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Award ID contains: 1741693

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  1. Recent successful integration of semiconductors into spintronic THz emitters has demonstrated a new pathway of control over terahertz (THz) radiation through ultrafast demagnetization dynamics. Here, the spintronic THz emission from different ultrawide bandgap (UWBG) semiconductors interfaced with ferromagnets is studied. The authors show that the Schottky barrier in the UWBG semiconductor AlN acts as a spin filter that increases the polarization of the spin current injected from the ferromagnet. Furthermore, the authors show that the two-dimensional electron gas at the interface between Al0.25Ga0.75N and GaN enhances the magnitude of the emitted radiation due to the high spin-to-charge conversion efficiency induced by the Rashba effect that results in a hallmark asymmetry in emission amplitude. The results provide a framework for future engineering of semiconducting/ferromagnet heterostructures for ultrafast communications technologies beyond 5G. 
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  3. In recent years, organic dye molecules as photosensitizers have played a significant role in the field of dye-sensitized solar cells. In this context, two primary dihydroindolocarbazole-based organic dyes (sk201 and sk202), which were synthesized recently by Song et al., and three further designed dyes (DMZ1-3) were theoretically investigated based on density functional theory and time-dependent density functional theory. Molecular geometries, absorption spectra, charge transfer, molecular electrostatic potential and nonlinear optical properties were quantificationally studied and visually presented to reveal the relationships between the molecular structures and performances of dyes. The effects of joining the isolated dyes and TiO2 on the molecular absorption spectra and energy levels were analyzed. Moreover, several parameters, such as efficiency of light-harvesting, driving forces of electron regeneration and injection, excited-state lifetime and vertical dipole moment, were calculated to give the multi-angle demonstrations of the photovoltaic performances for these dyes. 
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    Parity-time (PT) symmetry in non-Hermitian optical systems promises distinct optical effects and applications not found in conservative optics. Its counterpart, anti-PT symmetry, subscribes another class of intriguing optical phenomena and implies complementary techniques for exotic light manipulation. Despite exciting progress, so far, anti-PT symmetry has only been realized in bulky systems or with optical gain. Here, we report an on-chip realization of non-Hermitian optics with anti-PT symmetry by using a fully passive, nanophotonic platform consisting of three evanescently coupled waveguides. By depositing a metal film on the center waveguide to introduce strong loss, an anti-PT system is realized. Using microheaters to tune the waveguides’ refractive indices, striking behaviors are observed such as equal power splitting, synchronized amplitude modulation, phase-controlled dissipation, and transition from anti-PT symmetry to its broken phase. Our results highlight exotic anti-Hermitian nanophotonics to be consolidated with conventional circuits on the same chip, whereby valuable chip devices can be created for quantum optics studies and scalable information processing. 
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  6. null (Ed.)
    Parity-time (PT) symmetry in non-Hermitian optical systems promises distinct optical effects and applications not found in conservative optics. Its counterpart, anti-PT symmetry, subscribes another class of intriguing optical phenomena and implies complementary techniques for exotic light manipulation. Despite exciting progress, so far, anti-PT symmetry has only been realized in bulky systems or with optical gain. Here, we report an on-chip realization of non-Hermitian optics with anti- PT symmetry by using a fully passive, nanophotonic platform consisting of three evanescently coupled waveguides. By depositing a metal film on the center waveguide to introduce strong loss, an anti-PT system is realized. Using microheaters to tune the waveguides’ refractive indices, striking behaviors are observed such as equal power splitting, synchronized amplitude modulation, phase-controlled dissipation, and transition from anti-PT symmetry to its broken phase. Our results highlight exotic anti-Hermitian nanophotonics to be consolidated with conventional circuits on the same chip, whereby valuable chip devices can be created for quantum optics studies and scalable information processing. 
    more » « less