Title: Nuclear fission properties of super heavy nuclei described within the four-dimensional Langevin model
Understanding of fission properties of super-heavy nuclei (SHN) is essential not only for the synthesis of new elements but also for astrophysical nucleosynthesis because fission fragments from SHN are recycled as the seed nuclei of the r-process. A recent discovery of the r-process site by the gravitational wave observations requires more precise nuclear information for the detailed simulation of the r-process nucleosynthesis. However, the fission mechanisms of the SHN are not understood well, and therefore theoretical predictions of distributions of the fission fragments of SHN are very model-dependent. Our four-dimensional Langevin model can calculate various properties of the fission fragments, such as the distribution of fission yields, kinetic energies, and deformation of fission fragments and their correlations just after scission. Those results are consistent with the experimental data, especially in the actinide region without adjusting parameters. Based on such a reliable model, we previously investigated the fission of representative SHN where the experimental data exist and found that doubly-magic shell closure of 132 Sn and 208 Pb dominates the fission process. This paper demonstrates the results of our calculations for the systematics of fission yield and the total kinetic energies from the neutron-rich to the neutron-deficient side of SHN. We also show decomposition of fission modes, such as standard/super-long/super-short modes, based on a Brosa-like concept. more »« less
Vassh, Nicole; Mumpower, Matthew; Sprouse, Trevor; Surman, Rebecca; Vogt, Ramona
(, EPJ Web of Conferences)
Kawano, T.
(Ed.)
We review recent work examining the influence of fission in rapid neutron capture ( r -process) nucleosynthesis which can take place in astrophysical environments. We briefly discuss the impact of uncertain fission barriers and fission rates on the population of heavy actinide species. We demonstrate the influence of the fission fragment distributions for neutron-rich nuclei and discuss currently available treatments, including recent macroscopic-microscopic calculations. We conclude by comparing our nucleosynthesis results directly with stellar data for metal-poor stars rich in r -process elements to consider whether fission plays a role in the so-called ‘universality’ of r -process abundances observed from star to star.
Roederer, Ian U; Vassh, Nicole; Holmbeck, Erika M; Mumpower, Matthew R; Surman, Rebecca; Cowan, John J; Beers, Timothy C; Ezzeddine, Rana; Frebel, Anna; Hansen, Terese T; et al
(, Science)
The heaviest chemical elements are naturally produced by the rapid neutron-capture process (r-process) during neutron star mergers or supernovae. Ther-process production of elements heavier than uranium (transuranic nuclei) is poorly understood and inaccessible to experiments so must be extrapolated by using nucleosynthesis models. We examined element abundances in a sample of stars that are enhanced inr-process elements. The abundances of elements ruthenium, rhodium, palladium, and silver (atomic numbersZ= 44 to 47; mass numbersA= 99 to 110) correlate with those of heavier elements (63 ≤Z≤ 78,A> 150). There is no correlation for neighboring elements (34 ≤Z≤ 42 and 48 ≤Z≤ 62). We interpret this as evidence that fission fragments of transuranic nuclei contribute to the abundances. Our results indicate that neutron-rich nuclei with mass numbers >260 are produced inr-process events.
Psaltis, A.; Arcones, A.; Montes, F.; Mohr, P.; Hansen, C. J.; Jacobi, M.; Schatz, H.
(, The Astrophysical Journal)
Abstract A promising astrophysical site to produce the lighter heavy elements of the first r -process peak ( Z = 38 − 47) is the moderately neutron-rich (0.4 < Y e < 0.5) neutrino-driven ejecta of explosive environments, such as core-collapse supernovae and neutron star mergers, where the weak r -process operates. This nucleosynthesis exhibits uncertainties from the absence of experimental data from ( α , xn ) reactions on neutron-rich nuclei, which are currently based on statistical model estimates. In this work, we report on a new study of the nuclear reaction impact using a Monte Carlo approach and improved ( α , xn ) rates based on the Atomki-V2 α optical model potential. We compare our results with observations from an up-to-date list of metal-poor stars with [Fe/H] < −1.5 to find conditions of the neutrino-driven wind where the lighter heavy elements can be synthesized. We identified a list of ( α , xn ) reaction rates that affect key elemental ratios in different astrophysical conditions. Our study aims to motivate more nuclear physics experiments on ( α , xn ) reactions using the current and new generation of radioactive beam facilities and also more observational studies of metal-poor stars.
Jolie A. Cizewski, Andrew Ratkiewicz
(, Compound-Nuclear Reactions, Springer Proceedings in Physics 254)
null
(Ed.)
