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1. Constraints on bosonic dark matter from ultralow-field nuclear magnetic resonance

   https://doi.org/10.1126/sciadv.aax4539  

   Garcon, Antoine; Blanchard, John W.; Centers, Gary P.; Figueroa, Nataniel L.; Graham, Peter W.; Jackson Kimball, Derek F.; Rajendran, Surjeet; Sushkov, Alexander O.; Stadnik, Yevgeny V.; Wickenbrock, Arne; et al (October 2019, Science Advances)

   The nature of dark matter, the invisible substance making up over 80% of the matter in the universe, is one of the most fundamental mysteries of modern physics. Ultralight bosons such as axions, axion-like particles, or dark photons could make up most of the dark matter. Couplings between such bosons and nuclear spins may enable their direct detection via nuclear magnetic resonance (NMR) spectroscopy: As nuclear spins move through the galactic dark-matter halo, they couple to dark matter and behave as if they were in an oscillating magnetic field, generating a dark-matter–driven NMR signal. As part of the cosmic axion spin precession experiment (CASPEr), an NMR-based dark-matter search, we use ultralow-field NMR to probe the axion-fermion “wind” coupling and dark-photon couplings to nuclear spins. No dark matter signal was detected above background, establishing new experimental bounds for dark matter bosons with masses ranging from 1.8 × 10 −16 to 7.8 × 10 −14 eV. 

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2. Overview of the Cosmic Axion Spin Precession Experiment (CASPEr)

   Jackson Kimball, D. F.; Afach, S.; Aybas, D.; Blanchard, J. W.; Budker, D.; Centers, G.; Engler, M.; Figueroa, N. L.; Garcon, A.; Graham, P. W.; et al (January 2020, Springer proceedings in physics)

   Carosi, G.; Rybka, G. (Ed.)

   An overview of our experimental program to search for axion and axion-like-particle (ALP) dark matter using nuclear magnetic resonance (NMR) techniques is presented. An oscillating axion field can exert a time-varying torque on nuclear spins either directly or via generation of an oscillating nuclear electric dipole moment (EDM). Magnetic resonance techniques can be used to detect such an effect. The first-generation experiments explore many decades of ALP parameter space beyond the current astrophysical and laboratory bounds. It is anticipated that future versions of the experiments will be sensitive to the axions associated with quantum chromodynamics (QCD) having masses <10^(−9) eV/c^2. 

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3. Axion detection via superfluid 3He ferromagnetic phase and quantum measurement techniques

   https://doi.org/10.1007/JHEP09(2024)191  

   Chigusa, So; Kondo, Dan; Murayama, Hitoshi; Okabe, Risshin; Sudo, Hiroyuki (September 2024, Journal of High Energy Physics)

   A<sc>bstract</sc> We propose to use the nuclear spin excitation in the ferromagnetic A₁phase of the superfluid³He for the axion dark matter detection. This approach is striking in that it is sensitive to the axion-nucleon coupling, one of the most important features of the QCD axion introduced to solve the strong CP problem. We review a quantum mechanical description of the nuclear spin excitation and apply it to the estimation of the axion-induced spin excitation rate. We also describe a possible detection method of the spin excitation in detail and show that the combination of the squeezing of the final state with the Josephson parametric amplifier and the homodyne measurement can enhance the sensitivity. It turns out that this approach gives good sensitivity to the axion dark matter with the mass of$$ \mathcal{O} $$ $O$(1) μeV depending on the size of the external magnetic field. We estimate the parameters of experimental setups, e.g., the detector volume and the amplitude of squeezing, required to reach the QCD axion parameter space. 

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4. Search for axionlike dark matter using liquid-state nuclear magnetic resonance

   https://doi.org/10.1103/39nc-vr9m  

   Walter, Julian; Maliaka, Olympia; Zhang, Yuzhe; Blanchard, John W; Centers, Gary; Dogan, Arian; Engler, Martin; Figueroa, Nataniel L; Kim, Younggeun; Kimball, Derek_F Jackson; et al (September 2025, Physical Review D)

   We search for dark matter in the form of axionlike particles (ALPs) in the mass range $5.576741\mathrm{neV}/{\mathrm{c}}^2-5.577733\mathrm{neV}/{\mathrm{c}}^2$by probing their possible coupling to fermion spins through the ALP field gradient. This is achieved by performing proton nuclear magnetic resonance spectroscopy on a sample of methanol as a technical demonstration of the Cosmic Axion Spin Precession Experiment Gradient (CASPEr-Gradient) Low-Field apparatus. Searching for spin-coupled ALP dark matter in this mass range with associated Compton frequencies in a 240 Hz window centered at 1.348570 MHZ resulted in a sensitivity to the ALP-proton coupling constant of $g_{\mathrm{ap}}\approx 3\times {10}^{-2}{\mathrm{GeV}}^{-1}$. This narrow-bandwidth search serves as a proof-of-principle and a commissioning measurement, validating our methodology and demonstrating the experiment’s capabilities. CASPEr-Gradient Low-Field will probe the mass range from $4.1\mathrm{peV}/{\mathrm{c}}^2$to $17\mathrm{neV}/{\mathrm{c}}^2$with hyperpolarized samples to boost the sensitivity beyond the astronomical limits. 

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5. Searching for dark matter with a spin-based interferometer

   https://doi.org/10.1038/s41467-025-60178-6  

   Gavilan-Martin, Daniel; Łukasiewicz, Grzegorz; Padniuk, Mikhail; Klinger, Emmanuel; Smolis, Magdalena; Figueroa, Nataniel L; Jackson_Kimball, Derek F; Sushkov, Alexander O; Pustelny, Szymon; Budker, Dmitry; et al (December 2025, Nature Communications)

   Axion-like particles (ALPs) arise from well-motivated extensions to the Standard Model and could account for dark matter. ALP dark matter would manifest as a field oscillating at an (as of yet) unknown frequency. The frequency depends linearly on the ALP mass and plausibly ranges from 10⁻²²to 10 eV/c². This motivates broadband search approaches. We report on a direct search for ALP dark matter with an interferometer composed of two atomic K-Rb-³He comagnetometers, one situated in Mainz, Germany, and the other in Kraków, Poland. We leverage the anticipated spatio-temporal coherence properties of the ALP field and probe all ALP-gradient-spin interactions covering a mass range of nine orders of magnitude. No significant evidence of an ALP signal is found. We thus place new upper limits on the ALP-neutron, ALP-proton and ALP-electron couplings reaching belowg_aNN < 10⁻⁹ GeV⁻¹,g_aPP < 10⁻⁷ GeV⁻¹andg_aee < 10⁻⁶ GeV⁻¹, respectively. These limits improve upon previous laboratory constraints for neutron and proton couplings by up to three orders of magnitude. 

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