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1. Mid-IR spectroscopy of Er 3+ doped low-phonon CsCdCl 3 and CsPbCl 3 crystals

   https://doi.org/10.1364/JOSAB.470152  

   Brown, Ei_Ei ; Fleischman, Zackery_D ; McKay, Jason ; Hommerich, Uwe ; Kabir, Al_Amin ; Riggins, Jazmine ; Trivedi, Sudhir ; Dubinskii, Mark ( September 2022 , Journal of the Optical Society of America B)

   The mid-IR spectroscopic properties of${\mathrm{E}\mathrm{r}}^{3+}$doped low-phonon${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$crystals grown by the Bridgman technique have been investigated. Using optical excitations at$\sim <\#comment/>800\mathrm{n}\mathrm{m}$and$\sim <\#comment/>660\mathrm{n}\mathrm{m}$, both crystals exhibited IR emissions at$\sim <\#comment/>1.55$,$\sim <\#comment/>2.75$,$\sim <\#comment/>3.5$, and$\sim <\#comment/>4.5\text{µ<\#comment/>}\mathrm{m}$at room temperature. The mid-IR emission at 4.5 µm, originating from the${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition, showed a long emission lifetime of$\sim <\#comment/>11.6\mathrm{m}\mathrm{s}$for${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$, whereas${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$exhibited a shorter lifetime of$\sim <\#comment/>1.8\mathrm{m}\mathrm{s}$. The measured emission lifetimes of the${}^4{\mathrm{I}}_{9/2}$state were nearly independent of the temperature, indicating a negligibly small nonradiative decay rate through multiphonon relaxation, as predicted by the energy-gap law for low-maximum-phonon energy hosts. The room temperature stimulated emission cross sections for the${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition in${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$were determined to be$\sim <\#comment/>0.14\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$and$\sim <\#comment/>0.41\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$, respectively. The results of Judd–Ofelt analysis are presented and discussed.

    

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2. Strong optomechanical interactions with long-lived fundamental acoustic waves

   https://doi.org/10.1364/OPTICA.476764  

   Xu, Wendao ; Iyer, Arjun ; Jin, Lei ; Set, Sze_Y ; Renninger, William_H ( January 2023 , Optica)

   Traveling-wave optomechanical interactions, known as Brillouin interactions, have now been established as a powerful and versatile resource for photonic sources, sensors, and radio-frequency processors. However, established Brillouin-based interactions with sufficient interaction strengths involve short phonon lifetimes, which critically limit their performance for applications, including radio-frequency filtering and optomechanical storage devices. Here, we investigate a new paradigm of optomechanical interactions with tightly confined fundamental acoustic modes, which enables the unique and desirable combination of high optomechanical coupling, long phonon lifetimes, tunable phonon frequencies, and single-sideband amplification. Using sensitive four-wave mixing spectroscopy controlling for noise and spatial mode coupling, optomechanical interactions with long$><\#comment/>2\text{µ<\#comment/>}\mathrm{s}$phonon lifetimes and strong$><\#comment/>400{\mathrm{W}}^{-<\#comment/>1}{\mathrm{m}}^{-<\#comment/>1}$coupling are observed in a tapered fiber. In addition, we demonstrate novel phonon self-interference effects resulting from the unique combination of an axially varying device geometry with long phonon lifetimes. A generalized theoretical model, in excellent agreement with experiments, is developed with broad applicability to inhomogeneous optomechanical systems.

    

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3. Diel variability of bulk optical properties associated with the growth and division of small phytoplankton in the North Pacific Subtropical Gyre

   https://doi.org/10.1364/AO.394123  

   Henderikx_Freitas, Fernanda ; Dugenne, Mathilde ; Ribalet, François ; Hynes, Annette ; Barone, Benedetto ; Karl, David_M ; White, Angelicque_E ( July 2020 , Applied Optics)

