skip to main content
US FlagAn official website of the United States government
dot gov icon
Official websites use .gov
A .gov website belongs to an official government organization in the United States.
https lock icon
Secure .gov websites use HTTPS
A lock ( lock ) or https:// means you've safely connected to the .gov website. Share sensitive information only on official, secure websites.


Title: Quasisymmetry-Constrained Spin Ferromagnetism in Altermagnets
Altermagnets break time-reversal symmetry, and their spin-orbit coupling (SOC) allows for an anomalous Hall effect (AHE) that depends on the direction of the N´eel ordering vector. The AHE and the ferromagnetic spin moment share the same symmetry and hence are usually proportional. However, density functional theory (DFT) calculations find that the AHE exists with negligible ferromagnetic spin moment for some compounds, whereas it reaches sizable values for other altermagnets. By examining realistic minimal models for altermagnetism in which the DFT phenomenology is captured, we uncover a general SOC-enabled quasisymmetry, the uniaxial spin space group, that provides a natural explanation for the amplitude of the ferromagnetic spin moment across the vast range of different altermagnetic materials. Additionally, we derive analytic expressions for the magnetic anisotropy energy, providing a simple means of identifying the preferred N´eel vector orientation for altermagnets.  more » « less
Award ID(s):
2323857
PAR ID:
10637131
Author(s) / Creator(s):
; ; ; ; ;
Publisher / Repository:
Physical Review Letters
Date Published:
Journal Name:
Physical Review Letters
Volume:
135
Issue:
1
ISSN:
0031-9007
Format(s):
Medium: X
Sponsoring Org:
National Science Foundation
More Like this
  1. The anomalous Hall effect (AHE) is an efficient tool for detecting the Néel vector in collinear compensated magnets with spin-split bands, known as altermagnets (AMs). Here, we establish design principles for obtaining nonzero anomalous Hall conductivity in the recently proposed two-dimensional (2D) AMs using spin and magnetic group symmetry analysis. We show that only two of the seven nontrivial spin layer groups exhibit an unconventional in-plane AHE in which the Néel vector lies within the plane of the Hall current. Through first-principles simulations on bilayers of MnPSe3 and MnSe, we demonstrate the validity of our group theoretic framework for obtaining AHE with d- and i-wave altermagnetic orders, depending on the stacking of the bilayers. We find that the spin group symmetry is successful in determining the linear and cubic dependence of anomalous Hall conductivity in Néel vector space, although AHE is a relativistic effect. This work shows that the AHE in 2D AMs can probe the altermagnetic order and Néel vector reversal, thereby facilitating the miniaturization of altermagnetic spintronics. 
    more » « less
  2. Abstract Three-dimensional (3D) compensated MnBi 2 Te 4 is antiferromagnetic, but undergoes a spin-flop transition at intermediate fields, resulting in a canted phase before saturation. In this work, we experimentally show that the anomalous Hall effect (AHE) in MnBi 2 Te 4 originates from a topological response that is sensitive to the perpendicular magnetic moment and to its canting angle. Synthesis by molecular beam epitaxy allows us to obtain a large-area quasi-3D 24-layer MnBi 2 Te 4 with near-perfect compensation that hosts the phase diagram observed in bulk which we utilize to probe the AHE. This AHE is seen to exhibit an antiferromagnetic response at low magnetic fields, and a clear evolution at intermediate fields through surface and bulk spin-flop transitions into saturation. Throughout this evolution, the AHE is super-linear versus magnetization rather than the expected linear relationship. We reveal that this discrepancy is related to the canting angle, consistent with the symmetry of the crystal. Our findings bring to light a topological anomalous Hall response that can be found in non-collinear ferromagnetic, and antiferromagnetic phases. 
    more » « less
  3. Abstract The anomalous Hall effect (AHE), typically observed in ferromagnetic (FM) metals with broken time-reversal symmetry, depends on electronic and magnetic properties. In Co3Sn2-xInxS2, a giant AHE has been attributed to Berry curvature associated with the FM Weyl semimetal phase, yet recent studies report complicated magnetism. We use neutron scattering to determine the spin dynamics and structures as a function ofxand provide a microscopic understanding of the AHE and magnetism interplay. Spin gap and stiffness indicate a contribution from Weyl fermions consistent with the AHE. The magnetic structure evolves fromc-axis ferromagnetism at$$x = 0$$ x = 0 to a canted antiferromagnetic (AFM) structure with reducedc-axis moment and in-plane AFM order at$$x = 0.12$$ x = 0.12 and further reducedc-axis FM moment at$$x = 0.3$$ x = 0.3 . Since noncollinear spins can induce non-zero Berry curvature in real space acting as a fictitious magnetic field, our results revealed another AHE contribution, establishing the impact of magnetism on transport. 
    more » « less
  4. Crystallographic anisotropy of the spin-dependent conductivity tensor can be exploited to generate transverse spin-polarized current in a ferromagnetic film. This ferromagnetic spin Hall effect is analogous to the spin-splitting effect in altermagnets and does not require spin-orbit coupling. First-principles screening of 41 non-cubic ferromagnets revealed that many of them, when grown as a single crystal with tilted crystallographic axes, can exhibit large spin Hall angles comparable with the best available spin-orbit-driven spin Hall sources. Macroscopic spin Hall effect is possible for uniformly magnetized ferromagnetic films grown on some low-symmetry substrates with epitaxial relations that prevent cancellation of contributions from different orientation domains. Macroscopic response is also possible for any substrate if magnetocrystalline anisotropy is strong enough to lock the magnetization to the crystallographic axes in different orientation domains. 
    more » « less
  5. Altermagnets are crystallographic rotational symmetry breaking spin-ordered states, possessing a net zero magnetization despite manifesting Kramer's nondegenerate bands. Here, we show that momentum-independent local spin-nematic orders in monolayer, Bernal bilayer, and rhombohedral trilayer graphene give rise to 𝑝-wave, 𝑑-wave, and 𝑓-wave altermagnets, respectively, thereby inheriting the topology of linear, quadratic, and cubic free fermion band dispersions that are also described in terms of angular momentum ℓ=1,2, and 3 harmonics in the reciprocal space. The same conclusions also hold inside a spin-triplet nematic superconductor, featuring Majorana altermagnets. Altogether, these findings highlight the importance of electronic band structure in identifying such exotic magnetic orders in quantum materials. We depict the effects of in-plane magnetic fields on altermagnets, and propose spin-disordered alter-valley magnets in these systems. 
    more » « less