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The spin structure and transport behavior of B20-ordered CoSi nanomagnets are investigated experimentally and by theoretical calculations. B20 materials are of interest in spin electronics because their noncentrosymmetric crystal structure favors noncoplanar spin structures that yield a contribution to the Hall effect. However, stoichiometric bulk CoSi is nonmagnetic, and combining magnetic order at and above room temperature with small feature sizes has remained a general challenge. Our CoSi nanoclusters have an average size of 11.6 nm and a magnetic ordering temperature of 330 K. First-principle calculations and x-ray circular dichroism experiments show that the magnetic moment is predominantly confined to the shells of the clusters. The CoSi nanocluster ensemble exhibits a topological Hall effect, which is explained by an analytical model and by micromagnetic simulations on the basis of competing Dzyaloshinskii-Moriya and intra- and intercluster exchange interactions. The topological Hall effect is caused by formation of chiral spin textures in the shells of the clusters, which exhibit fractional skyrmion number and are therefore termed as paraskyrmions (closely related to skyrmion spin structures). This research shows how nanostructuring of a chiral atomic structure can create a spin-textured material with a topological Hall effect and a magnetic ordering temperature above room temperature.
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Spin disorder control of topological spin texture
Abstract Stabilization of topological spin textures in layered magnets has the potential to drive the development of advanced low-dimensional spintronics devices. However, achieving reliable and flexible manipulation of the topological spin textures beyond skyrmion in a two-dimensional magnet system remains challenging. Here, we demonstrate the introduction of magnetic iron atoms between the van der Waals gap of a layered magnet, Fe3GaTe2, to modify local anisotropic magnetic interactions. Consequently, we present direct observations of the order-disorder skyrmion lattices transition. In addition, non-trivial topological solitons, such as skyrmioniums and skyrmion bags, are realized at room temperature. Our work highlights the influence of random spin control of non-trivial topological spin textures.
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- PAR ID:
- 10548902
- Author(s) / Creator(s):
- ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; more »
- Publisher / Repository:
- Springer Nature
- Date Published:
- Journal Name:
- Nature Communications
- Volume:
- 15
- Issue:
- 1
- ISSN:
- 2041-1723
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript
- Journal Article:
- https://doi.org/10.1038/s41467-024-47715-5
