skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.

Explore Research Products in the PAR
It may take a few hours for recently added research products to appear in PAR search results.


Title: Breakdown of the drift-diffusion model for transverse spin transport in a disordered Pt film
Spin-accumulation and spin-current profiles are calculated for a disordered Pt film subjected to an in-plane electric current within the nonequilibrium Green's function approach. In the bulklike region of the sample, this approach captures the intrinsic spin Hall effect found in other calculations. Near the surfaces, the results reveal qualitative differences with the results of the widely used spin-diffusion model, even when the boundary conditions are modified to try to account for them. One difference is that the effective spin-diffusion length for transverse spin transport is significantly different from its longitudinal counterpart and is instead similar to the mean-free path. This feature may be generic for spin currents generated via the intrinsic spin Hall mechanism because of the differences in transport mechanisms compared to longitudinal spin transport. Orbital accumulation in the Pt film is only significant in the immediate vicinity of the surfaces and has a small component penetrating into the bulk only in the presence of spin-orbit coupling, as a secondary effect induced by the spin accumulation.  more » « less
Award ID(s):
1916275
PAR ID:
10470683
Author(s) / Creator(s):
; ; ; ; ; ;
Publisher / Repository:
American Physical Society
Date Published:
Journal Name:
Physical Review B
Volume:
108
Issue:
14
ISSN:
2469-9950
Page Range / eLocation ID:
144433
Subject(s) / Keyword(s):
spin Hall effect spin accumulation spin current spin diffusion spin-orbit torque nonequilibrium Green's function
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. ; ; ; ; ; ; ; ; (, Applied Physics Letters)
    Spin-to-charge conversion (S2CC) processes in thin-film heterostructures have attracted much attention in recent years. Here, we describe the S2CC in a 3D topological insulator Bi2Te3 interfaced with an epitaxial film of Fe75Co25. The quantification of spin-to-charge conversion is made with two complementary techniques: ferromagnetic resonance based inverse spin Hall effect (ISHE) at GHz frequencies and femtosecond light-pulse induced emission of terahertz (THz) radiation. The role of spin rectification due to extrinsic effects like anisotropic magnetoresistance (AMR) and planar Hall effects (PHE) is pronounced at the GHz timescale, whereas the THz measurements do not show any detectible signal, which could be attributed to AMR or PHE. This result may be due to (i) homodyne rectification at GHz, which is absent in THz measurements and (ii) laser-induced thermal spin current generation and magnetic dipole radiation in THz measurements, which is completely absent in GHz range. The converted charge current has been analyzed using the spin diffusion model for the ISHE. We note that regardless of the differences in timescales, the spin diffusion length in the two cases is comparable. Our results aid in understanding the role of spin pumping timescales in the generation of ISHE signals. 
    more » « less
  2. ; ; ; ; ; ; ; ; ; ; et al (, Journal of Applied Physics)
    Orbital current has attracted significant attention in recent years due to its potential for energy-efficient magnetization control without the need for materials with strong spin–orbit coupling. However, the fundamental mechanisms governing orbital transport remain elusive. In this study, we systematically explore orbital transport in Ti/Ni bilayers through orbital pumping, drawing an analogy to spin pumping. The orbital current is generated and injected into the Ti layer via the microwave-driven orbital dynamics in Ni, facilitated by its strong spin–orbit correlation. We employed thickness-dependent ferromagnetic resonance measurements and angular-dependent inverse orbital Hall effect (IOHE) detection to probe orbital transport in Ti based on the conventional spin-pumping methodology. The observed enhancement in the damping factor indicates an orbital-diffusion length of ∼5.3 ± 3.7 nm, while IOHE-based estimation suggests a value of around 4.0 ± 1.2 nm, which confirms its short orbital-diffusion length. Furthermore, oblique Hanle measurements in the longitudinal configuration reveal an orbital relaxation time of approximately 16 ps. Our results establish that orbital pumping, analogous to the conventional spin-pumping framework, can serve as a robust technique for elucidating orbital transport mechanisms, paving the way for the design of efficient spin-orbitronic devices. 
