More Like this

1. Towards an engineering framework for ultrafast quantum nonlinear optics

   https://doi.org/10.1117/12.2576098  

   Yanagimoto, Ryotatsu; Ng, Edwin; Onodera, Tatsuhiro; Mabuchi, Hideo (March 2021, Ultrafast Phenomena and Nanophotonics XXV)

   Betz, Markus; Elezzabi, Abdulhakem Y. (Ed.)

   The advent of dispersion-engineered and highly nonlinear nanophotonics is expected to open up an all-optical path towards the strong-interaction regime of quantum optics by combining high transverse field confinement with ultra-short-pulse operation. Obtaining a full understanding of photon dynamics in such broadband devices, however, poses major challenges in the modeling and simulation of multimode non-Gaussian quantum physics, highlighting the need for sophisticated reduced models that facilitate efficient numerical study while providing useful physical insight. In this manuscript, we review our recent efforts in modeling broadband optical systems at varying levels of abstraction and generality, ranging from multimode extensions of quantum input-output theory for sync-pumped oscillators to the development of numerical methods based on a field-theoretic description of nonlinear waveguides. We expect our work not only to guide ongoing theoretical and experimental efforts towards next-generation quantum devices but also to uncover essential physics of broadband quantum photonics. 

   more » « less
2. Ultrafast second-order nonlinear photonics—from classical physics to non-Gaussian quantum dynamics: a tutorial

   https://doi.org/10.1364/AOP.495768  

   Jankowski, Marc; Yanagimoto, Ryotatsu; Ng, Edwin; Hamerly, Ryan; McKenna, Timothy P; Mabuchi, Hideo; Fejer, M M (June 2024, Advances in Optics and Photonics)

   Photonic integrated circuits with second-order (χ⁽²⁾) nonlinearities are rapidly scaling to remarkably low powers. At this time, state-of-the-art devices achieve saturated nonlinear interactions with thousands of photons when driven by continuous-wave lasers, and further reductions in these energy requirements enabled by the use of ultrafast pulses may soon push nonlinear optics into the realm of single-photon nonlinearities. This tutorial reviews these recent developments in ultrafast nonlinear photonics, discusses design strategies for realizing few-photon nonlinear interactions, and presents a unified treatment of ultrafast quantum nonlinear optics using a framework that smoothly interpolates from classical behaviors to the few-photon scale. These emerging platforms for quantum optics fundamentally differ from typical realizations in cavity quantum electrodynamics due to the large number of coupled optical modes. Classically, multimode behaviors have been well studied in nonlinear optics, with famous examples including soliton formation and supercontinuum generation. In contrast, multimode quantum systems exhibit a far greater variety of behaviors, and yet closed-form solutions are even sparser than their classical counterparts. In developing a framework for ultrafast quantum optics, we identify what behaviors carry over from classical to quantum devices, what intuition must be abandoned, and what new opportunities exist at the intersection of ultrafast and quantum nonlinear optics. Although this article focuses on establishing connections between the classical and quantum behaviors of devices withχ⁽²⁾nonlinearities, the frameworks developed here are general and are readily extended to the description of dynamical processes based on third-orderχ⁽³⁾nonlinearities. 

   more » « less
3. Nonlinear optics in 2D materials: From classical to quantum

   https://doi.org/10.1063/5.0242014  

   Gu, Liuxin; Zhou, You (March 2025, Applied Physics Reviews)

   Nonlinear optics has long been a cornerstone of modern photonics, enabling a wide array of technologies, from frequency conversion to the generation of ultrafast light pulses. Recent breakthroughs in two-dimensional (2D) materials have opened a frontier in this field, offering new opportunities for both classical and quantum nonlinear optics. These atomically thin materials exhibit strong light–matter interactions and large nonlinear responses, thanks to their tunable lattice symmetries, strong resonance effects, and highly engineerable band structures. In this paper, we explore the potential that 2D materials bring to nonlinear optics, covering topics from classical nonlinear optics to nonlinearities at the few-photon level. We delve into how these materials enable possibilities, such as symmetry control, phase matching, and integration into photonic circuits. The fusion of 2D materials with nonlinear optics provides insights into the fundamental behaviors of elementary excitations—such as electrons, excitons, and photons—in low-dimensional systems and has the potential to transform the landscape of next-generation photonic and quantum technologies. 

   more » « less
4. Temporal trapping: a route to strong coupling and deterministic optical quantum computation

   https://doi.org/10.1364/OPTICA.473276  

   Yanagimoto, Ryotatsu; Ng, Edwin; Jankowski, Marc; Mabuchi, Hideo; Hamerly, Ryan (January 2022, Optica)

   The realization of deterministic photon–photon gates is a central goal in optical quantum computation and engineering. A longstanding challenge is that optical nonlinearities in scalable, room-temperature material platforms are too weak to achieve the required strong coupling, due to the critical loss-confinement trade-off in existing photonic structures. In this work, we introduce a spatio-temporal confinement method, dispersion-engineered temporal trapping, to circumvent the trade-off, enabling a route to all-optical strong coupling. Temporal confinement is imposed by an auxiliary trap pulse via cross-phase modulation, which, combined with the spatial confinement of a waveguide, creates a “flying cavity” that enhances the nonlinear interaction strength by at least an order of magnitude. Numerical simulations confirm that temporal trapping confines the multimode nonlinear dynamics to a single-mode subspace, enabling high-fidelity deterministic quantum gate operations. With realistic dispersion engineering and loss figures, we show that temporally trapped ultrashort pulses could achieve strong coupling on near-term nonlinear nanophotonic platforms. Our results highlight the potential of ultrafast nonlinear optics to become the first scalable, high-bandwidth, and room-temperature platform that achieves strong coupling, opening a path to quantum computing, simulation, and light sources. 

   more » « less
5. Classical-Nonclassical Polarity of Gaussian States

   https://doi.org/10.1103/PhysRevLett.132.240201  

   Liu, Jiru; Ge, Wenchao; Zubairy, M Suhail (June 2024, Physical Review Letters)

   Gaussian states with nonclassical properties such as squeezing and entanglement serve as crucial resources for quantum information processing. Accurately quantifying these properties within multimode Gaussian states has posed some challenges. To address this, we introduce a unified quantification: the “classical-nonclassical polarity,” represented by P. For a single mode, a positive value of P captures the reduced minimum quadrature uncertainty below the vacuum noise, while a negative value represents an enlarged uncertainty due to classical mixtures. For multimode systems, a positive P indicates bipartite quantum entanglement. We show that the sum of the total classical-nonclassical polarity is conserved under arbitrary linear optical transformations for any two-mode and three-mode Gaussian states. For any pure multimode Gaussian state, the total classical-nonclassical polarity equals the sum of the mean photon number from single-mode squeezing and two-mode squeezing. Our results provide a new perspective on the quantitative relation between single-mode nonclassicality and entanglement, which may find applications in a unified resource theory of nonclassical features. 

   more » « less