Neutron capture reactions are responsible for the synthesis of almost all of the elements heavier than iron through the slow s-process, that proceeds close to the line of stability, and the rapid r-process, with very neutron-rich waiting points. Uncertainties in (n,γ) rates in neutron rich nuclei, especially near closed neu- tron shells, can have significant impact [1] on the predictions of final abundances for different astrophysical scenarios for the r process. Understanding (n,γ) rates on neutron-rich fission fragments is also important for nuclear forensics and stockpile stewardship science. Ratkiewicz et al. [2 and references therein] has recently demonstrated that the (d,pγ) reaction is a valid surrogate for (n,γ), where the formation of the compound nu- cleus from the breakup of the deuteron has been calculated in a reaction model and the subsequent measured gamma-decay probabilities are reproduced with standard level density and strength functions in a Bayesian approach. In parallel to the surrogate validation efforts, we have demonstrated that the (d,pγ) reaction can be measured in inverse kinematics with Gammasphere ORRUBA: Dual Detectors for Experimental Structure Studies (GODDESS) [3] where the Gammasphere array of Compton-suppressed HPGe detectors is coupled to the Oak Ridge Rutgers University Barrel Array of position-sensitive silicon strip detectors. During the commis- sioning campaign we measured the (d,pγ) reaction with 134Xe and 95Mo beams, the latter to demonstrate the surrogate method in inverse kinematics. The present talk will present preliminary results from this campaign including γ-decay probabilities and prospects for surrogate (n,γ) measurements with 143Ba fission-fragment beams.
β -decay rates of neutron-rich nuclei, in particular those located at neutron shell closures, play a central role in simulations of the heavy-element nucleosynthesis and resulting abundance distributions. We present β -decay half-lives of even-even N = 82 and N = 126 r -process waiting-point nuclei calculated in the approach based on relativistic quasiparticle random phase approximation with quasiparticle-vibration coupling. The calculations include both allowed and first-forbidden transitions. In the N = 82 chain, the quasiparticlevibration coupling has an important impact close to stability, as it increases the contribution of Gamow-Teller modes and improves the agreement with the available data. In the N = 126 chain, we find the decay to proceed dominantly via first-forbidden transitions, even when the coupling to vibrations is included.
Ishizuka, Chikako, Zhang, Xuan, Shimada, Kazuya, Usang, Mark, Ivanyuk, Fedir, and Chiba, Satoshi. Nuclear fission properties of super heavy nuclei described within the four-dimensional Langevin model. Retrieved from https://par.nsf.gov/biblio/10464901. Frontiers in Physics 11. Web. doi:10.3389/fphy.2023.1111868.
Ishizuka, Chikako, Zhang, Xuan, Shimada, Kazuya, Usang, Mark, Ivanyuk, Fedir, & Chiba, Satoshi. Nuclear fission properties of super heavy nuclei described within the four-dimensional Langevin model. Frontiers in Physics, 11 (). Retrieved from https://par.nsf.gov/biblio/10464901. https://doi.org/10.3389/fphy.2023.1111868
Ishizuka, Chikako, Zhang, Xuan, Shimada, Kazuya, Usang, Mark, Ivanyuk, Fedir, and Chiba, Satoshi.
"Nuclear fission properties of super heavy nuclei described within the four-dimensional Langevin model". Frontiers in Physics 11 (). Country unknown/Code not available. https://doi.org/10.3389/fphy.2023.1111868.https://par.nsf.gov/biblio/10464901.
@article{osti_10464901,
place = {Country unknown/Code not available},
title = {Nuclear fission properties of super heavy nuclei described within the four-dimensional Langevin model},
url = {https://par.nsf.gov/biblio/10464901},
DOI = {10.3389/fphy.2023.1111868},
abstractNote = {Understanding of fission properties of super-heavy nuclei (SHN) is essential not only for the synthesis of new elements but also for astrophysical nucleosynthesis because fission fragments from SHN are recycled as the seed nuclei of the r-process. A recent discovery of the r-process site by the gravitational wave observations requires more precise nuclear information for the detailed simulation of the r-process nucleosynthesis. However, the fission mechanisms of the SHN are not understood well, and therefore theoretical predictions of distributions of the fission fragments of SHN are very model-dependent. Our four-dimensional Langevin model can calculate various properties of the fission fragments, such as the distribution of fission yields, kinetic energies, and deformation of fission fragments and their correlations just after scission. Those results are consistent with the experimental data, especially in the actinide region without adjusting parameters. Based on such a reliable model, we previously investigated the fission of representative SHN where the experimental data exist and found that doubly-magic shell closure of 132 Sn and 208 Pb dominates the fission process. This paper demonstrates the results of our calculations for the systematics of fission yield and the total kinetic energies from the neutron-rich to the neutron-deficient side of SHN. We also show decomposition of fission modes, such as standard/super-long/super-short modes, based on a Brosa-like concept.},
journal = {Frontiers in Physics},
volume = {11},
author = {Ishizuka, Chikako and Zhang, Xuan and Shimada, Kazuya and Usang, Mark and Ivanyuk, Fedir and Chiba, Satoshi},
}
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