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1. Electro-optic interface for ultrasensitive intracavity electric field measurements at microwave and terahertz frequencies

   https://doi.org/10.1364/OPTICA.384160  

   Benea-Chelmus, Ileana-Cristina ; Salamin, Yannick ; Settembrini, Francesca_Fabiana ; Fedoryshyn, Yuriy ; Heni, Wolfgang ; Elder, Delwin_L ; Dalton, Larry_R ; Leuthold, Juerg ; Faist, Jérôme ( May 2020 , Optica)

   Electro-optic quantum coherent interfaces map the amplitude and phase of a quantum signal directly to the phase or intensity of a probe beam. At terahertz frequencies, a fundamental challenge is not only to sense such weak signals (due to a weak coupling with a probe in the near-infrared) but also to resolve them in the time domain. Cavity confinement of both light fields can increase the interaction and achieve strong coupling. Using this approach, current realizations are limited to low microwave frequencies. Alternatively, in bulk crystals, electro-optic sampling was shown to reach quantum-level sensitivity of terahertz waves. Yet, the coupling strength was extremely weak. Here, we propose an on-chip architecture that concomitantly provides subcycle temporal resolution and an extreme sensitivity to sense terahertz intracavity fields below 20 V/m. We use guided femtosecond pulses in the near-infrared and a confinement of the terahertz wave to a volume of$V_{\mathrm{T}\mathrm{H}\mathrm{z}}\sim <\#comment/>{10}^{-<\#comment/>9}({\mathrm{\lambda <\#comment/>}}_{\mathrm{T}\mathrm{H}\mathrm{z}}/2{)}^3$in combination with ultraperformant organic molecules ($r_{33}=170\mathrm{p}\mathrm{m}/\mathrm{V}$) and accomplish a record-high single-photon electro-optic coupling rate of$g_{\mathrm{e}\mathrm{o}}=2\mathrm{\pi <\#comment/>}\times <\#comment/>0.043\mathrm{G}\mathrm{H}\mathrm{z}$, 10,000 times higher than in recent reports of sensing vacuum field fluctuations in bulk media. Via homodyne detection implemented directly on chip, the interaction results into an intensity modulation of the femtosecond pulses. The single-photon cooperativity is$C_0=1.6\times <\#comment/>{10}^{-<\#comment/>8}$, and the multiphoton cooperativity is$C=0.002$at room temperature. We show$><\#comment/>70\mathrm{d}\mathrm{B}$dynamic range in intensity at 500 ms integration under irradiation with a weak coherent terahertz field. Similar devices could be employed in future measurements of quantum states in the terahertz at the standard quantum limit, or for entanglement of subsystems on subcycle temporal scales, such as terahertz and near-infrared quantum bits.

    

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2. Mid-IR spectroscopy of Er 3+ doped low-phonon CsCdCl 3 and CsPbCl 3 crystals

   https://doi.org/10.1364/JOSAB.470152  

   Brown, Ei_Ei ; Fleischman, Zackery_D ; McKay, Jason ; Hommerich, Uwe ; Kabir, Al_Amin ; Riggins, Jazmine ; Trivedi, Sudhir ; Dubinskii, Mark ( September 2022 , Journal of the Optical Society of America B)

   The mid-IR spectroscopic properties of${\mathrm{E}\mathrm{r}}^{3+}$doped low-phonon${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$crystals grown by the Bridgman technique have been investigated. Using optical excitations at$\sim <\#comment/>800\mathrm{n}\mathrm{m}$and$\sim <\#comment/>660\mathrm{n}\mathrm{m}$, both crystals exhibited IR emissions at$\sim <\#comment/>1.55$,$\sim <\#comment/>2.75$,$\sim <\#comment/>3.5$, and$\sim <\#comment/>4.5\text{µ<\#comment/>}\mathrm{m}$at room temperature. The mid-IR emission at 4.5 µm, originating from the${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition, showed a long emission lifetime of$\sim <\#comment/>11.6\mathrm{m}\mathrm{s}$for${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$, whereas${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$exhibited a shorter lifetime of$\sim <\#comment/>1.8\mathrm{m}\mathrm{s}$. The measured emission lifetimes of the${}^4{\mathrm{I}}_{9/2}$state were nearly independent of the temperature, indicating a negligibly small nonradiative decay rate through multiphonon relaxation, as predicted by the energy-gap law for low-maximum-phonon energy hosts. The room temperature stimulated emission cross sections for the${}^4{\mathrm{I}}_{9/2}\to <\#comment/>{}^4{\mathrm{I}}_{11/2}$transition in${\mathrm{E}\mathrm{r}}^{3+}$doped${\mathrm{C}\mathrm{s}\mathrm{C}\mathrm{d}\mathrm{C}\mathrm{l}}_3$and${\mathrm{C}\mathrm{s}\mathrm{P}\mathrm{b}\mathrm{C}\mathrm{l}}_3$were determined to be$\sim <\#comment/>0.14\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$and$\sim <\#comment/>0.41\times <\#comment/>{10}^{-<\#comment/>20}{\mathrm{c}\mathrm{m}}^2$, respectively. The results of Judd–Ofelt analysis are presented and discussed.

