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Title: Pixel Geometry Effect on PbS Quantum Dot/Graphene Nanohybrid Broadband Photodetectors
Abstract Photodetectors based on colloidal quantum dots (QD)/graphene nanohybrids are quantum sensors due to strong quantum confinement in both QD and graphene. The optoelectronic properties of QD/graphene nanohybrids are affected by the quantum physics that predicts a high photoconductive gain and hence photoresponsivity (R*) depending on the pixel length (L) asR*∝L−2. Experimental confirmation of the effect of the pixel geometric parameters on the optoelectronic properties of the QD/graphene photodetector is therefore important to elucidate the underlying quantum physics. Motivated by this, an array of PbS QDs/graphene nanohybrid photodetectors are designed with variable QD/graphene pixel lengthLand width (W) in the range of 10–150 µm for a study ofR*, noise, and specific detectivity (D*) in a broad spectrum of 400–1500 nm. Intriguingly,R*exhibits a monotonic decreasing trend of 1/L2while being independent ofW, confirming experimentally the theoretical prediction. Interestingly, this geometric effect on the photoresponsivity seems to be partially compensated by that in noise, leading toD*independent ofLandWat wavelengths in the ultraviolet‐visible‐near infrared range. This result sheds light on the quantum physics underlying the optoelectronic process in QD/graphene nanohybrids, which is important to the design of high‐quality QD/graphene photodetectors and imaging systems.  more » « less
Award ID(s):
2314401 1909292
PAR ID:
10521257
Author(s) / Creator(s):
; ; ; ;
Publisher / Repository:
Wiley
Date Published:
Journal Name:
Advanced Optical Materials
Volume:
12
Issue:
13
ISSN:
2195-1071
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
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