    more » « less
  3. ; ; ; ; ; ; ; ; (, AIP Advances)
    We present a study of the transport properties of thermally generated spin currents in an insulating ferrimagnetic-antiferromagnetic-ferrimagnetic trilayer over a wide range of temperature. Spin currents generated by the spin Seebeck effect (SSE) in a yttrium iron garnet (YIG) YIG/NiO/YIG trilayer on a gadolinium gallium garnet (GGG) substrate were detected using the inverse spin Hall effect (ISHE) in Pt. By studying samples with different NiO thicknesses, the spin diffusion length of NiO was determined to be ∼3.8 nm at room temperature. Surprisingly, a large increase of the SSE signal was observed below 30 K, and the field dependence of the signal closely follows a Brillouin function for an S=7/2 spin. The increase of the SSE signal at low temperatures could thus be associated with the paramagnetic SSE from the GGG substrate. Besides, a broad peak in the SSE response was observed around 100 K. These observations are important in understanding the generation and transport properties of spin currents through magnetic insulators and the role of a paramagnetic substrate in spin current generation. 
    more » « less
  4. ; ; ; ; ; (, Journal of Applied Physics)
    Spin-to-charge conversion and the reverse process are now critically important physical processes for a wide range of fundamental and applied studies in spintronics. Here, we experimentally demonstrate effective spin-to-charge conversion in thermally evaporated chromium thin films using the longitudinal spin Seebeck effect (LSSE). We present LSSE results measured near room temperature for Cr films with thicknesses from 2 to 11 nm, deposited at room temperature on bulk polycrystalline yttrium-iron-garnet (YIG) substrates. Comparison of the measured LSSE voltage, [Formula: see text], in Cr to a sputtered Pt film at the same nominal thickness grown on a matched YIG substrate shows that both films show comparably large spin-to-charge conversion. As previously shown for other forms of Cr, the LSSE signal for evaporated Cr/YIG shows the opposite sign compared to Pt, indicating that Cr has a negative spin Hall angle, [Formula: see text]. We also present measured charge resistivity, [Formula: see text], of the same evaporated Cr films on YIG. These values are large compared to Pt and comparable to [Formula: see text]-W at a similar thickness. Non-monotonic behavior of both [Formula: see text] and [Formula: see text] with film thickness suggests that spin-to-charge conversion in evaporated Cr, which we expect has a different strain state than previously investigated sputtered films, could be modified by spin density wave antiferromagnetism in Cr. 
    more » « less
  5. ; ; ; ; ; ; ; (, Advanced Materials Interfaces)
    Abstract Magnetic heterostructures consisting of single‐crystal yttrium iron garnet (YIG) films coated with platinum are widely used in spin‐wave experiments related to spintronic phenomena such as the spin‐transfer‐torque, spin‐Hall, and spin‐Seebeck effects. However, spin waves in YIG/Pt bilayers experience much stronger attenuation than in bare YIG films. For micrometer‐thick YIG films, this effect is caused by microwave eddy currents in the Pt layer. This paper reports that by employing an excitation configuration in which the YIG film faces the metal plate of the microstrip antenna structure, the eddy currents in Pt are shunted and the transmission of the Damon–Eschbach surface spin wave is greatly improved. The reduction in spin‐wave attenuation persists even when the Pt coating is separated from the ground plate by a thin dielectric layer. This makes the proposed excitation configuration suitable for injection of an electric current into the Pt layer and thus for application in spintronics devices. The theoretical analysis carried out within the framework of the electrodynamic approach reveals how the platinum nanolayer and the nearby highly conductive metal plate affect the group velocity and the lifetime of the Damon–Eshbach surface wave and how these two wavelength‐dependent quantities determine the transmission characteristics of the spin‐wave device. 
    more » « less
  • Citation Formats
  • MLA
  • APA
  • Chicago
  • BibTeX
  • Save / Share this Record
  • Send to Email