Abstract The search for Kitaev’s quantum spin liquid in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions required to stabilize the elusive entangled quantum state. The layered honeycomb Na3Co2SbO6has been singled out as a leading candidate provided that the trigonal crystal field acting on Co 3dorbitals, which enhances non-Kitaev exchange interactions between$${J}_{{{\rm{eff}}}}=\frac{1}{2}$$ spin-orbital pseudospins, is reduced. Here we show that applied pressure leads to anisotropic compression of the layered structure, significantly reducing the trigonal distortion of CoO6octahedra. Ferromagnetic correlations between pseudospins are enhanced in the spin-polarized (3 Tesla) phase up to about 60 GPa. Higher pressures drive a high-spin to low-spin transition destroying the$${J}_{{{\rm{eff}}}}=\frac{1}{2}$$ moments required to map the spin Hamiltonian into Kitaev’s model. The spin transition strongly suppresses the low-temperature magnetic susceptibility and appears to stabilize a paramagnetic phase driven by frustration. The possible emergence of frustrated magnetism of localized$$S=\frac{1}{2}$$ moments opens the door for exploration of novel magnetic quantum states in compressed honeycomb lattices of divalent cobaltates.
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Numerical signatures of ultra-local criticality in a one dimensional Kondo lattice model
Heavy fermion criticality has been a long-standing problem in condensed matter physics. Here we study a one-dimensional Kondo lattice model through numerical simulation and observe signatures of local criticality. We vary the Kondo couplingJ_K at fixed doping x. At large positiveJ_K , we confirm the expected conventional Luttinger liquid phase with2k_F=\frac{1+x}{2} (in units of2\pi ), an analogue of the heavy Fermi liquid (HFL) in the higher dimension. In theJ_K ≤ 0 side, our simulation finds the existence of a fractional Luttinger liquid (LL\star ) phase with2k_F=\frac{x}{2} , accompanied by a gapless spin mode originating from localized spin moments, which serves as an analogue of the fractional Fermi liquid (FL\star ) phase in higher dimensions. The LL\star phase becomes unstable and transitions to a spin-gapped Luther-Emery (LE) liquid phase at small positiveJ_K . Then we mainly focus on the “critical regime” between the LE phase and the LL phase. Approaching the critical point from the spin-gapped LE phase, we often find that the spin gap vanishes continuously, while the spin-spin correlation length in real space stays finite and small. For a certain range of doping, in a point (or narrow region) ofJ_K , the dynamical spin structure factor obtained through the time-evolving block decimation (TEBD) simulation shows dispersion-less spin fluctuations in a finite range of momentum space above a small energy scale (around0.035 J ) that is limited by the TEBD accuracy. All of these results are unexpected for a regular gapless phase (or critical point) described by conformal field theory (CFT). Instead, they are more consistent with exotic ultra-local criticality with an infinite dynamical exponentz=+ . The numerical discovery here may have important implications on our general theoretical understanding of the strange metals in heavy fermion systems. Lastly, we propose to simulate the model in a bilayer optical lattice with a potential difference.
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- Award ID(s):
- 2237031
- PAR ID:
- 10574523
- Publisher / Repository:
- Scipost
- Date Published:
- Journal Name:
- SciPost Physics
- Volume:
- 17
- Issue:
- 2
- ISSN:
- 2542-4653
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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