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1. Efficient and highly tunable second-harmonic generation in Z-cut periodically poled lithium niobate nanowaveguides

   https://doi.org/10.1364/OL.393445  

   Chen, Jia-Yang ; Tang, Chao ; Ma, Zhao-Hui ; Li, Zhan ; Meng Sua, Yong ; Huang, Yu-Ping ( July 2020 , Optics Letters)

   Thin-film lithium-niobate-on-insulator (LNOI) has emerged as a superior integrated-photonics platform for linear, nonlinear, and electro-optics. Here we combine quasi-phase-matching, dispersion engineering, and tight mode confinement to realize nonlinear parametric processes with both high efficiency and wide wavelength tunability. On a millimeter-long, Z-cut LNOI waveguide, we demonstrate efficient ($1900\pm <\#comment/>500\mathrm{\%<\#comment/>}{\mathrm{W}}^{-<\#comment/>1}{\mathrm{c}\mathrm{m}}^{-<\#comment/>2}$) and highly tunable ($-<\#comment/>1.71\mathrm{n}\mathrm{m}/\mathrm{K}$) second-harmonic generation from 1530 to 1583 nm by type-0 quasi-phase-matching. Our technique is applicable to optical harmonic generation, quantum light sources, frequency conversion, and many other photonic information processes across visible to mid-IR spectral bands.

    

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2. Broadband ultraviolet-visible frequency combs from cascaded high-harmonic generation in quasi-phase-matched waveguides

   https://doi.org/10.1364/JOSAB.427086  

   Rutledge, Jay ; Catanese, Anthony ; Hickstein, Daniel D. ; Diddams, Scott A. ; Allison, Thomas K. ; Kowligy, Abijith S. ( July 2021 , Journal of the Optical Society of America B)

   High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to the ninth order (333 nm) in chirped periodically poled lithium niobate waveguides driven by phase-stable$\le <\#comment/>12\mathrm{n}\mathrm{J}$, 100 fs pulses at 3 µm with 100 MHz repetition rate. A mid-infrared to ultraviolet-visible conversion efficiency as high as 10% is observed, among an overall 23% conversion of the fundamental to all harmonics. We verify the coherence of the harmonic frequency combs despite the complex highly nonlinear process. Accommodating the extreme spectral bandwidth, numerical simulations based on a single broadband envelope equation with only quadratic nonlinearity give estimates for the conversion efficiency within approximately 1 order of magnitude over a wide range of experimental parameters. From this comparison between theory and experiment, we identify a dimensionless parameter capturing the competition between three-wave mixing and group-velocity walk-off of the harmonics that governs the cascaded HHG physics. We also gain insights into spectral optimization via tuning the waveguide poling profile and pump pulse parameters. These results can inform cascaded HHG in a range of different platforms.

    

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3. Mid-IR spectroscopy of Er 3+ doped low-phonon CsCdCl 3 and CsPbCl 3 crystals

   https://doi.org/10.1364/JOSAB.470152  

   Brown, Ei Ei ; Fleischman, Zackery D. ; McKay, Jason ; Hommerich, Uwe ; Kabir, Al Amin ; Riggins, Jazmine ; Trivedi, Sudhir ; Dubinskii, Mark ( September 2022 , Journal of the Optical Society of America B)

   The mid-IR spectroscopic properties of${\mathrm{E}\mathrm{r}}^{3+}$doped low-phonon${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$crystals grown by the Bridgman technique have been investigated. Using optical excitations at$\sim <\#comment/>800\mathrm{n}\mathrm{m}$and$\sim <\#comment/>660\mathrm{n}\mathrm{m}$, both crystals exhibited IR emissions at$\sim <\#comment/>1.55$,$\sim <\#comment/>2.75$,$\sim <\#comment/>3.5$, and$\sim <\#comment/>4.5\text{µ<\#comment/>}\mathrm{m}$at room temperature. The mid-IR emission at 4.5 µm, originating from the${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition, showed a long emission lifetime of$\sim <\#comment/>11.6\mathrm{m}\mathrm{s}$for${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$, whereas${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$exhibited a shorter lifetime of$\sim <\#comment/>1.8\mathrm{m}\mathrm{s}$. The measured emission lifetimes of the${}^4{\mathrm{I}}_{9/2}$state were nearly independent of the temperature, indicating a negligibly small nonradiative decay rate through multiphonon relaxation, as predicted by the energy-gap law for low-maximum-phonon energy hosts. The room temperature stimulated emission cross sections for the${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition in${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$were determined to be$\sim <\#comment/>0.14\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$and$\sim <\#comment/>0.41\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$, respectively. The results of Judd–Ofelt analysis are presented and discussed.