   Cross-platform observing systems are requisite to capturing the temporal and spatial dynamics of particles in the ocean. We present simultaneous observations of bulk optical properties, including the particulate beam attenuation (${\mathit{\text{c}}}_{\mathit{\text{p}}}$) and backscattering ($b_{\text{bp}}$) coefficients, and particle size distributions collected in the North Pacific Subtropical Gyre. Clear and coherent diel cycles are observed in all bulk and size-fractionated optical proxies for particle biomass. We show evidence linking diurnal increases in${\mathit{\text{c}}}_{\mathit{\text{p}}}$and${\mathit{\text{b}}}_{\text{bp}}$to daytime particle growth and division of cells, with particles$<<\#comment/>7\text{µ<\#comment/>}\mathrm{m}$driving the daily cycle of particle production and loss within the mixed layer. Flow cytometry data reveal the nitrogen-fixing cyanobacteriumCrocosphaera($\sim <\#comment/>4-<\#comment/>7\text{µ<\#comment/>}\mathrm{m}$) to be an important driver of${\mathit{\text{c}}}_{\mathit{\text{p}}}$at the time of sampling, whereasProchlorococcusdynamics ($\sim <\#comment/>0.5\text{µ<\#comment/>}\mathrm{m}$) were essential to reproducing temporal variability in${\mathit{\text{b}}}_{\text{bp}}$. This study is a step towards improved characterization of the particle size range represented byin situbulk optical properties and a better understanding of the mechanisms that drive variability in particle production in the oligotrophic open ocean.

    

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4. Electro-optic interface for ultrasensitive intracavity electric field measurements at microwave and terahertz frequencies

   https://doi.org/10.1364/OPTICA.384160  

   Benea-Chelmus, Ileana-Cristina ; Salamin, Yannick ; Settembrini, Francesca_Fabiana ; Fedoryshyn, Yuriy ; Heni, Wolfgang ; Elder, Delwin_L ; Dalton, Larry_R ; Leuthold, Juerg ; Faist, Jérôme ( May 2020 , Optica)

   Electro-optic quantum coherent interfaces map the amplitude and phase of a quantum signal directly to the phase or intensity of a probe beam. At terahertz frequencies, a fundamental challenge is not only to sense such weak signals (due to a weak coupling with a probe in the near-infrared) but also to resolve them in the time domain. Cavity confinement of both light fields can increase the interaction and achieve strong coupling. Using this approach, current realizations are limited to low microwave frequencies. Alternatively, in bulk crystals, electro-optic sampling was shown to reach quantum-level sensitivity of terahertz waves. Yet, the coupling strength was extremely weak. Here, we propose an on-chip architecture that concomitantly provides subcycle temporal resolution and an extreme sensitivity to sense terahertz intracavity fields below 20 V/m. We use guided femtosecond pulses in the near-infrared and a confinement of the terahertz wave to a volume of$V_{\mathrm{T}\mathrm{H}\mathrm{z}}\sim <\#comment/>{10}^{-<\#comment/>9}({\mathrm{\lambda <\#comment/>}}_{\mathrm{T}\mathrm{H}\mathrm{z}}/2{)}^3$in combination with ultraperformant organic molecules ($r_{33}=170\mathrm{p}\mathrm{m}/\mathrm{V}$) and accomplish a record-high single-photon electro-optic coupling rate of$g_{\mathrm{e}\mathrm{o}}=2\mathrm{\pi <\#comment/>}\times <\#comment/>0.043\mathrm{G}\mathrm{H}\mathrm{z}$, 10,000 times higher than in recent reports of sensing vacuum field fluctuations in bulk media. Via homodyne detection implemented directly on chip, the interaction results into an intensity modulation of the femtosecond pulses. The single-photon cooperativity is$C_0=1.6\times <\#comment/>{10}^{-<\#comment/>8}$, and the multiphoton cooperativity is$C=0.002$at room temperature. We show$><\#comment/>70\mathrm{d}\mathrm{B}$dynamic range in intensity at 500 ms integration under irradiation with a weak coherent terahertz field. Similar devices could be employed in future measurements of quantum states in the terahertz at the standard quantum limit, or for entanglement of subsystems on subcycle temporal scales, such as terahertz and near-infrared quantum bits.

    

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5. Optomechanical inertial sensors

   https://doi.org/10.1364/AO.393061  

   Hines, Adam ; Richardson, Logan ; Wisniewski, Hayden ; Guzman, Felipe ( June 2020 , Applied Optics)

   We present a performance analysis of compact monolithic optomechanical inertial sensors that describes their key fundamental limits and overall acceleration noise floor. Performance simulations for low-frequency gravity-sensitive inertial sensors show attainable acceleration noise floors on the order of$1\times <\#comment/>{10}^{-<\#comment/>11}\mathrm{m}/{\mathrm{s}}^2\sqrt{\mathrm{H}\mathrm{z}}$. Furthermore, from our performance models, we devised an optimization approach for our sensor designs, sensitivity, and bandwidth trade space. We conducted characterization measurements of these compact mechanical resonators, demonstrating$\mathit{\text{mQ}}$-products at levels of 250 kg, which highlight their exquisite acceleration sensitivity.

    

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