Peak Member, Eocene Green River Formation potentially preserve paleoclimate information relating to the conditions of their formation and preservation within the lake basin during the Early Eocene Climatic Optimum. The Green River Formation comprises the world’s largest sodium-carbonate evaporite deposit in the form of trona (Na2CO3⋅NaHCO3⋅2H2O) in the Bridger sub-basin and nahcolite (NaHCO3) in the neighboring Piceance Creek basin. Modern analogues suggest that these minerals necessitate the existence of an alkaline source water. Detrital provenance geochronometers suggest that the most likely source for volcanic waters to the Greater Green River Basin is the Colorado Mineral Belt, connected to the basin via the Aspen paleo-river. We tested the hypothesis that magmatic waters from the Colorado Mineral Belt could have supplied the Greater Green River Basin with the alkalinity needed to precipitate sodium-carbonate evaporites that are preserved in the Wilkins Peak Member by numerically simulating the evaporation of modern soda spring waters from northwestern Colorado at various temperature and atmospheric pCO2 conditions. We compare the resulting simulated evaporite sequences of the modern soda spring waters to the mineralogy preserved within the Wilkins Peak Member. Simulated evaporation of Steamboat Springs water produces the closest match to core observations and mineralogy. These simulations provide constraints on the salinities at which various minerals precipitated in the Wilkins Peak Member as well as insights into the regional temperature (>15ºC for gaylussite and trona; >27º for pirssonite and trona) and pCO2 conditions (<1200ppm for gaylussite and trona) during the EECO. 
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  2. (, Geological Society of America bulletin)
    The Green River Formation of Wyoming, USA, is host to the world’s largest known lacustrine sodium carbonate deposits, which accumulated in a closed basin during the early Eocene greenhouse. Alkaline brines are hypothesized to have been delivered to ancient Gosiute Lake by the Aspen paleoriver that flowed from the Colorado Mineral Belt. To precisely trace fluvial provenance in the resulting deposits, we conducted X-ray fluorescence analyses and petrographic studies across a suite of well-dated sandstone marker beds of the Wilkins Peak Member of the Green River Formation. Principal component analysis reveals strong correlation among elemental abundances, grain composition, and sedimentary lithofacies. To isolate a detrital signal, elements least affected by authigenic minerals, weathering, and other processes were included in a principal component analysis, the results of which are consistent with petrographic sandstone modes and detrital zircon chronofacies of the basin. Sandstone marker beds formed during eccentricity-paced lacustrine lowstands and record the migration of fluvial distributary channel networks from multiple catchments around a migrating depocenter, including two major paleorivers. The depositional topography of these convergent fluvial fans would have inversely defined bathymetric lows during subsequent phases of lacustrine inundation, locations where trona could accumulate below a thermocline. Provenance mapping verifies fluvial connectivity to the Aspen paleoriver and to sources of alkalinity in the Colorado Mineral Belt across Wilkins Peak Member deposition, and shows that the greatest volumes of sediment were delivered from the Aspen paleoriver during deposition of marker beds A, B, D, and I, each of which were deposited coincident with prominent “hyperthermal” isotopic excursions documented in oceanic cores. 
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  3. ; ; ; ; ; ; ; ; ; ; et al (, Geological Society of America Bulletin)
    None (Ed.)
    Abstract The Green River Formation of Wyoming, USA, is host to the world’s largest known lacustrine sodium carbonate deposits, which accumulated in a closed basin during the early Eocene greenhouse. Alkaline brines are hypothesized to have been delivered to ancient Gosiute Lake by the Aspen paleoriver that flowed from the Colorado Mineral Belt. To precisely trace fluvial provenance in the resulting deposits, we conducted X-ray fluorescence analyses and petrographic studies across a suite of well-dated sandstone marker beds of the Wilkins Peak Member of the Green River Formation. Principal component analysis reveals strong correlation among elemental abundances, grain composition, and sedimentary lithofacies. To isolate a detrital signal, elements least affected by authigenic minerals, weathering, and other processes were included in a principal component analysis, the results of which are consistent with petrographic sandstone modes and detrital zircon chronofacies of the basin. Sandstone marker beds formed during eccentricity-paced lacustrine lowstands and record the migration of fluvial distributary channel networks from multiple catchments around a migrating depocenter, including two major paleorivers. The depositional topography of these convergent fluvial fans would have inversely defined bathymetric lows during subsequent phases of lacustrine inundation, locations where trona could accumulate below a thermocline. Provenance mapping verifies fluvial connectivity to the Aspen paleoriver and to sources of alkalinity in the Colorado Mineral Belt across Wilkins Peak Member deposition, and shows that the greatest volumes of sediment were delivered from the Aspen paleoriver during deposition of marker beds A, B, D, and I, each of which were deposited coincident with prominent “hyperthermal” isotopic excursions documented in oceanic cores. 
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  4. ; ; ; ; ; (, Geosites)
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  5. ; ; ; ; ; ; ; (, Sedimentology)
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