    

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4. Spectrally simplified approach for leveraging legacy geostationary oceanic observations

   https://doi.org/10.1364/AO.465491  

   Houskeeper, Henry F. ; Hooker, Stanford B. ; Cavanaugh, Kyle C. ( September 2022 , Applied Optics)

   The use of multispectral geostationary satellites to study aquatic ecosystems improves the temporal frequency of observations and mitigates cloud obstruction, but no operational capability presently exists for the coastal and inland waters of the United States. The Advanced Baseline Imager (ABI) on the current iteration of the Geostationary Operational Environmental Satellites, termed the$R$Series (GOES-R), however, provides sub-hourly imagery and the opportunity to overcome this deficit and to leverage a large repository of existing GOES-R aquatic observations. The fulfillment of this opportunity is assessed herein using a spectrally simplified, two-channel aquatic algorithm consistent with ABI wave bands to estimate the diffuse attenuation coefficient for photosynthetically available radiation,$K_d(\mathrm{P}\mathrm{A}\mathrm{R})$. First, anin situABI dataset was synthesized using a globally representative dataset of above- and in-water radiometric data products. Values of$K_d(\mathrm{P}\mathrm{A}\mathrm{R})$were estimated by fitting the ratio of the shortest and longest visible wave bands from thein situABI dataset to coincident,in situ$K_d(\mathrm{P}\mathrm{A}\mathrm{R})$data products. The algorithm was evaluated based on an iterative cross-validation analysis in which 80% of the dataset was randomly partitioned for fitting and the remaining 20% was used for validation. The iteration producing the median coefficient of determination ($R^2$) value (0.88) resulted in a root mean square difference of$0.319{\mathrm{m}}^{-<\#comment/>1}$, or 8.5% of the range in the validation dataset. Second, coincident mid-day images of central and southern California from ABI and from the Moderate Resolution Imaging Spectroradiometer (MODIS) were compared using Google Earth Engine (GEE). GEE default ABI reflectance values were adjusted based on a near infrared signal. Matchups between the ABI and MODIS imagery indicated similar spatial variability ($R^2=0.60$) between ABI adjusted blue-to-red reflectance ratio values and MODIS default diffuse attenuation coefficient for spectral downward irradiance at 490 nm,$K_d(490)$, values. This work demonstrates that if an operational capability to provide ABI aquatic data products was realized, the spectral configuration of ABI would potentially support a sub-hourly, visible aquatic data product that is applicable to water-mass tracing and physical oceanography research.

    

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5. Efficient second-harmonic generation in high Q-factor asymmetric lithium niobate metasurfaces

   https://doi.org/10.1364/OL.413764  

   Kang, Lei ; Bao, Huaguang ; Werner, Douglas H. ( January 2021 , Optics Letters)

   Lithium niobate (LN) has been widely used for second-harmonic generation (SHG) from bulk crystals. Recent studies have reported improved SHG efficiency in LN micro-ring resonators and hybrid waveguiding structures, as well as in LN nanostructures supporting anapole modes and plasmon-assisted dipole resonances. Here we numerically demonstrate that high$Q$-factor resonances associated with symmetry-protected bound states in the continuum can lead to highly efficient frequency doubling in LN metasurfaces. Simulations show that the radiative$Q$-factor and on-resonance field enhancement factor observed in the metasurface are closely dependent on the asymmetric parameter$\mathrm{\alpha <\#comment/>}$of the system. Furthermore, high$Q$-factor resonances boost the SH conversion process in the LN nanostructures. In particular, for a LN metasurface with a$Q$-factor of$\sim <\#comment/>8\times <\#comment/>{10}^4$, a 0.49% peak SH conversion efficiency is achieved at a pump intensity of$3.3{\mathrm{k}\mathrm{W}/\mathrm{c}\mathrm{m}}^2$. This suggests that such high$Q$-factor LN metasurfaces may be good candidates for practical blue–ultraviolet light sources. Our work provides insight into the possible implementation of metadevices based on nanoengineering of conventional nonlinear crystals.

    

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