    

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3. Resonance tuning for dynamic Huygens metasurfaces

   https://doi.org/10.1364/JOSAB.427848  

   Ollanik, Adam_J ; Oguntoye, Isaac ; Ji, Yaping ; Escarra, Matthew_D ( July 2021 , Journal of the Optical Society of America B)

   Metasurfaces with dynamic optical performance have the potential to enable a broad range of applications. We computationally investigate the potential of dielectric Huygens metasurfaces, supporting both electric and magnetic dipole resonances, as a candidate platform for dynamic tuning. The asymmetric response of the two dipole resonances to changes in geometric and material parameters, and the potential for separate control of amplitude and phase, is analyzed. A review of dynamic materials, and their promise and limitations for use in dynamic Huygens metasurfaces, is discussed. Vanadium dioxide (${\mathrm{V}\mathrm{O}}_2$) is recognized as a singularly interesting material, due to its variable refractive index and optical absorption in response to several stimuli. Transmitted phase modulation of$\pm <\#comment/>\mathrm{\pi <\#comment/>}$is computationally demonstrated as a function of decaying resonance utilizing only the first 5% of the insulator-metal transition, corresponding to a temperature change of$<<\#comment/>{10}^{\circ <\#comment/>}\mathrm{C}$. As another case study utilizing asymmetric resonance tuning in response to changing incidence angle, phase modulation ($2\mathrm{\pi <\#comment/>}$range for reflected light and$><\#comment/>1.5\mathrm{\pi <\#comment/>}$for transmitted light) and amplitude modulation (from$\mathrm{R}=1$to$\mathrm{T}=1$) are demonstrated using a simple silicon metasurface with varying incident angle within a range of$\sim <\#comment/>{15}^{\circ <\#comment/>}$on two axes. A promising implementation within a micro-electromechanical system (MEMS)-based spatial light modulator, similar to conventional digital micromirror devices, is discussed.

    

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4. Bell state analyzer for spectrally distinct photons

   https://doi.org/10.1364/OPTICA.443302  

   Lingaraju, Navin_B ; Lu, Hsuan-Hao ; Leaird, Daniel_E ; Estrella, Steven ; Lukens, Joseph_M ; Weiner, Andrew_M ( March 2022 , Optica)

   We demonstrate a Bell state analyzer that operates directly on frequency mismatch. Based on electro-optic modulators and Fourier-transform pulse shapers, our quantum frequency processor design implements interleaved Hadamard gates in discrete frequency modes. Experimental tests on entangled-photon inputs reveal fidelities of$\sim <\#comment/>98\mathrm{\%<\#comment/>}$for discriminating between the$|{\mathrm{\Psi <\#comment/>}}^{+}⟩<\#comment/>$and$|{\mathrm{\Psi <\#comment/>}}^{-<\#comment/>}⟩<\#comment/>$frequency-bin Bell states. Our approach resolves the tension between wavelength-multiplexed state transport and high-fidelity Bell state measurements, which typically require spectral indistinguishability.

    

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5. InGaP quantum nanophotonic integrated circuits with 1.5% nonlinearity-to-loss ratio

   https://doi.org/10.1364/OPTICA.440383  

   Zhao, Mengdi ; Fang, Kejie ( February 2022 , Optica)

   Optical nonlinearity plays a pivotal role in quantum information processing using photons, from heralded single-photon sources and coherent wavelength conversion to long-sought quantum repeaters. Despite the availability of strong dipole coupling to quantum emitters, achieving strong bulk optical nonlinearity is highly desirable. Here, we realize quantum nanophotonic integrated circuits in thin-film InGaP with, to our knowledge, a record-high ratio of$1.5\mathrm{\%<\#comment/>}$between the single-photon nonlinear coupling rate ($g/2\mathrm{\pi <\#comment/>}=11.2\mathrm{M}\mathrm{H}\mathrm{z}$) and cavity-photon loss rate. We demonstrate second-harmonic generation with an efficiency of$71200\pm <\#comment/>10300\mathrm{\%<\#comment/>}/\mathrm{W}$in the InGaP photonic circuit and photon-pair generation via degenerate spontaneous parametric downconversion with an ultrahigh rate exceeding 27.5 MHz/µW—an order of magnitude improvement of the state of the art—and a large coincidence-to-accidental ratio up to$1.4\times <\#comment/>{10}^4$. Our work shows InGaP as a potentially transcending platform for quantum nonlinear optics and quantum information applications.

    

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